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Natural radioactivity concentrations of 226Ra, 232Th,and 40K in commercial building materials and their lifetime cancer risk assessment in dwellers
Authors:Omeje M.  Adewoyin O. Olusegun  Emmanuel S. Joel  Ehi-Eromosele C. O  Emenike C. PraiseGod  Usikalu M. R.
Affiliation:1. Department of Physics, College of Science and Technology, Covenant University, Ota, Ogun State, Nigeriamaxwell.omeje@covenantuniversity.edu.ng"ORCIDhttp://orcid.org/0000-0001-9124-1093;2. Department of Physics, College of Science and Technology, Covenant University, Ota, Ogun State, Nigeria;3. Department of Chemistry, College of Science and Technology, Covenant University, Ota, Ogun State, Nigeria;4. Department of Civil Engineering, College of Engineering, Covenant University, Ota, Ogun State, Nigeria"ORCIDhttp://orcid.org/0000-0001-6778-6413;5. Department of Physics, College of Science and Technology, Covenant University, Ota, Ogun State, Nigeria"ORCIDhttp://orcid.org/0000-0003-2233-4055
Abstract:Elevated radioactivity levels of 226Ra, 232Th, and 40K in building materials were measured using gamma-ray spectrometry and their associated lifetime cancer risks were also determined. The mean activity concentrations of 226Ra, 232Th, and 40K are 45.72 ± 0.55, 65.90 ± 8.89, and 487.32 ± 15.20 Bq kg?1, respectively. Statistically, the principal component (PC) analysis indicates that higher loadings were recorded in Principal Component One (PC1) with large contribution from 232Th and 40K. The leverage studies indicate that BN Ceramics (BNC) contributes more to the loadings in PC1 followed by Golden Crown Ceramic (GCC) sample. The mean values of 0.399 mSv y?1 do not surpass the world average value of 0.7 mSv y?1. The mean gamma index from the measured samples is 0.644, whereas a mean value of 0.271 for alpha index is noted in the samples. The activity utilization index (AUI) from the samples satisfied the AUI <2, which corresponded with the annual effective dose of <0.3 mSv y?1, except interlock Site 2 and Gomez Spain tiles. Significantly, the mean value of excess lifetime cancer risk of 0.0014 is slightly lower than the world average value of 0.29 × 10?3.
Keywords:building materials  radioactivity  gamma spectroscopy  excess lifetime cancer risk  annual effective dose  alpha index
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