Stream Nitrate Responds Rapidly to Decreasing Nitrate Deposition |
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Authors: | Dolly N Kothawala Shaun A Watmough Martyn N Futter Leiming Zhang Peter J Dillon |
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Institution: | (1) Chemistry Department, Trent University, 1600 West Bank Drive, Peterborough, Ontario, K9J 7B8, Canada;(2) Environmental Resource Studies Program, Trent University, 1600 West Bank Drive, Peterborough, Ontario, K9J 7B8, Canada;(3) Department of Aquatic Sciences and Assessment, Swedish University of Agricultural Sciences, Uppsala, 75007, Sweden;(4) Air Quality Research Division, Science and Technology Branch, Environment Canada, 4905 Dufferin St., Toronto, Ontario, M3H 5T4, Canada |
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Abstract: | Ecosystem acidification and eutrophication resulting from increased deposition of dissolved inorganic nitrogen (DIN) are issues
of increasing global concern. Consequently, costly policy decisions are being implemented to decrease nitrogen oxide (NO
x
) emissions. Although declining DIN deposition along with rapid declines of DIN in surface waters have been reported in parts
of Europe, the same observation is just emerging in North America. Here we find a significant decline in bulk deposition NO3
− during the later part of a 28-year record in southcentral Ontario, Canada. Despite high N retention and substantial inter-annual
variability in the long-term record due to periods of drought, we find significant declines in annual NO3
− concentrations and export at six out of 11 streams that drain upland-dominated catchments. In contrast, five streams draining
primarily wetland-dominated catchments with lower levels of NO3
− show no decreasing trend in NO3
− concentration or export. The rapid response in stream NO3
− to declining atmospheric inputs was observed at sites with historically moderate inputs of DIN (~870 mg m−2 y−1) in bulk deposition. Topographic features such as slope, and related catchment features including wetland cover, appear to
influence which catchments will respond positively to declining DIN deposition. These findings force us to revise our original
conceptualization of the N saturation status of these catchments. |
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