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1.
Age-dependent accumulation of 137Cs in the muscles and bodies of the pike Esox lucius (aged two to seven years) inhabiting a section of the Yenisei River polluted with artificial radionuclides has been studied. The content of 137Cs in muscles varied from 0.5 to 7.0 Bq/kg of fresh weight. The maximum content of the radionuclide has been found in juveniles. The content of 137Cs in pike muscles and body decreased considerably with age. The high content of 137Cs in the muscles of juveniles is probably a consequence of their higher intensity of feeding as compared to older individuals, which is due to the intense growth of juveniles.  相似文献   

2.
The deposition of radiocaesium from nuclear weapons testing and the Chernobyl accident upon the Llyn Llygad Rheidol catchment in mid-Wales is described. Inventories of soil cores from the catchment support estimates of total atmospheric fallout. The mean inventory of weapons testing 137Cs in lake sediment cores is broadly similar to that in soil cores. The inventory of Chernobyl fallout in sediment cores is significantly lower and raises questions concerning the residence time of 137Cs in the catchment soils and lake waters. 137Cs and 241Am activities in a sediment core record the 1963 peak of fallout from nuclear weapons testing. The association of the peak activities of 137Cs and 241Am in the sediments with the falloot maximum is confirmed by 210Pb dating. The 210Pb dates also reveal a significant increase in sediment accumulation rates over the past 20 years.  相似文献   

3.
The analysis of planktic foraminiferal assemblages from Site 1090 (ODP Leg 177), located in the central part of the Subantarctic Zone south of South Africa, provided a geochronology of a 330-m-thick sequence spanning the Middle Eocene to Early Pliocene. A sequence of discrete bioevents enables the calibration of the Antarctic Paleogene (AP) Zonation with lower latitude biozonal schemes for the Middle–Late Eocene interval. In spite of the poor recovery of planktic foraminiferal assemblages, a correlation with the lower latitude standard planktic foraminiferal zonations has been attempted for the whole surveyed interval. Identified bioevents have been tentatively calibrated to the geomagnetic polarity time scale following the biochronology of Berggren et al. (1995). Besides planktic foraminiferal bioevents, the disappearance of the benthic foraminifera Nuttallides truempyi has been used to approximate the Middle/Late Eocene boundary. A hiatus of at least 11.7 Myr occurs between 78 and 71 m composite depth extending from the Early Miocene to the latest Miocene–Early Pliocene. Middle Eocene assemblages exhibit a temperate affinity, while the loss of several planktic foraminiferal species by late Middle to early Late Eocene time reflects cooling. During the Late Eocene–Oligocene intense dissolution caused impoverishment of planktic foraminiferal assemblages possibly following the emplacement of cold, corrosive bottom waters. Two warming peaks are, however, observed: the late Middle Eocene is marked by the invasion of the warmer water Acarinina spinuloinflata and Hantkenina alabamensis at 40.5 Ma, while the middle Late Eocene experienced the immigration of some globigerinathekids including Globigerinatheka luterbacheri and Globigerinatheka cf. semiinvoluta at 34.3 Ma. A more continuous record is observed for the Early Miocene and the Late Miocene–Early Pliocene where planktic foraminiferal assemblages show a distinct affinity with southern mid- to high-latitude faunas.  相似文献   

4.
The regularities of 137Cs distribution in trees (Pinus sylvestris and Betula pendula) growing in different types of forest ecosystems were investigated. High levels of heterogeneity of 137Cs activity concentrations in different parts of the trees, resulting from their varied metabolism have been shown. The data obtained demonstrate a non-uniform character of 137Cs distribution along the trunks, which can be explained by radio- nuclide fixation by the xylem vessel walls and by geometry changes along the tree trunk. It has been found that the radial distribution of 137Cs in the tree trunk is dependent on the availability of 137Cs in soil, which governs the transfer of this radionuclide via xylem sap and on the properties of the xylem. The accumulation of 137Cs by trees was influenced by the vertical distribution and availability of 137Cs in the soil as well as by the root biomass distribution in different soil horizons. A bioavailability factor, which takes into account the vertical distribution of radiocesium in soil, bioavailability of this radionuclide and distribution of root biomass in different soil horizons is proposed for comparative analyses of 137Cs transfer from soil to trees in different types of forest ecosystems. Received: 8 February 2000 / Accepted: 1 December 2000  相似文献   

5.
241Am dating of lake sediments   总被引:2,自引:0,他引:2  
241Am derived from decay of fallout 241Pu is now frequently detected in analyses of lake sediments by low-background gamma assay, and offers an alternative to weapons test 137Cs in dating recent sediments at those sites where the 137Cs record has been degraded by post-depositional mobility or obliterated by Chernobyl fallout. Calculations of the in-growth of 241Am from 241Pu indicate a nominal distribution broadly similar to that of 137Cs, with the maximum 241Am activity occuring in fallout dating from 1963. Results from a number of sites suggest that 241Am is significantly less mobile in lake sediments than 137Cs, and that its distribution in cores reflects more closely the fallout record. Since further decay of existing weapons debris will increase 241Am concentrations by about 24% over the next 40 years, 241Am is likely to play an increasingly important role in assessing the validity of 210Pb dates at sites with varying sediment accumulation rates.  相似文献   

6.
In many Swedish lakes, the fallout of 137Cs from the Chernobyl accident in April 1986 has largely accumulated in the sediments. The availability and transfer of deposited 137Cs to biota is influenced by factors such as resuspension. The frequency of resuspension and the 137Cs-content of different fish species was studied in three shallow lakes in Uppland, central Sweden, and in one deeper lake in northern Sweden. Resuspension was measured by the use of sediment traps. Sedimentation rates measured from the traps in the shallower lakes were 5–10 times higher than normal for this type of lake, indicating that resuspension was an important factor. The decrease of the 137Cs-content in muscle tissue of pike, perch and roach was slow in each of the shallow lakes. 137Cs decreased by about 30% over a period of 2 years in the shallowest lake (maximum depth 4 m), whereas 137Cs decreased by 50% in the deeper lakes (maximum depth 10 m). The slower rates of decline of 137Cs in biota from the shallow lakes, are probably a function of sediment dynamics (mainly influenced by lake morphometry, wind direction and strength). They may be influenced, also, by bioavailability of resuspended sediment material. In the deepest northern lake, much of the 137Cs-containing material collected in the sediment traps originated from the catchment area. Resuspension was minimal, and the high activity of 137Cs in the sediment had no effect on content or decline of 137Cs in lake fish.  相似文献   

7.
The accumulation levels of anthropogenic 90Sr and 134Cs and 137Cs radionuclides in the marsh frog have been studied in the areas of the Beloyarskii water-storage reservoir (an industrial storm-water discharge channel of the nuclear power station) and the Verkhnii Tagil water-storage reservoir (the Tagil River down-stream of the dam). No significant distinction in the radionuclide accumulation (90Sr and 137Cs) depending on the amphibian sex and age is detected. Comparable levels of the accumulation of radionuclides in the marsh frog, when compared to the other representatives of the water ecosystem, are estimated. An assumption of the presence of some unidentified source of radioactive contamination of marsh frogs has been made; cesium-137 may be transferred from it to the Tagil River by the frogs.  相似文献   

8.
Ge F L  Zhang J H  Su Z A  Nie X J 《农业工程》2007,27(2):459-463
Severe soil erosion of cultivated sloping land in hilly areas of Sichuan, China, has resulted in deterioration of soil quality, and therefore has an adverse impact on crop production. A hillslope of 110 m in length was selected with a slope steepness of 10.12% where the soils were classified as Regosols. Soil samples for determining 137Cs, soil organic matter (SOM), total N, P, K, available N, P, K and particle size fraction were collected at 10 m intervals along a transect of the hillslope. Loss of soil nutrients owing to soil erosion was studied by using 137Cs technique, and the relationships between 137Cs-derived soil redistribution rates and soil nutrients were established over the cultivated sloping land in hilly areas of Sichuan, China (30o26′N, 104o28′E). The values of SOM, total N, available N, P, K and the soil particle fractions of size < 0.002 mm were smaller at upper and middle slope positions where 137Cs inventories were lower (i.e., soil erosion rates were higher) than at downslope positions where 137Cs inventories were higher (i.e., soil erosion rates were lower). The lowest 137Cs inventories were found at the hilltop, showing that besides erosion owing to water flow, tillage also contributed to soil losses, and intensive tillage was mostly responsible for severe erosion at upper slope positions. There were significant differences in SOM, total N, available N, P, K and the soil particle fractions of size < 0.002 mm between different slope segments, and these properties were significantly correlated with slope length. These soil properties were also significantly correlated with 137Cs inventories, indicating that both 137Cs and nutrient concentrations varied with topographical changes. The variation in soil properties was strongly influenced by erosion-induced soil redistribution, and therefore 137Cs inventories mirroring soil redistribution rates would be considered as an integrated indicator of soil quality.  相似文献   

9.
Recent rates of peat accretion (as determined by137Cs) and N, P, organic C, Ca and Na accumulation were measured along a 10 km eutrophication gradient in the northern Everglades area of Water Conservation Area 2A (WCA 2A) that has received agricultural drainage from the Hillsboro canal for the past 25–30 yrs. Rates of peat accretion were highest at sampling locations closest to the Hillsboro canal, 1.6 km downstream, (5.67 ± 0.50 mm/yr) and decreased to 2.01 ± 0.31 mm/yr at distances of 7.1 to 10.7 km downstream. Phosphorus and Na accumulation were a function of both peat accretion and soil P and Na concentrations. The concentration and accumulation of P in peat deposited in the past 26 years was highest near the Hillsboro canal (1478 ± 67 ug/g, 0.66 ± 0.06 g/m2/yr) and decreased to 560 ± 20 ug/g and 0.10 ± 0.02 g/m2/yr at distances of 8.8 to 10.7 km downstream. Like phosphorus, the concentration and rate of Na accumulation was highest near the Hillsboro canal (3205 ± 1021 ug/g, 1.48 ± 0.53 g/m2/yr). Although sodium enrichment of the peat was limited to 1.6 km downstream of the Hillsboro canal, increased rates of Na accumulation penetrated 5.2 km downstream of the Hillsboro canal, the extent of the area of enhanced peat accretion. In contrast to P and Na, there was no difference in the concentration of soil organic C, N and Ca along the eutrophication gradient. However, there was a gradient of organic C, N and Ca accumulation corresponding to the area of enhanced peat accretion. The highest rates occurred 1.6 km south of the Hillsboro canal (212 ± 5 g organic C/m2/yr, 14.1 ± 0.4 g N/m2/yr, 22.1 ± 5.2 g Ca/m2/yr). Accumulation of organic C, N and Ca at distances of 7.1–10.7 km downstream averaged 87 ± 11, 6.3 ± 0.7 and 6.5 ± 0.9 g/m2/yr, respectively. The areal extent of enhanced peat accretion and organic C, N, Ca and Na accumulation encompasses approximately 7700 ha of the northern part of WCA 2A. The area of enhanced P accumulation is larger, covering 11,500 ha or 26% of the total area of WCA 2A. The 11,500 ha area has functioned as a sink for P for the past 25–30 yr removing 74% (49.3 MT/yr) of the 67 MT/yr that enters via agricultural drainage and rainfall. Moreover, P accumulation along the gradient was related to mean (1989–1990) surface water P concentration, decreasing as surface water P decreases. These findings suggest that P accumulation is dependent on the P concentration in the water column and that decreasing P loadings per unit area result in less P storage per unit area. The potential longterm equilibrium of the 11,500 ha area as a sink for P is based on a mean annual loading of 67 metric tons P/yr. Input rates exceeding this loading rate could result in an expansion of the 11,500 ha area until a new equilibrium size is reached.  相似文献   

10.
Airborne particles of nuclear fuel from the Chernobyl reactor that had been collected on air filters and stored, were characterised using in vitro dissolution tests to assess effective doses after their inhalation. As solvent, the Gamble biological fluid was used to simulate lung fluid. The solubility of the measured radionuclides decreased in the order 137Cs>90Sr>>241Am239+240Pu in the simulated lung fluid. The dissolution rate constant of e.g. 239+249Pu ranged from 0.72 to 5.4×10–6 g·cm–2 d–1 and decreased (for all nuclides) with increasing particle size as predicted from theoretical considerations. Considering the inhalation dose, decreasing dose with size and increasing doses with lower solubility may partly counterbalance each other for 137Cs and 90Sr. On the other hand, for 239Pu and 241Am larger particles and associated lower solubility both change the resulting dose in the same direction towards lower values. The comparison of the experimentally determined dose coefficients with ICRP values indicates that nuclear fuel particles closely resemble type M material characteristics for 137Cs and 90Sr and type S material characteristics for 239Pu and 241Am.  相似文献   

11.
The influence of Bifezh (a hexacyanoferrate compound as veterinary feed additive) on the transfer of 137Cs to meat was investigated in broiler chickens after application of an artificially contaminated feed mixture. The reduction factors reached 2.23 and 8.46 for single and multiple 137Cs administration, respectively. The elimination rate of 137Cs in the decontamination period was only slightly increased by Bifezh. The reduction effect of Bifezh was considerably and positively limited by various amounts of the additive during both radiocaesium accumulation and decontamination. No significant differences in the reduction effect between breast and thigh meat were observed. In conclusion, the hexacyanoferrate-cellulose binder Bifezh can be recommended as an alternative chemical measure for reducing 137Cs contamination of broiler chicken meat, although administration rates may need to be enhanced over those currently recommended.  相似文献   

12.
Field-grown maize hybrids were assessed for variability in 137Cs accumulation in vegetative parts of young and mature maize shoots and grains during 2 years with contrasting climatic conditions. Trials were carried out at different sites in the Tula region of Russia, which is characterized by a highly homogenous soil classified as Luvic Chernozem according to FAO/UNESCO, and average contamination levels of about 509–564 Bq 137Cs kg−1 soil. In the first year, 19 hybrids were tested. The two hybrids with the highest and the two with the lowest 137Cs concentration ratios (C r) were also tested in the second year, together with another 11 hybrids. All samples were additionally assessed for their potassium content. In both investigation periods 137Cs accumulation in vegetative shoots and grains was found to vary up to more than twofold between hybrids. However, C r values of those hybrids that showed a relatively low 137Cs accumulation in the first year were not necessarily low in the second year, and the ratio between the 137Cs C r of low- and high-accumulating hybrids was much smaller than in the year before. In both vegetative shoots and grains the variance caused by the different years was larger than the genotypic variance, thus indicating the limits of genotype selection for this trait. Significant correlations were determined between the 40K and 137Cs C r values in the same tissue, but for one hybrid indications for uncoupling of the two traits were found. Average Cs/K ratios in young shoots, mature shoots and grains were 0.06, 0.05 and 0.02, respectively, indicating tissue- and stage-specific regulation of accumulation within each plant. The findings are discussed with respect to new approaches towards a better understanding of 137Cs accumulation and its potential reduction in plants. Katharina Schneider was deceased.  相似文献   

13.
Radionuclide dating of the recent sediments of Blelham Tarn   总被引:9,自引:0,他引:9  
Lake sediments of the last 1000 years provide a unique record of environmental changes. Methods of dating this record are reviewed and discussed. Sediments of the last 20 years, which are of particular biological significance because of their record of man-made changes in lakes (including enrichment and pollution) have been dated successfully by the distribution within them of the fallout product 137Cs, present in the atmosphere since 1954 and reaching a peak of supply in 1963. The structured pattern shown by the curve for 137Cs concentration in most sediments investigated indicates that faunal mixing of the surface muds does not destroy the vertical stratification of the sediment profile. Sediments up to 120 years old have been dated by a lead isotope technique, and the results of this proved consistent with both 137Cs dating and with palaeomagnetic dating where this was possible. Theoretical considerations of the application of radiocarbon dating to organic material of 18th and 19th century date are reviewed. Results of application of these radionuclide techniques to the sediments of a small lake, Blelham Tarn, near Windermere, are presented. Evidence from 137Cs and 210Pb dating of profiles from several different positions within the lake shows that the depth of the annual increment to the sediments varies by a factor of × 2 from place to place. The concentration within the sediment of chemical and biological variables shows no significant variation from one position to another; therefore calculated values for amounts of each variable included within unit area of the annual increment depend primarily on the thickness of this at the site chosen, and so cannot be directly related to the rates of supply of, for example, pollen grains or total organic matter, and so to rates of productivity. Results from nine 14C dates on material 400–1000 years old, when correlated with analyses for pollen and sediment composition, demonstrate the profound effects of agricultural practices in the catchment (assumed to be deforestation and ploughing) in disturbing the orderly transfer to lake sediments of material eroded from the catchment.  相似文献   

14.
The oxygen- and carbon-isotope compositions of planktic and benthic foraminifera and calcareous nannofossils from Middle Oligocene-Early Miocene Equatorial Atlantic sediments (DSDP Site 354) indicate two important paleoceanographic changes, in the Late Oligocene (foraminiferal Zone P.21) and in the Early Miocene (foraminiferal Zone N.5). The first change, reflected by a δ18O increase of 1.45‰ inGlobigerina venezuelana, affected only intermediate pelagic and not surface, deep or bottom waters. The second change affected surface and intermediate waters, whereas deep and bottom waters showed only minor fluctuations. In the case of the former the isotope effect of the moderate ice accumulation on the Antarctic continent is amplified in the Equatorial Atlantic by changes in the circulation pattern. The latter paleoceanographic change, reflected by a significant increase in18O in both planktic and benthic forms (about 1.0‰ and 0.5‰, respectively), may have been caused by ice volume increase and temperature decrease. Both oxygen- and carbon-isotope compositions indicate a marked depth-habitat stratification for planktic foraminifera and calcareous nannofossils. Three different dwelling groups are recognized: shallowGlobigerinoides, Globoquadrina dehiscens, Globorotalia mayeri and nannofossils; intermediateGlobigerina venezuelana; and deepCatapsydrax dissimilis. The comparison of foraminifera and calcareous nannofossils suggests that the isotopic compositions of nannofossils are generally controlled by the same parameters which control the isotopic composition of shallow-dwelling foraminifera, but the former are more enriched in18O.  相似文献   

15.
The distribution of 137Cs and 239,240Pu in sediment core samples of the Finnish lakes Laukunlampi, Lovojärvi and Pääjärvi were determined. The sediment samples were collected using dry ice and liquid nitrogen freezing methods. The sediments of these lakes are annually laminated. A clear maximum concentration of 137Cs and 239,240Pu was found in sediment layers formed during 1962–1964, the years of maximum fallout, and the middle of the 1950's can be estimated from the 137Cs and 239,240Pu profiles. The highest concentrations, 11 500 and 820 pCi kg–1 dry wt for 137Cs and 239,240Pu, respectively, were found in the sediment of Laukunlampi. The vertical distribution was similar for 137Cs and 239,240Pu in the lakes investigated. A slight migration of 239,240Pu and 137Cs was found and the migration of 137Cs seems to be higher than that of 239,240Pu. The advantages of 137Cs dating method are rapidity and simplicity. 239,240Pu is preferable when the sample size is small. The agreement found between 137Cs and 239,240Pu dates and the annual laminae show that these fallout radio isotopes can be used for dating sediments formed during the past 25 years.  相似文献   

16.
Planktic foraminiferal assemblages are well known to vary in accordance with seasonal fluctuations in ocean properties, periodic reproduction cycles, and variations between water masses. Here we report that storms also can significantly influence foraminiferal assemblages. During the RV Meteor cruise 21 to the Northeast Atlantic Ocean ( area), from March to May 1992, planktic foraminifera were sampled using a multiple opening-closing net. While sampling, two storms with wind forces up to 12 Beaufort caused intensified surface layer mixing with shifts in the depth of the upper ocean mixed-layer from 20–40 m to 170–240 m. Subsequently, planktic foraminiferal growth rates increased, resulting in an elevated quantity of small (100–150 μm) tests (Phase 1). When the wind strength increased a second time, the mixed-layer deepened to a depth below the former position of the pycnocline, and again the abundance of small tests increased (Phase 2). During Phase 2, the weight of calcite in specimens of the productive zone reached its maximum. In the export zone, an associated increase in empty tests occurred with a lag time depending on the test sinking velocity. In the upper export zone, down to 700 m water depth, CaCO3 flux increased from 9.3 to 49.8 mg CaCO3 m−2 d−1 after the first storm and from 8.9 to 19.9 mg CaCO3 m−2d−1 after the second storm. In the 700 to 2500 m depth interval, the flux increased from 5.1 mg CaCO3 m−2 d−1 to about 9.2 mg CaCO, m−2 d−1. Thus, the standing stock of living foraminifera and export of empty tests from the productive zone increased after the storms, leading to pulses of CaCO3 exported from the surface to deep water.  相似文献   

17.
Spring wheat (Triticum aestivum L. cv. Tonic) was grown for 16 days in a sandy loam soil which was contaminated with 137Cs. The soil was fertilised with K at three rates (0,1 and 2 mmol K per 950 g dry soil) and with NO3 --N at two rates (0 and 2 mmol per 950 g dry soil) in a factorial design. The 137Cs Activity Concentration (AC) in the shoot tissue significantly reduced 8.2-fold (nil N treatment, p<0.001) and 9.3-fold (highest N dose, p<0.001) with increasing K supply. In contrast, the K application increased the 137Cs AC in soil solution 1.7 fold (nil N treatment) or had no significant effect (highest N dose). At similar K application, the application of N increased the 137Cs AC in the shoot compared to the control. This effect is most probably due to the increased NH4 + concentration in soil solution which increased the 137Cs AC in soil solution. The soil solution composition (137Cs and K concentration) in the rhizosphere was estimated from the average soil solution composition at day 16 and solute transport calculations. The 137Cs AC in the shoot tissue was predicted from the estimated soil solution composition in the rhizosphere and the relationship between K concentration and 137Cs uptake derived from a nutrient solution experiment. The predictions of 137Cs AC's in the shoot are qualitatively correct for the fertiliser effects but underestimate the observations between 1.4 and 9.9 fold.  相似文献   

18.
A dynamic model was developed for evaluation of the fish contamination by 137Cs. The dynamics of the accumulation of the radionuclide and the elimination is calculated taking into account the ecological and physiological characteristics of the fish, such as growth and metabolic rates, its position in the food chains of the aquatic ecosystem. The biological elimination of 137Cs from the freshwater fish is proportional to the metabolic rate of the fish. The dimensionless coefficient of the proportionality is equal to epsilonA = 0.3 +/- 0.1. The model was applied for the reconstruction of the long-term dynamics of 137Cs in the food chain "goldfish-pike" from Lake Kozhanovskoe (Bryansk Region, Russia). In 1990-1999 the specific activity of 137Cs in goldfish (generation of 1990) varied in range about 5-20 kBq/kg, whereas the specific activity of 137Cs in pike (generation of 1989) varied in range about 20-40 kBq/kg. The comparison with the data of the observations confirmed that the presented method allows to evaluate adequately the levels and the dynamics of 137Cs accumulation by the freshwater fish.  相似文献   

19.
This article presents the results of an investigation into the occurrence of elevated levels of radionuclides in soils associated with a seabird colony in the Arctic. Soils and other materials were collected from a seabird colony (primarily composed of kittiwakes) in Kongsfjorden, located in the High Arctic archipelago of Svalbard. The samples were analyzed for a suite of gamma emitting natural and anthropogenic radionuclides, including 137Cs and nuclides of the 238U and 232Th series, to establish the level of enrichment and the behavior of the radionuclides in the immediate area. The results indicate that soils near the colony exhibit enrichment factors of 8 for 137Cs, 5 for 238U and 2 for 226Ra compared to the nuclide content of soils from the general area. The spatial patterns of the nuclides in the soil are consistent with enrichment of the soil via run-off draining from a large accumulation of fecal and nesting material that has developed at the base of the colony. 137Cs ingress to the soil appears to have peaked at some point in the past as patterns of enrichment at the colony are different to those exhibited by 238U, which must be assumed to be a steady state contribution. The means of introduction of radionuclides to the colony remains unclear but the transfer of 137Cs from the marine environment to the terrestrial environment via the food chain and deposition of feces is discussed.  相似文献   

20.
Concentrations of some radionuclides, including137Cs, in desert truffles in Kuwait were studied and compared with similar samples from other countries in the Middle East, namely Iran, Egypt, and Tunisia. In addition, sand samples from Kuwait were assayed to calculate the transfer factor of the radionuclides under consideration. The measured concentrations of40K,226Ra, and137Cs show that137Cs is much higher in Egyptian samples, whereas40K is much lower in samples from Tunisia. The average effective dose equivalent calculated for the Kuwaiti population according to their diet habits was found to be in the range 0.14-0.23 ΜSv/a. The results are compared with values from other countries.  相似文献   

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