Actively Tunable Fano Resonance Based on a T-Shaped Graphene Nanodimer

We present the strength modulation and frequency tuning of Fano resonance by employing a graphene nanodimer formed by two coplanar perpendicular nanostrips with different dimensions. The Fano resonance is induced by destructive interference between the bright dipole mode of a short nanostrip and the dark quadrupole mode of a long nanostrip. The strength, line width, and resonance frequency of the Fano resonance can be actively modulated by changing the spatial separation of those two graphene nanostrips and the Fermi energy of the graphene nanodimer, respectively, without re-fabricating the nanostructures. The tuning of the strength and resonance frequency can be attributed to the coupling strength and optical properties of graphene, respectively. Importantly, a figure of merit value as high as 39 is achieved in the proposed nanostructures. Our results may provide potential applications in optical switching and bio-chemical sensing.     

Magneto-Electric Double Fano Resonances in Hybrid Split Ring/Disk Hetero-Cavity

In this work, we conceive and demonstrate the magneto-electric double Fano resonances of a hetero-cavity composed of Si disk and Au split ring, where Si disk can provide additional magnetic responses besides electric responses. The interference between electric and magnetic responses in proposed hetero-cavity gives rise to magneto-electric double Fano resonances with magnetic and electric near-field enhancements. Dipole radiative enhancement is used to analyze magnetic and electric responses of hetero-cavity and the spectral features of hetero-cavity can be used to quantitatively characterize by coupled oscillator model. And the spectral tunability of magneto-electric double Fano resonances is investigated, highlighting a potential for applications in low-loss sensing and nanophotonic devices.     

Designing Commensurate and Incommensurate Resonances for Enhanced Dipole Emission in Coupled Plasmonic Nanorods

Plasmonic nanorods and their clusters are the fundamental units in plasmonic nanoantenna engineering. A theory that can predict the resonance of single nanorod already exists but is in lack for a heterodimer. Here, we propose a model combining the effective circuit theory for the response of spherical nanoparticles together with standard transmission line theory for hemispherically capped nanorod antennas. The resonances of multiple orders are predictable by defining the reflection phase at the terminals of such antennas, in both symmetric and asymmetric coupled nanorods. The theoretical results compare favorably with full-wave finite element numerical calculations. By the analytical formula, it is easy to control the length of the antennas for regulating the cooperative resonant properties and consequently the radiation characteristics of a nearby electric dipole. Consequently, we obtain both commensurate and incommensurate resonance features in such nanorod-based heterodimer antennas, showing respectively cumulative and selective responses from the individual nanorods.     

Generation of Multiple Fano Resonances in Plasmonic Split Nanoring Dimer

We present a computational study of the plasmonic response of a split nanoring dimer resonator which supports multiple plasmonic Fano-like resonances that arises by the coupling and interference of the dimer plasmon modes. For the generation of Fano resonances with large modulation depths, numerous configurations of the dimer resonator are analyzed which are observed to be highly dependent on the polarization of incident light. Moreover, the influence of dimension of the split nanoring structure on the spectral positions and intensities of the higher order Fano resonances are also investigated, and it is found that the asymmetric Fano line shapes can be flexibly tuned in the spectrum by varying various geometrical parameters. Such Fano resonators are also discovered to offer high values of figure of merit and contrast ratio due to which they are suitable for high-performance biological sensors.     

Electromagnetically Induced Transparency and Sharp Asymmetric Fano Line Shapes in All-Dielectric Nanodimer

Low-loss electromagnetically induced transparency (EIT) and asymmetric Fano line shapes are investigated in a simple planar silicon dimer resonator. The EIT and Fano effects emerge due to near-field coupling of the modes supported by both the nanoparticles in a dimer structure. Different configurations of the dimer nanostructure are analyzed, which provide distinct EIT and Fano resonances. Furthermore, the tunability of EIT and Fano resonant modes are incorporated by changing the structural parameters. It is also found that the dimer resonator exhibits high Q factor and large electromagnetic field enhancement at Fano resonance and EIT window due to extremely low absorption loss. Such values and narrow resonances are supposed to be useful highly sensitive sensors and slow-light applications.     

Excitation of Multiple Fano-Like Resonances Induced by Higher Order Plasmon modes in Three-Layered Bimetallic Nanoshell Dimer

The presence of plasmonic Fano-like resonances in the optical response of isolated and dimer metal-dielectric-metal nanostructures are investigated theoretically. The nanostructures are engineered in such a way to support multiple Fano-like resonances that are induced by the interference of bright and dark plasmon modes. It is found that the dimer resonators exhibit different types of Fano resonances for both the transverse and longitudinal polarizations unlike conventional nanodimers. Several configurations of the dimer Fano resonator are analyzed with special emphasis on the Fano spectral line shape. Breaking the symmetry of the dimer nanostructure in various directions control the asymmetric line shape and provides different kinds of unique Fano resonances. In certain cases, the Fano resonators exhibit multiple Fano resonances that are particularly significant for plasmon line shaping and can serve as platforms for multi-wavelength sensing applications.     

Tunable Multi-Fano Resonances in MDM-Based Side-Coupled Resonator System and its Application in Nanosensor

In this paper, two Fano resonances are achieved in the proposed plasmonic system. Theoretical analysis and simulation results show that two discrete states coupled with a continua lead to these Fano resonances. The discrete states are provided by the side-coupled square cavity, and a baffle plate placed in metal-dielectric-metal waveguide is used to produce a continuous transmission spectrum. The resonant wavelengths and the linewidth of these Fano resonances can be easily tuned by adjusting the parameters of system. This system exhibits high sensitivities as high as 850 and 1120 nm/RIU corresponding to two Fano resonances, and the figure of merit can reach to 1.7 × 10⁵ by optimizing the system. By introducing another square cavity, four Fano resonances are obtained which originate from four discrete states coupled with continua, and they can be tuned independently. The flexible multi-Fano resonances system has significant application bio-nanosensor, nonlinear, and slow light devices.     

All-Optical Strong Coupling Switches Based on a Coupled Meta-atom and MIM Nanocavity Configuration

Based on a coupled meta-atom and metal-nonlinear dielectric-metal nanocavity, nonlinear all-optical strong coupling switches are proposed and numerically investigated. In the absence of the external pumping light, the resonances of the meta-atom are continuously tuned across the one of the nanocavity by changing the size of the meta-atom. The meta-atomic electric dipole and quadrupole interaction with the plasmonic nanocavity is obtained. The characteristic anticrossing behaviors manifest the occurrence of the strong coupling. With the resonance of the meta-atom being tuned to the one of the nanocavity, we dynamically tune the coupled strength of the system by changing intensity (power) of the pumping light and realize the transition from the strong coupling regime to the weak one. This means that this system can be used as an on/off switch in which the strong coupling can be on/off with an external control light, and the on/off states correspond to strong/weak coupling regime, respectively. Such a strong coupling all-optical switching is of considerable interest for applications in nanoscale plasmonic circuits.     

Tunable Fano Resonances in Mid-Infrared Waveguide-Coupled Otto Configuration

A planar silicon carbide/dielectric multilayer structure is investigated in Otto geometry, where surface phonon polaritons and planar waveguide mode can be coupled to realize Fano resonances under transverse magnetic polarization. The resonance coupling is analytically demonstrated using the coupled harmonic oscillator model and numerically presented through rigorous coupled-wave analysis calculations, which shows that the coupling strength between different resonances and the resonant wavelength matching condition plays an important role in the bandwidth and position of the Fano resonance (FR); the magnetic field distribution was also shown to explain the origin of FRs qualitatively.

     

Higher Order Tunable Fano Resonances in Multilayer Nanocones

We present a computational study of the plasmonic response of a gold–silica–gold multilayered nanostructure based on truncated nanocones. Symmetry breaking is introduced by rotating the nanostructure and by offsetting the layers. Nanocones with coaxial multilayers show dipole–dipole Fano resonances with resonance frequencies depending on the polarization of the incident light, which can be changed by rotating the nanostructure. By breaking the axial symmetry, plasmonic modes of distinct angular momenta are strongly mixed, which provide a set of unique and higher order tunable Fano resonances. The plasmonic response of the multilayered nanocones is compared to that of multishell nanostructures with the same volume and the former are discovered to render visible high-order dark modes and to provide sharp tunable Fano resonances. In particular, higher order tunable Fano resonances arising in non-coaxial multilayer nanocones can vary the plasmon lines at various spectral regions simultaneously, which makes these nanostructures greatly suitable for plasmon line shaping both in the extinction and near field spectra.     

Ultra-high Sensitivity Plasmonic Nanosensor Based on Multiple Fano Resonance in the MDM Side-Coupled Cavities

We propose a compact plasmonic structure comprising a metal-dielectric-metal (MDM) waveguide coupled with a side cavity and groove resonators. The proposed system is investigated by the finite element method. Simulation results show that the side-coupled cavity supports a local discrete state and the groove provides a continuous spectrum, the interaction between them, gives rise to the Fano resonance. The asymmetrical line shape and the resonant wavelength can be easily tuned by changing the geometrical parameters of the structure. Moreover, we can extend this plasmonic structure by the double side-coupled cavities to gain the multiple Fano resonances. The proposed structure can serve as an excellent plasmonic sensor with a sensitivity of ～1900 nm/RIU and a figure of merit of about ～3.8?×?10⁴, which can find wide applications for nanosensors.     

Förster Energy Transfer in the Vicinity of Two Metallic Nanospheres (Dimer)

We present a detailed theoretical analysis of the Förster energy transfer process when a pair of molecules (donor and acceptor) is located nearby a cluster of two metallic nanospheres (dimer). We consider the case in which plasmonic resonances are within the overlap between the donor emission and acceptor absorption spectra, as well as the case that excludes such resonances from the aforementioned spectral overlap. Moreover, we explore the dependence of the Förster energy transfer rate on different dimer configurations (size and separation of nanospheres) and several dipole orientations of molecules. The dimer perturbs strongly the Förster energy transfer rate when plasmons are excited, donor dipole is oriented along the longitudinal axis of the dimer, and the radii of nanospheres and the sphere-gap distance are on the order of a few nanometers. In case of plasmonic excitation, the Förster energy transfer rate is degraded as the sphere-gap distance and size of the nanoparticles increase due to the dephasing of electronic motion arising from ohmic losses of metal. Also, we study the Förster efficiency influenced by the dimer, finding that the high efficiency region (delimited by the Förster radius curve) is reduced as a consequence of significant enhancement of the direct donor decay rate. Our study could impact applications that involve Förster energy transfer.     

Decorated Core-Shell Architectures: Influence of the Dimensional Properties on Hybrid Resonances

Emerging nanoplasmonics utilizing asymmetric core-shell architectures present opportunities to precisely control the plasmon position and signal amplification within a single particle. In particular, asymmetric gold nanorods, assembled into a “matryoshka” structure (gold nanorod core, silica spacer shell, and outer gold shell) have the unique ability to enhance and precisely manipulate the plasmonic signature when compared to single gold nanorods via the generation of hybridized plasmonic modes. Currently, the fundamental understanding of the impact of the gold nanorod matryoshka dimensional parameters on the subsequent resonance behavior is incomplete. In this work, we elucidate the structural-hybridized resonance relationship of gold nanorod nanomatryoshka designs by experimentally varying the key geometrical properties; including silica spacer thickness, gold nanorod core size, and gold shell thickness/continuity.     

Structure of Multiple Fano Resonances in Double-baffle MDM Waveguide Coupled Cascaded Square Cavity for Application of High Throughput Detection

A structure of double-baffle metal-dielectric-metal (MDM) waveguide coupled cascaded square cavity is designed based on the transmission characteristics of the surface plasmon polaritons. Combined with coupled mode theory (CMT), the mechanism of multiple Fano resonances generated by this structure is analyzed qualitatively. The wide-band spectrum mode generated by the F-P resonant cavity and the four narrow-band spectrum modes produced by the cascaded square resonant cavities interfere with each other. Moreover, an new scheme of introducing a semiconductor material InGaAsP into this structure is designed for improving the transmittance of the Fano peaks. Analyze the influence of refractive indexes of the test objects on sensing performance by finite element method (FEM) quantitatively, which shows the improved structure can achieve the independent tuning of multiple Fano resonances. Combining with 96-well microplate technology, the structure can achieve the detection of multiple different samples with high-performance simultaneously. It is believed that the proposed structure has a strong reference significance for the design of optical micro-nanostructures for high throughput detection.

     

High-Q Fano Resonances in Asymmetric and Symmetric All-Dielectric Metasurfaces

We present high-quality (high-Q) Fano resonances in all-dielectric metasurfaces consisting of a periodic array of air holes on silicon (Si) film, deposited on the top of quartz substrate. With the control of the radius difference Δr and center distance Δd between the air holes, two asymmetric all-dielectric metasurfaces are proposed to achieve extremely high-Q Fano resonances. Numerical method with finite difference time domain and equivalent circuit model is employed to analyse the excitation mechanism of the sharp Fano resonances. It is shown that the high-Q Fano resonances come from the interference of two Fabry-Perot resonances, resulting in an extremely narrow window. Moreover, we also demonstrate that the high-Q Fano resonances can also be realized as electromagnetic wave is obliquely incident on the symmetric all-dielectric metasurface. Finally, we show the high-Q Fano resonances caused by asymmetric configurations can coexist with the Fano resonances in the symmetric configuration induced by oblique incidence. As a result, a tri-band Fano resonance is obtained. It is expected that our results will provide important mechanisms for tuning and switching a wide variety of optical devices such as angular sensors, filters, switches, and modulators.     

Controllable Coupling of Localized and Propagating Surface Plasmons to Tamm Plasmons

We theoretically investigate the coupling between Tamm plasmons and localized surface plasmons (LSPs) as well as propagating surface plasmons (PSPs) in a multilayer structure consisting of a metallic nanowire array and a spatially separated metal–dielectric Bragg reflector (DBR). A clear anticrossing behavior of the resonances is observed in the dispersion diagram resulting from the coupling, which is well explained by the coupled oscillator model. The coupling also creates new hybrid LSP or PSP modes with narrow bandwidths and unique spectral features. Upon the excitation of these hybrid modes, the local fields underneath the nanowires for the hybrid LSPs or near the lower metal layer surface for the hybrid PSPs are both enhanced greatly as compared with those achieved in the structure without DBR, which has potential applications in nonlinear optics and surface-enhanced spectroscopies.     

Single-Particle Spectroscopy of Supported Silver Clusters on Silicon: Substrate Effects on Localized Surface Plasmons

The presence of a surrounding medium strongly affects the spectral properties of localized surface plasmons at metallic nanoparticles. Vice versa, plasmonic resonances have large impact on the electric polarization in a surrounding or supporting material. For applications, e.g., in light-converting devices, the coupling of localized surface plasmons with polarizations in semiconducting substrates is of particular importance. Using photoemission electron microscopy with tunable laser excitation, we perform single-particle spectroscopy of silver nanoclusters directly grown on Si(100). Two distinct localized surface plasmon modes are observed as resonances in the two-photon photoemission signals from individual silver clusters. The strengths of these resonances strongly depend on the polarization of the exciting electric field, which allows us to assign them to plasmon modes with polarizations parallel and perpendicular, respectively, to the supporting silicon substrate. Our mode assignment is supported by simulations which provide insight into the mutual interaction of charge oscillations at the particle surface with electric polarizations at the silver/silicon interface.

     

Subradiant,Superradiant Plasmon Modes and Fano Resonance in a Multilayer Nanocylinder Array Standing on a Thin Metal Film

The optical properties of a novel nanostructure consisting of a hexagonal array of aligned vertically three-layered metal-dielectric-metal nanodisks on a silver film are theoretically studied through the finite-difference time-domain method. The novel nanostructure exhibits three obvious optical transmission bands due to the excitation of subradiant plasmon modes, superradiant plasmon modes, and Fano resonances. Surface plasmon polaritons of the underlying Ag film also play a significant role on these three optical transmission bands via coupling with localized surface plasmons of nanodisk pairs. Moreover, the nanostructure also exhibits a good tunability of optical response by modifying the sizes of cylinders, the thickness of underlying metal film, and the dielectric constant of middle layer. These results demonstrate the nanostructure with great advantages in optical sensors and filters.

     

Enhancing Diamond Fluorescence via Optimized Nanorod Dimer Configurations

Light extraction from silicon (SiV) and nitrogen (NV) vacancy diamond color centers coupled to plasmonic silver and gold nanorod dimers was numerically improved. Numerical optimization of the coupled dipolar emitter—plasmonic nanorod dimer configurations was realized to attain the highest possible fluorescence enhancement by simultaneously improving the color centers excitation and emission through antenna resonances. Conditional optimization was performed by setting a criterion regarding the minimum quantum efficiency of the coupled system (cQE) to minimize losses. By comparing restricted symmetric and allowed asymmetric dimers, the advantages of larger degrees of freedom achievable in asymmetric configurations was proven. The highest 2.59?×?10⁸ fluorescence enhancement was achieved with 46.08% cQE via NV color center coupled to an asymmetric silver dimer. This is 3.17-times larger than the 8.19?×?10⁷ enhancement in corresponding symmetric silver dimer configuration, which has larger 68.52% cQE. Among coupled SiV color centers the highest 1.04?×?10⁸ fluorescence enhancement was achieved via asymmetric silver dimer with 37.83% cQE. This is 1.06-times larger than the 9.83?×?10⁷ enhancement in corresponding symmetric silver dimer configuration, which has larger 57.46% cQE. Among gold nanorod coupled configurations the highest fluorescence enhancement of 4.75?×?10⁴ was shown for SiV color center coupled to an asymmetric dimer with 21.8% cQE. The attained enhancement is 8.48- (92.42-) times larger than the 5.6?×?10³ (5.14?×?10²) fluorescence enhancement achievable via symmetric (asymmetric) gold nanorod dimer coupled to SiV (NV) color center, which is accompanied by 16.01% (7.66%) cQE.     

Ultra-High Sensitivity Nanosensor Based on Multiple Fano Resonance in the MIM Coupled Plasmonic Resonator

This paper proposes a compact plasmonic structure that is composed of a metal-insulator-metal (MIM) waveguide coupled with a groove and stub resonators, and then investigates it by utilizing the finite element method (FEM). Simulation results show that the interaction between the local discrete state caused by the stub resonator and the continuous spectrum caused by the groove resonator gives rise to one of the two Fano resonances, while the generation of the other resonance relies only on the groove. Meanwhile, the asymmetrical linear shape and the resonant wavelength can be easily tuned by changing the parameters of the structure. By adding stubs on the groove, we excited multiple Fano resonances. The proposed structure can serve as an excellent plasmonic sensor with a sensitivity of 2000 nm/RIU and a figure of merit of about 3.04?×?10³, which can find extensive applications for nanosensors.