Pulsed submicrosecond multichannel sliding discharges of opposite polarities: Filling of the discharge gap with spark channels

Results are presented from measurements of the discharge current and the factor of the discharge gap filling with spark channels during pulsed sliding discharges of opposite polarities in Ne, Ar, and Xe on an aluminum oxide ceramic surface. The measurements were performed in the regime of single pulses of submi-crosecond duration at discharge voltages of 0?C12 kV with two discharge chambers with different thicknesses of the ceramic plate (0.4 and 0.17 cm) and different electrode gap lengths (4 and 10.3 cm) at gas pressures of 30 and 100 kPa. The results obtained for discharges of opposite polarities are compared with one another, and common features of discharges in three gases are revealed. It is shown that the filling of the discharge gap with spark channels in the gases under study is more efficient in the case of the positive polarity of the discharge voltage, except Xe at a pressure of 100 kPa in the electrode gap of length 10.3 cm. The quasi-homogeneous regime of discharge in each of the three gases is attained easier at lower gas pressures. Comparison of the data on the filling factors of the discharge gap and the peak currents of opposite-polarity discharges for each gas at a given pressure indicates that the higher the discharge current, the more densely the discharge gap is filled with spark channels.     

Specific features of a single-pulse sliding discharge in neon near the threshold for spark breakdown

Experimental data on the spatial structure of a single-pulse sliding discharge in neon at voltages below, equal to, and above the threshold for spark breakdown are discussed. The experiments were carried at gas pressures of 30 and 100 kPa and different polarities of the discharge voltage. Photographs of the plasma structure in two discharge chambers with different dimensions of the discharge zone and different thicknesses of an alumina dielectric plate on the surface of which the discharge develops are inspected. Common features of the prebreakdown discharge and its specific features depending on the voltage polarity and gas pressure are analyzed. It is shown that, at voltages below the threshold for spark breakdown, a low-current glow discharge with cathode and anode spots develops in the electrode gap. Above the breakdown threshold, regardless of the voltage polarity, spark channels directed from the cathode to the anode develop against the background of a low-current discharge.     

Observation and Investigation of “Reverse Breakdown” in a Discharge Tube

A discharge operating in a 80-cm-long discharge tube with an inner diameter of 15 mm, filled with a 3 : 1 neon–argon mixture at a pressure of 1 Torr, was investigated experimentally. Square voltage pulses with a period of 1 s were supplied to one of the tube electrodes, the second electrode being ungrounded. The initial stage of breakdown—the primary breakdown between the high-voltage (active) electrode and the tube wall, accompanied by the propagation of the prebreakdown ionization wave—was the same as in the conventional scheme with a grounded low-voltage electrode. Since the discharge gap was not closed, the discharge was not ignited. An essentially new effect was observed after the end of the voltage pulse. After a certain time interval, voltage spikes of opposite polarity, the amplitude and shape of which were close to those observed during the primary breakdown, appeared in the voltage and current waveforms of the active electrode. Simultaneously, a radiation pulse from the region adjacent to the active electrode was observed and an ionization wave began to propagate toward the second electrode. This work is dedicated to investigating this effect (which was named “reverse breakdown”) and analyzing its mechanism. A conclusion is made on the similarity of this phenomenon to the processes occurring in atmospheric-pressure dielectric barrier discharges.     

Alternating nonsteady gas-discharge modes in an atmospheric-pressure air flow blown through a point-plane gap

The electric and spectral characteristics of a nonsteady discharge in an atmospheric air flow blown through a point-plane interelectrode gap were investigated experimentally. The discharge was produced by applying a constant positive voltage to the point electrode, the amplitude of the applied voltage being much higher than the corona ignition voltage. The nonsteady character of the discharge is due to the spontaneously repeating streamer-spark breakdown, followed by the formation of either a diffuse ultracorona or a filamentary glow discharge. In the latter case, the length of the plasma column increases progressively, being blown off by the gas flow from the discharge gap. The extinction of a filamentary discharge is unrelated to the break of the current channel: the discharge decays abruptly when the filament length reaches its critical value. The distribution of active particles (O, OH, and N*₂) carried out from the discharge gap is determined from the data of spectral measurements.     

Hydrodynamic model of a dielectric-barrier discharge in pure chlorine

A one-dimensional hydrodynamic model of a dielectric-barrier discharge (DBD) in pure chlorine is developed, and the properties of the discharge are modeled. The discharge is excited in an 8-mm-long discharge gap between 2-mm-thick dielectric quartz layers covering metal electrodes. The DBD spatiotemporal characteristics at gas pressures of 15–100 Torr are modeled for the case in which a 100-kHz harmonic voltage with an amplitude of 8 kV is applied to the electrodes. The average power density deposited in the discharge over one voltage period is 2.5–5.8 W/cm³. It is shown that ions and electrons absorb about 95 and 5% of the discharge power, respectively. In this case, from 67 to 97% of the power absorbed by electrons is spent on the dissociation and ionization of Cl₂ molecules. Two phases can be distinguished in the discharge dynamics: the active (multispike) phase, which follows the breakdown of the discharge gap, and the passive phase. The active phase is characterized by the presence of multiple current spikes, a relatively high current, small surface charge density on the dielectrics, and large voltage drop across the discharge gap. The passive phase (with no current spikes) is characterized by a low current, large surface charge density on the dielectrics, and small voltage drop across the discharge gap. The peak current density in the spikes at all pressures is about 4 mA/cm². In the multispike phase, there are distinct space charge sheaths with thicknesses of 1.5–1.8 mm and a mean electron energy of 4.3–7 eV and the central region of quasineutral plasma with a weak electric field and a mean electron energy of 0.8–3 eV. The degree of ionization of chlorine molecules in the discharge is ~0.02% at a pressure of 15 Torr and ~0.01% at 100 Torr. The DBD plasma is electronegative due to the fast attachment of electrons to chlorine atoms: e + Cl₂ → Cl + Cl^–. The most abundant charged particles are Cl ₂ ⁺ and Cl^? ions, and the degree of ionization during current spikes in the active phase is (4.1–5.5) × 10^–7. The mechanism of discharge sustainment is analyzed. The appearance of a series of current spikes in the active phase of the discharge is explained.     

Electric characteristics of a surface barrier discharge with a plasma induction electrode

Static and dynamic current-voltage and charge-voltage characteristics of a surface barrier discharge with a plasma induction electrode have been investigated experimentally. The dependences of the discharge current on both the gas pressure in the induction electrode tube and the winding pitch of the corona electrode, as well as of the discharge power efficiency on the applied voltage, have been measured.     

Numerical analysis of similarity of barrier discharges in the 0.95 Ne/0.05 Xe mixture

Established dynamic regimes of similar (with a scale factor of 10) barrier discharges in the 0.95 Ne/0.05 Xe mixture are simulated in a one-dimensional drift-diffusion model. The similarity is examined of barrier discharges excited in gaps of lengths 0.4 and 4 mm at gas pressures of 350 and 35 Torr and dielectric layer thicknesses of 0.2 and 2 mm, the frequencies of the 400-V ac voltage applied to the discharge electrodes being 100 and 10 kHz, respectively.     

Experimental Study of Heating of a Liquid Cathode and Transfer of Its Components into the Gas Phase under the Action of a DC Discharge

An atmospheric-pressure dc discharge in air (i = 10–50 mA) with metal and liquid electrolyte electrodes was studied experimentally. An aqueous solution of sodium chloride (0.5 mol/L) was used as the cathode or anode. The electric field strength in the plasma and the cathode (anode) voltage drops were obtained from the measured dependences of the discharge voltage on the electrode gap length. The gas temperature was deduced from the spectral distribution of nitrogen emission in the band N₂(C³Π _u → B³Π _g , 0–2). The time dependences of the temperatures of the liquid electrolyte electrodes during the discharge and in its afterglow, as well as the evaporation rate of the solution, were determined experimentally. The contributions of ion bombardment and heat flux from the plasma to the heating of the liquid electrode and transfer of solvent (water) into the gas phase are discussed using the experimental data obtained.     

Dynamics of the optical emission from a high-voltage diffuse discharge in a rod-plane electrode system in atmospheric-pressure air

Results are presented from experimental investigations of the dynamics of optical emission from a nanosecond diffuse discharge in a rod-plane electrode system. A study was made of discharges in a 10-cm-long interelectrode gap in atmospheric-pressure air (the cathode being a 1-cm-diameter rod with a bullet-shaped end). The voltage across the discharge gap was 220 kV and the voltage pulse duration was 180 ns, the voltage rise time being 10 ns. In experiments, the discharges were observed to evolve through two stages: the bridging stage and the conduction stage. The bridging stage begins with intense optical emission from the cathode region, the onset of the emission being delayed with respect to the beginning of the voltage pulse. Simultaneously with the onset of optical emission, a displacement current corresponding to the motion of charged particles begins to be generated in the cathode region. The duration of this current corresponds to the time the emission front takes to bridge the gap. As the emission front reaches the anode region, the current increases abruptly, indicating the beginning of the conduction stage. It was found that the time delay of optical emission relative to the beginning of the voltage pulse largely governs the discharge parameters: as the time delay becomes longer, the emission front velocity in the bridging stage increases from 0.6 to 1.5 cm/ns, the probability of realizing a multichannel structure of the discharge becomes higher, and the discharge current and the intensity of X-ray emission from the discharge grow.     

Influence of the Distributed Phase of Gas Bubbles on a Pulsed Electrical Discharge in Water

The development of a pulsed electrical discharge in water with vapor–air microbubbles, the volume distribution of which in water is close to uniform, has been studied experimentally. The presence of volumetric microbubbles with an average diameter of ~50 μm and a bulk gas content of no more than 1% does not change the thermal mechanism of the development of the discharge in water with a conductivity of ~300 μS/cm at overvoltages of 1–1.5, the minimum breakdown voltage being ~9 kV. Under these conditions, the determining role is played by the surface bubbles, which change the observed mechanism of the discharge development. The discharge is initiated in the surface bubbles simultaneously on both electrodes. The growth of the cathode channel at a velocity of ~60 m/s leads to the closure of the 1-cm-long gap during a time of ~160 μs.     

Study of the Formation Time of a Self-Sustained Subnanosecond Discharge at High and Ultrahigh Gas Pressures

The formation times of self-sustained subnanosecond discharges in nitrogen at pressures of 1?40 atm and in hydrogen at pressures of 1–60 atm are analyzed in terms of the avalanche model. In experiments, a subnanosecond voltage pulse with an amplitude of 102 ± 2 kV was applied to a 0.5-mm-long discharge gap with a uniformly distributed electric field (the curvature radii of both the cathode and anode ends were 1 cm). The rise time of the voltage pulse from 0.1 to 0.9 of its amplitude value was about 250 ps. Breakdown occurred at the leading edge of the pulse. The discharge formation time was measured at different gas pressures with a step of 5–10 atm. Analysis of the experimental results shows that, in nitrogen at pressures of 10–40 atm and in hydrogen at pressures of 20–50 atm, breakdown occurs earlier than the electron avalanche reaches its critical length and that the critical avalanche length lies in the range of (2–8) × 10^–2 mm, which is one order of magnitude shorter than the discharge gap length. This means that the avalanche–streamer model is inapplicable in this case. The fast formation of a conducting channel under these conditions can be explained by ionization of gas by runaway electrons. In this case, the conducting column develops as a result of simultaneous development of a large number of electron avalanches in the gas volume. An increase in the hydrogen pressure from 50 to 60 atm leads to an abrupt increase in the discharge formation time by about 50%. As a result, the growth time of the electron avalanche to its critical length becomes shorter than the discharge formation time. In this case, the electrons cease to pass into the runaway regime and the discharge is initiated from the cathode due to field emission from microinhomogeneities on its surface. Under these conditions, the discharge formation time is well described by the avalanche–streamer model.     

Pulsed Regime of the Diffusive Mode of a Barrier Discharge in Helium

Periodic pulsations of the active current component are revealed experimentally in transversely homogeneous barrier discharges in helium at small values of the parameter Pd (below 500 torr mm) and moderate frequencies of the applied voltage (f < 100 kHz). The frequency of the current pulsations is higher than the frequency of the well-studied pulsations in a transversely inhomogeneous streamer barrier discharge in air by a factor of approximately 100. Numerical calculations show that the physical nature of the observed pulsations can be explained in terms of the negative differential resistance of the cathode fall region, which occupies essentially the entire interelectrode gap in each half-period of the applied voltage.     

Dynamics of the spatial structure of pulsed discharges in dense gases in point cathode−plane anode gaps and their erosion effect on the plane electrode surface

The dynamics of the spatial structure of the plasma of pulsed discharges in air and nitrogen in a nonuniform electric field and their erosion effect on the plane anode surface were studied experimentally. It is established that, at a nanosecond front of the voltage pulse, a diffuse discharge forms in the point cathode–plane anode gap due to the ionization wave propagating from the cathode. As the gap length decreases, the diffuse discharge transforms into a spark. A bright spot on the anode appears during the diffuse discharge, while the spark channel forms in the later discharge stage. The microstructure of autographs of anode spots and spark channels in discharges with durations of several nanoseconds is revealed. The autographs consist of up to 100 and more microcraters 5–100 μm in diameter. It is shown that, due to the short duration of the voltage pulse, a diffuse discharge can be implemented, several pulses of which do not produce appreciable erosion on the plane anode or the soot coating deposited on it.     

Asymmetric long-wavelength surface modes of isotropic plasma waveguides

A theoretical study is made of the dispersion properties of electromagnetic surface waves with arbitrary azimuthal mode numbers and a small axial wavenumber in cylindrical isotropic waveguides partially filled with plasma. The plasma is assumed to be cold and radially inhomogeneous, and the problem is solved in the hydrodynamic approximation. The eigenfrequency of the waves is investigated as a function of the plasma parameters, the width and the permittivity of the dielectric gap between the metal waveguide wall and the plasma column, the axial wavenumber, and the azimuthal mode number. It is shown that the axial phase velocities of asymmetric surface modes are higher than the speed of light in a dielectric and that the surface modes do not propagate in a waveguide with a vanishingly small width of the dielectric gap. The theory developed is employed in practice in the calculation of the electrodynamic model of a gas discharges maintained by asymmetric long-wavelength surface modes. The power absorbed by the gas-discharge plasma in the regimes of Ohmic damping and resonant damping is calculated, and the plasma produced during the discharge is shown to be azimuthally homogeneous.     

On the theory of microwave discharges excited on the surface of a dielectric antenna

Microwave gas discharges excited near a dielectric surface are investigated. Such discharges can exist over a broad range of gas pressures and thereby can be used to solve a wide variety of applied problems. The wave dispersion properties favorable for discharge excitation are analyzed, and a kinetic discharge model is considered that can be used to calculate the discharge parameters. A model of a steady discharge at gas pressures of 10²–10⁴ Pa is constructed.     

Atmospheric-pressure electric discharge as an instrument of chemical activation of water solutions

Results of experimental studies and numerical simulations of physicochemical characteristics of plasmas generated in different types of atmospheric-pressure discharges (pulsed streamer corona, gliding electric arc, dielectric barrier discharge, glow-discharge electrolysis, diaphragmatic discharge, and dc glow discharge) used to initiate various chemical processes in water solutions are analyzed. Typical reactor designs are considered. Data on the power supply characteristics, plasma electron parameters, gas temperatures, and densities of active particles in different types of discharges excited in different gases and their dependences on the external parameters of discharges are presented. The chemical composition of active particles formed in water is described. Possible mechanisms of production and loss of plasma particles are discussed.     

Study of electric discharges between moving electrodes in air

A barrier electric discharge excited between a fixed electrode and a rotating electrode covered with a dielectric layer in atmospheric-pressure air is studied experimentally. A distinctive feature of this type of discharge is that it operates at a constant voltage between the electrodes. An advantage of the proposed method for plasma generation in the boundary layer of the rotating electrode (e.g., for studying the influence of plasma on air flows) is the variety of forms of the discharge and conditions for its initiation, simplicity of the design of the discharge system, and ease of its practical implementation     

Influence of the voltage polarity on the properties of a nanosecond surface barrier discharge in atmospheric-pressure air

The properties of a surface barrier discharge in atmospheric-pressure air at different polarities of applied voltage were studied experimentally. The influence of the voltage polarity on the spatial structure of the discharge and the electric field in the discharge plasma was determined by means of spectroscopic measurements. It is found that the energy deposited in the discharge does not depend on the voltage polarity and that discharges of positive polarity are more homogenous and the electric fields in them are higher.     

A prototype of an electric-discharge gas flow oxygen−iodine laser: I. Modeling of the processes of singlet oxygen generation in a transverse cryogenic slab RF discharge

The existing kinetic model describing self-sustained and electroionization discharges in mixtures enriched with singlet oxygen has been modified to calculate the characteristics of a flow RF discharge in molecular oxygen and its mixtures with helium. The simulations were performed in the gas plug-flow approximation, i.e., the evolution of the plasma components during their motion along the channel was represented as their evolution in time. The calculations were carried out for the O₂: He = 1: 0, 1: 1, 1: 2, and 1: 3 mixtures at an oxygen partial pressure of 7.5 Torr. It is shown that, under these conditions, volumetric gas heating in a discharge in pure molecular oxygen prevails over gas cooling via heat conduction even at an electrode temperature as low as ~100 K. When molecular oxygen is diluted with helium, the behavior of the gas temperature changes substantially: heat removal begins to prevail over volumetric gas heating, and the gas temperature at the outlet of the discharge zone drops to ~220–230 K at room gas temperature at the inlet, which is very important in the context of achieving the generation threshold in an electric-discharge oxygen?iodine laser based on a slab cryogenic RF discharge.     

Determination of the electron density and electric field in the plasma of a low-pressure microwave electrode discharge in hydrogen from the measured spectral line intensities

The parameters of the plasma of a microwave electrode discharge in hydrogen at pressures of 1–8 torr and incident powers of 20–80 W are measured by the so-called “relative intensity” method. The method allows one to determine the electron density and electric field in plasma by measuring the relative intensities of the H_α, H_β, and 763.5-nm Ar line emission and calculating the electron-impact rate constants from the homogeneous Boltzmann equation. The measurements show that there are regions in the discharge where the electron density is higher (a bright electrode sheath) and lower (a spherical region) than the critical density for the frequency 2.45 GHz (n_cr～7×10¹⁰ cm^?3). Inside the spherical region, the electric field varies slightly over the radius and the electron density increases as the discharge boundary is approached. The observed discharge structure can be attributed to the presence of a self-sustained discharge zone (electrode sheath); a non-self-sustained discharge zone (spherical region); and a decaying plasma region, which is separated from the active discharge zone by an electric double layer.