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Dewu Lin Dehuan Shi Anquan Zhu Chengkai Yang Tian Zhang Kai Liu Kunlun Liu Guo Hong Wenjun Zhang 《Liver Transplantation》2024,14(14):2304535
The engineering of anode-electrolyte interphase for highly reversible and dendrite-free Zn plating-stripping continues to pose a significant challenge in the progression of aqueous Zn-ion batteries (AZIBs). In this study, a novel approach is introduced that involves the design of a hierarchical carbon nanotube (CNT)-based host through functionalization with cetyltrimethylammonium cations (CTA+). This hierarchical host enables dynamically switchable repulsive shielding to regulate Zn plating. The CNT scaffold, featured with high flexibility and conductivity, facilitates expandable accommodation of continuous Zn plating. Concurrently, the entangled CTA+ cations, acting as manipulators to form switchable repulsive shields, dynamically suppress the growth of Zn dendrites, and result in uniform Zn plating within cationic CNT (C-CNT) hosts. The cationic shielding effect is further elucidated through density functional theory calculations. By incorporating the self-adaptive C-CNT host, Zn symmetric cells exhibit an impressively stable cycling lifespan exceeding 6500 h at 1 mA·cm−2 and achieve a cumulative capacity of 6000 mAh·cm−2 at 4 mA·cm−2. Full batteries, by coupling the C-CNT@Zn anode and MnO2 cathode, demonstrate an 88% capacity retention after 2000 cycles at 2 A·g−1. The design of the self-adaptive C-CNT host offers a promising approach in electrode-electrolyte interphase engineering toward the practical applications of Zn-based energy storage systems. 相似文献
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Lithium‐Ion Batteries: All‐Nanomat Lithium‐Ion Batteries: A New Cell Architecture Platform for Ultrahigh Energy Density and Mechanical Flexibility (Adv. Energy Mater. 22/2017) 下载免费PDF全文
Ju‐Myung Kim Jeong A. Kim Seung‐Hyeok Kim In Sung Uhm Sung Joong Kang Guntae Kim Sun‐Young Lee Sun‐Hwa Yeon Sang‐Young Lee 《Liver Transplantation》2017,7(22)
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Energy Harvesting: Optically Switchable Smart Windows with Integrated Photovoltaic Devices (Adv. Energy Mater. 3/2015) 下载免费PDF全文
Hyun‐Keun Kwon Kyu‐Tae Lee Kahyun Hur Sung Hwan Moon Malik M. Quasim Timothy D. Wilkinson Ji‐Young Han Hyungduk Ko Il‐Ki Han Byoungnam Park Byoung Koun Min Byeong‐Kwon Ju Stephen M. Morris Richard H. Friend Doo‐Hyun Ko 《Liver Transplantation》2015,5(3)
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