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1.
Ivan Valiela Coralie Barth-Jensen Thomas Stone John Crusius Sophia Fox Megan Bartholomew 《Biogeochemistry》2013,115(1-3):299-315
A series of eight watersheds on the Pacific coast of Panama where conversion of mature lowland wet forest to pastures by artisanal burning provided watershed-scale experimental units with a wide range of forest cover (23, 29, 47, 56, 66, 73, 73, 91, and 92 %). We used these watersheds as a landscape-scale experiment to assess effects of degree of deforestation on within-watershed retention and hydrological export of atmospheric inputs of nutrients. Retention was estimated by comparing rainfall nutrient concentrations (volume-weighted to allow for evapotranspiration) to concentrations in freshwater reaches of receiving streams. Retention of rain-derived nutrients in these Panama watersheds averaged 77, 85, 80, and 62 % for nitrate, ammonium, dissolved organic N, and phosphate, respectively. Retention of rain-derived inorganic nitrogen, however, depended on watershed cover: retention of nitrate and ammonium in pasture-dominated watersheds was 95 and 98 %, while fully forested watersheds retained 65 and 80 % of atmospheric nitrate and ammonium inputs. Watershed forest cover did not affect retention of dissolved organic nitrogen and phosphate. Exports from more forested watersheds yielded DIN/P near 16, while pasture-dominated watersheds exported N/P near 2. The differences in magnitude of exports and ratios suggest that deforestation in these Panamanian forests results in exports that affect growth of plants and algae in the receiving stream and estuarine ecosystems. Watershed retention of dissolved inorganic nitrogen calculated from wet plus dry atmospheric deposition varied from 90 % in pasture- to 65 % in forest-dominated watersheds, respectively. Discharges of DIN to receiving waters from the watersheds therefore rose from 10 % of atmospheric inputs for pasture-dominated watersheds, to about 35 % of atmospheric inputs for fully forested watersheds. These results from watersheds with no agriculture or urbanization, but different conversion of forest to pasture by burning, show significant, deforestation-dependent retention within tropical watersheds, but also ecologically significant, and deforestation-dependent, exports that are biologically significant because of the paucity of nutrients in receiving tropical stream and coastal waters. 相似文献
2.
Christiane Hudon Pierre Gagnon Myriam Rondeau Serge Hébert Denis Gilbert Brad Hill Michel Patoine Michel Starr 《Biogeochemistry》2017,132(3):251-272
Changes in atmospheric deposition, stream water chemistry, and solute fluxes were assessed across 15 small forested catchments. Dramatic changes in atmospheric deposition have occurred over the last three decades, including a 70% reduction in sulphur (S) deposition. These changes in atmospheric inputs have been associated with expected changes in levels of acidity, sulphate and base cations in streams. Soil retention of S appeared to partially explain rates of chemical recovery. In addition to these changes in acid–base chemistry we also observed unexpected changes in nitrogen (N) biogeochemistry and nutrient stoichiometry of stream water, including decreased stream N concentrations. Among all catchments the average flux of dissolved inorganic nitrogen (DIN) was best predicted by average runoff, soil chemistry (forest floor C/N) and levels of acid deposition (both S and N). The rate of change in stream DIN flux, however, was much more closely correlated with reductions in rates of S deposition rather than those of DIN. Unlike DIN fluxes, the average concentrations as well as the rates of decline in streamwater nitrate (NO3) concentration over time were tightly linked to stream dissolved organic carbon/dissolved organic nitrogen ratios DOC/DON and DON/TP rather than catchment characteristics. Declines in phosphorus adsorption with increasing soil pH appear to contribute to the relationship between C, N, and P in our study catchments. Our observations suggest that catchment P availability and its alteration due to environmental changes (e.g. acidification) might have profound effects on N cycling and catchment N retention that have been largely unrecognized. 相似文献
3.
本文对美国科罗拉多洛基山国家公园内LochVale,小流域溪流商边的湿地土壤水溶液中的含氮量进行了研究,并比较了与其相邻的溪流中的含氮量。结果发现,溪流中的硝态氮含量显著高于3个湿地土壤水溶液中的,而氨态氮则并没有显著差异;溪流水中的pH值要显著高于土壤水溶液中的,而电导率又显著低于后者。同时,还发现取自不同地点的溪流水分的化学性质也有显著的不同,采自溪流支流水分的pH,电导率和硝态氮都要显著高于取自主溪流中的水分的。另外,还分析比较了3个湿地样地的地上部分生产力以及土壤和生物量中的碳和全氮含量。最后,我们认为溪流两边的湿地对溪流中的氮的含量并没有显著的影响。 相似文献
4.
Andreas Musolff Benny Selle Olaf Büttner Michael Opitz Jörg Tittel 《Global Change Biology》2017,23(5):1891-1901
Reductions in emissions have successfully led to a regional decline in atmospheric nitrogen depositions over the past 20 years. By analyzing long‐term data from 110 mountainous streams draining into German drinking water reservoirs, nitrate concentrations indeed declined in the majority of catchments. Furthermore, our meta‐analysis indicates that the declining nitrate levels are linked to the release of dissolved iron to streams likely due to a reductive dissolution of iron(III) minerals in riparian wetland soils. This dissolution process mobilized adsorbed compounds, such as phosphate, dissolved organic carbon and arsenic, resulting in concentration increases in the streams and higher inputs to receiving drinking water reservoirs. Reductive mobilization was most significant in catchments with stream nitrate concentrations <6 mg L?1. Here, nitrate, as a competing electron acceptor, was too low in concentration to inhibit microbial iron(III) reduction. Consequently, observed trends were strongest in forested catchments, where nitrate concentrations were unaffected by agricultural and urban sources and which were therefore sensitive to reductions of atmospheric nitrogen depositions. We conclude that there is strong evidence that the decline in nitrogen deposition toward pre‐industrial conditions lowers the redox buffer in riparian soils, destabilizing formerly fixed problematic compounds, and results in serious implications for water quality. 相似文献
5.
本文对美国科罗拉多洛基山国家公园内Loch Vale小流域溪流两边的湿地土壤水溶液中的含氮量进行了研究,并比较了与其相邻的溪流中的含氮量。结果发现,溪流中的硝态氮含量显著高于3个湿地土壤水溶液中的,而氨态氮则并没有显著差异;溪流水中的pH值要显著高于土壤水溶液中的,而电导率又显著低于后者。同时,还发现取自不同地点的溪流水分的化学性质也显著的不同,采自溪流支流水分的pH,电导率和硝态氮都要显著高于取自主溪流中的水分的。另外,还分析比较了3个湿地样地的地上部分生产力以及土壤和生物量中的碳和全氮含量。最后,我们认为溪流两边的湿地对溪流中的氮的含量并没有显著的影响。 相似文献
6.
E. N. JACK BROOKSHIRE STEFAN GERBER JACKSON R. WEBSTER JAMES M. VOSE WAYNE T. SWANK 《Global Change Biology》2011,17(1):297-308
The microbial conversion of organic nitrogen (N) to plant available forms is a critical determinant of plant growth and carbon sequestration in forests worldwide. In temperate zones, microbial activity is coupled to variations in temperature, yet at the ecosystem level, microbial N mineralization seems to play a minor role in determining patterns of N loss. Rather, N losses often appear to vary with seasonality in hydrology and plant demand, while exports over longer periods are thought to be associated with increasing rates of anthropogenic N deposition. We analyzed long‐term (21–32 years) time series of climate and stream and atmospheric chemistry from two temperate deciduous forest watersheds in the southeastern USA to understand the sensitivity of internal forest N cycles to climate variation and atmospheric deposition. We evaluated the time series with a simple analytical model that incorporates key biotic constraints and mechanisms of N limitation and cycling in plant–soil systems. Through maximum likelihood analysis, we derive biologically realistic estimates of N mineralization and its temperature sensitivity (Q10). We find that seasonality and long‐term trends in stream nitrate (NO3) concentrations can in large part be explained by the dynamics of internal biological cycling responding to climate rather than external forcing from atmospheric chemistry. In particular, our model analysis suggests that much of the variation in N cycling in these forests results from the response of microbial activity to temperature, causing NO3 losses to peak in the growing season and to accelerate with recent warming. Extrapolation of current trends in temperature and N deposition suggests that the upturn in temperature may increase future N export by greater than threefold more than from increasing deposition, revealing a potential direct effect of anthropogenic warming on terrestrial N cycles. 相似文献
7.
Dissolved organic carbon (DOC) and NO3– are important forms of C and N in stream water. Hypotheses concerning relationships between DOC and NO3– concentrations have been proposed, but there are no reports demonstrating a relationship between them in stream water. We observed 35 natural streams in the Lake Biwa watershed, central Japan, and found an inverse relationship between DOC and NO3– concentrations. This relationship was also found in observations of their seasonal variations in the Lake Biwa watershed. Moreover, this relationship was also found to apply to watersheds in other regions in Japan. These results suggest that forest biogeochemical processes which control DOC and NO3– concentrations in Japanese streams are closely related. Excess N availability together with a C (energy) deficit in a soil environment may explain this relationship. DOC and NO3– concentrations in streams will thus be a useful index indicating C and N availability in catchments. 相似文献
8.
Melannie D. Hartman Jill S. Baron Holly A. Ewing Kathleen C. Weathers 《Biogeochemistry》2014,119(1-3):85-108
Concurrent changes in climate, atmospheric nitrogen (N) deposition, and increasing levels of atmospheric carbon dioxide (CO2) affect ecosystems in complex ways. The DayCent-Chem model was used to investigate the combined effects of these human-caused drivers of change over the period 1980–2075 at seven forested montane and two alpine watersheds in the United States. Net ecosystem production (NEP) increased linearly with increasing N deposition for six out of seven forested watersheds; warming directly increased NEP at only two of these sites. Warming reduced soil organic carbon storage at all sites by increasing heterotrophic respiration. At most sites, warming together with high N deposition increased nitrous oxide (N2O) emissions enough to negate the greenhouse benefit of soil carbon sequestration alone, though there was a net greenhouse gas sink across nearly all sites mainly due to the effect of CO2 fertilization and associated sequestration by plants. Over the simulation period, an increase in atmospheric CO2 from 350 to 600 ppm was the main driver of change in net ecosystem greenhouse gas sequestration at all forested sites and one of two alpine sites, but an additional increase in CO2 from 600 to 760 ppm produced smaller effects. Warming either increased or decreased net greenhouse gas sequestration, depending on the site. The N contribution to net ecosystem greenhouse gas sequestration averaged across forest sites was only 5–7 % and was negligible for the alpine. Stream nitrate (NO3 ?) fluxes increased sharply with N-loading, primarily at three watersheds where initial N deposition values were high relative to terrestrial N uptake capacity. The simulated results displayed fewer synergistic responses to warming, N-loading, and CO2 fertilization than expected. Overall, simulations with DayCent-Chem suggest individual site characteristics and historical patterns of N deposition are important determinants of forest or alpine ecosystem responses to global change. 相似文献
9.
Osamu Nakahara Masamichi Takahashi Hiroyuki Sase Toshiro Yamada Kazuhide Matsuda Tsuyoshi Ohizumi Haruo Fukuhara Takanobu Inoue Akiomi Takahashi Hiroyasu Kobayashi Ryusuke Hatano Tomoyuki Hakamata 《Biogeochemistry》2010,97(2-3):141-158
Rapid industrialization in East Asia is causing adverse effects due to atmospheric deposition in terrestrial and freshwater ecosystems. Decreasing stream pH and alkalinity and increasing NO3 ? concentrations were observed throughout the 1990s in the forested Lake Ijira catchment in central Japan. We investigated these changes using data on atmospheric deposition, soil chemistry, stream water chemistry, and forest growth. Average atmospheric depositions (wet + dry) of 0.83, 0.57, and 1.37 kmol ha?1 year?1 for hydrogen, sulfur, and nitrogen, respectively, were among the highest levels in Japan. Atmospheric deposition generally decreased before 1994 and increased thereafter. The catchment was acid-sensitive; stream alkalinity was low (134 μmolc l?1) and pH in surface mineral soils decreased from 4.5 in 1990 to 3.9 in 2003. Stream NO3 ? concentration nearly doubled (from 22 to 42 μmolc l?1) from the late 1980s to the early 2000s. Stream NO3 ? concentration was controlled primarily by water temperature before 1996/1997 and by stream discharge thereafter. Stream NO3 ? concentrations decreased during the growing season before 1996/1997, but this seasonality was lost thereafter. The catchment became nitrogen-saturated (changing from stage 1 to 2) in 1996/1997, possibly because of declining forest growth rates due to the 1994 summer drought, defoliation of Japanese red pine by pine wilt disease, maturation of Japanese cedar stands, and stimulation of nitrogen mineralization and nitrification due to alkalinization of soils (increased exchangeable Ca2+ and soil pH) after the summer drought. Stream pH and alkalinity began decreasing in 1996/1997. The enhanced growing-season NO3 ? discharge since 1996/1997 appeared to be the major cause of stream acidification. Increased atmospheric deposition since 1994 may have contributed to this change. 相似文献
10.
Leaching losses of nitrate from forests can have potentially serious consequences for soils and receiving waters. In this
study, based on extensive sampling of forested watersheds in the Catskill Mountains of New York State, we examine the relationships
among stream chemistry, the properties of the forest floor, and the tree species composition of watersheds. We report the
first evidence from North America that nitrate export from forested watersheds is strongly influenced by the carbon:nitrogen
(C:N) ratio of the watershed soils. We also show that variation in soil C:N ratio is associated with variation in tree species
composition. This implies that N retention and release in forested watersheds is regulated at least in part by tree species
composition and that changes in species composition caused by introduced pests, climate change, or forest management could
affect the capacity of a forest ecosystem to retain atmospherically deposited N.
Received 4 March 2002; Accepted 4 June 2002. 相似文献
11.
Does Anthropogenic Nitrogen Enrichment Increase Organic Nitrogen Concentrations in Runoff from Forested and Human-dominated Watersheds? 总被引:1,自引:0,他引:1
Although the effects of anthropogenic nitrogen (N) inputs on the dynamics of inorganic N in watersheds have been studied extensively,
“the influence of N enrichment on organic N loss” is not as well understood. We compiled and synthesized data on surface water
N concentrations from 348 forested and human-dominated watersheds with a range of N loads (from less than 100 to 7,100 kg
N km−2 y−1) to evaluate the effects of N loading via atmospheric deposition, fertilization, and wastewater on dissolved organic N (DON)
concentrations. Our results indicate that, on average, DON accounts for half of the total dissolved N (TDN) concentrations
from forested watersheds, but it accounts for a smaller fraction of TDN in runoff from urban and agricultural watersheds with
higher N loading. A significant but weak correlation (r
2 = 0.06) suggests that N loading has little influence on DON concentrations in forested watersheds. This result contrasts
with observations from some plot-scale N fertilization studies and suggests that variability in watershed characteristics
and climate among forested watersheds may be a more important control on DON losses than N loading from atmospheric sources.
Mean DON concentrations were positively correlated, however, with N load across the entire land-use gradient (r
2 = 0.37, P < 0.01), with the highest concentrations found in agricultural and urban watersheds. We hypothesize that both direct contributions
of DON from wastewater and agricultural amendments and indirect transformations of inorganic N to organic N represent important
sources of DON to surface waters in human-dominated watersheds. We conclude that DON is an important component of N loss in
surface waters draining forested and human-dominated watersheds and suggest several research priorities that may be useful
in elucidating the role of N enrichment in watershed DON dynamics. 相似文献
12.
Fate and Transport of Organic Nitrogen in Minimally Disturbed Montane Streams of Colorado,USA 总被引:1,自引:0,他引:1
In two montane watersheds that receive minimal deposition of atmospheric nitrogen, 15–71% of dissolved organic nitrogen (DON)
was bioavailable in stream water over a 2-year period. Discharge-weighted concentrations of bulk DON were between 102 and
135 μg/l, and the C:N ratio differed substantially between humic and non-humic fractions of DON. Approximately 70% of DON export
occurred during snowmelt, and 40% of that DON was biologically available to microbes in stream sediments. Concentrations of
bioavailable DON in stream water were 2–16 times greater than dissolved inorganic nitrogen (DIN) during the growing season,
and bioavailable DON was depleted within 2–14 days during experimental incubations. Uptake of DON was influenced by the concentration
of inorganic N in stream water, the concentration of non-humic DON in stream water, and the C:N ratio of the non-humic fraction
of dissolved organic matter (DOM). Uptake of DON declined logarithmically as the concentration of inorganic N in stream water
increased. Experimental additions of inorganic N also caused a decline in uptake of DON and net production of DON when the
C:N ratio of non-humic DOM was high. This study indicates that the relative and absolute amount of bioavailable DON can vary
greatly within and across years due to interactions between the availability of inorganic nutrients and composition of DOM.
DOM has the potential to be used biotically at a high rate in nitrogen-poor streams, and it may be generated by heterotrophic
microbes when DIN and labile DOM with low relative nitrogen content become abundant. 相似文献
13.
Stream water dissolved organic carbon (DOC) correlates positively with soil organic carbon (SOC) in many biomes. Does this relationship hold in a small geographic region when variations of temperature, precipitation and vegetation are driven by a significant altitudinal gradient? We examined the spatial connectivity between concentrations of DOC in headwater stream and contents of riparian SOC and water-soluble soil organic carbon (WSOC), riparian soil C:N ratio, and temperature in four vegetation types along an altitudinal gradient in the Wuyi Mountains, China. Our analyses showed that annual mean concentrations of headwater stream DOC were lower in alpine meadow (AM) than in subtropical evergreen broadleaf forest (EBF), coniferous forest (CF), and subalpine dwarf forest (SDF). Headwater stream DOC concentrations were negatively correlated with riparian SOC as well as WSOC contents, and were unrelated to riparian soil C:N ratio. Our findings suggest that DOC concentrations in headwater streams are affected by different factors at regional and local scales. The dilution effect of higher precipitation and adsorption of soil DOC to higher soil clay plus silt content at higher elevation may play an important role in causing lower DOC concentrations in AM stream of the Wuyi Mountains. Our results suggest that upscaling and downscaling of the drivers of DOC export from forested watersheds when exploring the response of carbon flux to climatic change or other drivers must done with caution. 相似文献
14.
Long-term watershed research conducted in Shenandoah National Park (SNP) in Virginia and elsewhere in the eastern U.S. indicates that annual export of dissolved nitrogen (N) from gaged forested watersheds to surface waters increases dramatically in response to vegetation disturbances. Dissolved N leakage is a common, well-documented response of small forested watersheds to logging in the larger region, while recent defoliation outbreaks of the gypsy moth ( Lymantria dispar) larva in the deciduous forests of SNP have been shown to generate similar biogeochemical responses. A recent modeling analysis further suggests that a parsimonious, empirical, unit N export response function (UNERF) model can explain large percentages of the temporal variation in annual N export from a group of small gaged forested watersheds in the years following disturbance. The empirical UNERF modeling approach is completely analogous to the unit hydrograph technique for describing storm runoff, with the model representing annual N export as a linear deterministic process both in space and in time. The purposes of this analysis are to (1) test the applicability of the UNERF model using quarterly streamwater nitrate data from a group of ungaged watersheds in SNP; (2) demonstrate a park-wide application of a regional UNERF model that references the geographic distributions of bedrock geology and the timing and extent of gypsy moth defoliation over the entire SNP area; and (3) visualize the temporal and spatial patterns in vegetation disturbance and annual dissolved N export through the use of computer animation software. During water year 1992, the year of peak defoliation, our modeling study suggests that park-wide export had transiently increased by 1700% from a baseline rate of about 0.1 kg/ha/year. SNP forests appear to be characteristic of other N-limited second-growth forests in the eastern U.S. that leak little N under undisturbed conditions, despite receiving relatively large inputs of N from atmospheric deposition sources. Vegetation disturbances can apparently cause major changes in N input-output balances with potentially important ramifications for low-order forest streams and downstream receiving waters. 相似文献
15.
Stottlemyer R 《TheScientificWorldJournal》2001,1(Z2):581-588
There is much interest in the relationship of atmospheric nitrogen (N) inputs to ecosystem outputs as an indicator of possible "nitrogen saturation" by human activity. Longer-term, ecosystem-level mass balance studies suggest that the relationship is not clear and that other ecosystem processes may dominate variation in N outputs. We have been studying small, forested watershed ecosystems in five northern watersheds for periods up to 35 years. Here I summarize the research on ecosystem processes and the N budget. During the past 2 decades, average wet-precipitation N inputs ranged from about 0.1 to 6 kg N ha(-1) year(-1) among sites. In general, sites with the lowest N inputs had the highest output-to-input ratios. In the Alaska watersheds, streamwater N output exceeded inputs by 70 to 250%. The ratio of mean monthly headwater nitrate (NO3-) concentration to precipitation NO3- concentration declined with increased precipitation concentration. A series of ecosystem processes have been studied and related to N outputs. The most important appear to be seasonal change in hydrologic flowpath, soil freezing, seasonal forest-floor inorganic N pools resulting from over-winter mineralization beneath the snowpack, spatial variation in watershed forest-floor inorganic N pools, the degree to which snowmelt percolates soils, and gross soil N mineralization rates. 相似文献
16.
Increased nitrogen deposition has resulted in increased nitrogen pools and nitrogen leaching in European and North American forest soils. The development in Asia in general, and China in particular, suggests increased deposition of reduced nitrogen from changes in agricultural practices and of oxidized nitrogen from rapid growth of the transportation sector. Decreased nitrogen retention in forested areas in the future may cause increased NO3- leaching and, thus, acidification and eutrophication in surface waters. The differences in climate, ecosystems, land use, and deposition history make direct application of knowledge from studies in Europe and North America difficult. In Southwest China the potential for nitrogen mobilization from forest soils may be high because of the warm and humid climate, resulting in high decomposition rates of soil organic matter. However, there are very few data available for quantifying the suspected potential for increased nitrogen leaching in forest ecosystems. Here we present data from two forested catchments, dominated by Masson pine (Pinus massoniana), near Guiyang and Chongqing, respectively, in Southwest China. The present nitrogen deposition is moderate, estimated in the range from 10 to 40 kg N ha(-1) year(-1). The C/N ratios of the soils are generally below 15. Nitrate concentrations in soil water are rather variable in space, with highest values of several hundred microequivalents per liter. The turnover rate of nitrogen in the forest ecosystem is quite high compared to the atmospheric deposition rate. At present, nitrate runoff from the catchments is low and intermediate in Guiyang and Chongqing, respectively. More research is needed to improve our ability to predict future nitrogen leaching from subtropical Asian coniferous forests. 相似文献
17.
Impact of N-Saturated Upland Forests on Downstream N Pollution in the Tatara River Basin, Japan 总被引:1,自引:0,他引:1
This study evaluated whether nitrogen (N) saturated upland forests can degrade downstream water quality in the Tatara River
Basin, northern Kyushu, western Japan. Our hypothesis is that elevated atmospheric N deposition degrades downstream water
quality in a watershed containing N-saturated forests because a considerable amount of atmospherically deposited N passes
into the streams without being retained. Synoptic stream water samplings were conducted at 23 sites across a wide range of
land-use categories in the basin over 1 year. A long-term temporal analysis of downstream water quality over the last 30 years
(1977–2007) was conducted and compared with long-term trends in related factors such as urban/agricultural activity, sewage
wastewater treatment, atmospheric N deposition, and forest condition. The results showed that atmospherically deposited N
to N-saturated forests can be a large enough non-point source of N leaving the watershed to impact downstream water quality.
This was highlighted by the reduction in pollutant exports derived from urban/agricultural activities, an increase in atmospheric
N deposition, and the maturation of coniferous plantation forests in the past 30 years. These have led to reductions in total
phosphorus and organic nitrogen concentrations in downstream water, whereas downstream nitrate (NO3
−) concentrations increased over the last 30 years. The consequent increase in the downstream N:P ratio indicated P limitation.
Reducing the NO3
− exports from N-saturated upland forests is suggested as a strategy to improve regional downstream NO3
− pollution, but involves intercontinental-scale action in reducing atmospheric N emissions. 相似文献
18.
Nitrogen (N) Dynamics in the Mineral Soil of a Central Appalachian Hardwood Forest During a Quarter Century of Whole-Watershed N Additions 总被引:1,自引:0,他引:1
Frank S. Gilliam Christopher A. Walter Mary Beth Adams William T. Peterjohn 《Ecosystems》2018,21(8):1489-1504
The structure and function of terrestrial ecosystems are maintained by processes that vary with temporal and spatial scale. This study examined temporal and spatial patterns of net nitrogen (N) mineralization and nitrification in mineral soil of three watersheds at the Fernow Experimental Forest, WV: 2 untreated watersheds and 1 watershed receiving aerial applications of N over a 25-year period. Soil was sampled to 5 cm from each of seven plots per watershed and placed in two polyethylene bags—one bag brought to the laboratory for extraction/analysis, and the other bag incubated in situ at a 5 cm depth monthly during growing seasons of 1993–1995, 2002, 2005, 2007–2014. Spatial patterns of net N mineralization and nitrification changed in all watersheds, but were especially evident in the treated watershed, with spatial variability changing non-monotonically, increasing then decreasing markedly. These results support a prediction of the N homogeneity hypothesis that increasing N loads will increase spatial homogeneity in N processing. Temporal patterns for net N mineralization and nitrification were similar for all watersheds, with rates increasing about 25–30% from 1993 to 1995, decreasing by more than 50% by 2005, and then increasing significantly to 2014. The best predictor of these synchronous temporal patterns across all watersheds was number of degree days below 19°C, a value similar to published temperature maxima for net rates of N mineralization and nitrification for these soils. The lack of persistent, detectable differences in net nitrification between watersheds is surprising because fertilization has maintained higher stream-water nitrate concentrations than in the reference watersheds. Lack of differences in net nitrification among watersheds suggests that N-enhanced stream-water nitrate following N fertilization may be the result of a reduced biotic demand for nitrate following fertilization with ammonium sulfate. 相似文献
19.
The effects of forest on stream water quality in two coastal plain watersheds of the Chesapeake Bay 总被引:2,自引:0,他引:2
Forest had varying effects on stream nutrients in two coastal plain basins of the Delmarva Peninsula, USA. In the Choptank basin, forest was strongly associated with low stream total nitrogen (TN) and nitrate (NO3−) concentrations (r20.70), and forest placement along first order streams was important in maintaining low stream nitrogen (N) concentrations (r20.35). In addition, a multiple regression model explained 40% of the stream total phosphorus (TP) variance and indicated that forest directly adjacent to streams (0–100 m) acted as a TP source and forest further away (100–300 m) from streams acted as a TP sink. In contrast, stream nutrients in the nearby Chester basin demonstrated a strong relationship with soil hydrologic properties. Forest had no significant effect on stream N and P because the finer-textured soils, higher stream slopes, and higher runoff potential of the Chester basin appeared to result in less baseflow compared to that in the Choptank basin. This reduced the opportunity for forest to intercept N via plant uptake and denitrification in the high runoff potential soils of the Chester basin. The high percentage of stormflow (40%) coupled with high stream slopes resulted in high soil erosion potential, which may explain the higher TP stream concentrations measured in the Chester compared to that in the Choptank. Differences in the hydrologic pathway appear to explain the different effects of forest on water quality in these two basins. 相似文献
20.
Concentrations of soluble reactive phosphorus (SRP), nitrate, and soluble reactive silicon (SRSi) were monitored in 12 streams
draining small catchments (<10 km2) in the English Lake District. The catchments varied with respect to underlying geology,
soil type and land cover. Average concentrations of SRP were in the range 0.5–11.2 μg P l-1, and estimated loads ranged from
0.01 to 0.14 kg P ha-1 a-1. The higher concentrations and loads were associated with catchments containing improved pasture.
Mean streamwater concentrations of nitrate varied from 55 to 660 μg N l-1, while loads were in the range 0.8–9.6 kg N ha-1
a-1; no general dependence on catchment properties was discerned. Concentrations of SRSi were similar in all the streams (0.8–2
mg Si l-1), and annual loads were in the range 10–26 kg Si ha-1 a-1. Loads of all three nutrients were greatest during the
winter, because of higher discharges, but in some catchments containing improved pasture, considerable transport of P also
took place during the summer. Concentrations of nitrate in streams draining unimproved moorland catchments are approximately
twice those reported for samples taken from similar streams in 1973 and 1974, possibly because of increased atmospheric deposition
of inorganic nitrogen (ammonium and nitrate). Concentrations of SRP in such streams were similar to those reported for the
earlier samples. Comparisons of stream loads of SRP and nitrate with estimated inputs suggest that catchment soils retain
substantial amounts of these nutrients. Implications for surface water eutrophication of changes in P retention by soils are
discussed.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献