Efficient Solar Cells Based on Light‐Harvesting Antimony Sulfoiodide |
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| Authors: | Riming Nie Hyun‐sung Yun Min‐Jae Paik Aarti Mehta Byung‐wook Park Yong Chan Choi Sang Il Seok |
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| Institution: | 1. Perovtronics Research Center, School of Energy and Chemical Engineering, Ulsan National Institute of Science and Technology (UNIST), Eonyang‐eup, Ulju‐gun, Ulsan, Republic of Korea;2. Convergence Research Center for Solar Energy, DGIST, Hyeonpung‐Myeon, Dalseong‐gun, Daegu, Republic of Korea;3. Division of Advanced Materials, Korea Research Institute of Chemical Technology (KRICT), Yuseong‐Gu, Daejeon, Republic of Korea |
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| Abstract: | Although antimony sulfoiodide (SbSI) exhibits very interesting properties including high photoconductivity, ferroelectricity, and piezoelectricity, it is not applied to solar cells. Meanwhile, SbSI is predominantly prepared as a powder using a high‐temperature, high‐pressure system. Herein, the fabrication of solar cells utilizing SbSI as light harvesters is reported for the first time to the best of knowledge. SbSI is prepared by solution processing, followed by annealing under mild temperature conditions by a reaction between antimony trisulfide, which is deposited by chemical bath deposition on a mesoporous TiO2 electrode and antimony triiodide, under air at a low temperature (90 °C) without any external pressure. The solar cells fabricated using SbSI exhibit a power conversion efficiency of 3.05% under standard illumination conditions of 100 mW cm?2. |
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| Keywords: | antimony sulfoiodide (SbSI) chalcohalides lead‐free perovskite materials solar cells |
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