Formation of a strong electric field resulting in the excitation of microplasma discharges at the edge of a dielectric film on a metal in a plasma flow

Results are presented from experimental and analytical studies of the processes resulting in the excitation of microplasma discharges (MPDs) on a metal surface partially covered with a thin dielectric film under the action of an external plasma flow in vacuum. It is shown experimentally that MPDs are excited at the interface between the open metal surface and the region covered by the dielectric film. The probability of MPD excitation is investigated as a function of the thickness of the dielectric film deposited on the metal. It is found that, for a film thickness of 1 μm, the probability of MPD excitation is close to unity. As the film thickness decreases below ~10 nm or increases above ~10 μm, the probability of MPD excitation is reduced by more than two orders of magnitude. A two-dimensional kinetic numerical code is developed that allows one to model the processes of Debye sheath formation and generation of a strong electric field near the edge of a finite-thickness dielectric film on a metal surface in a plasma flow for different configurations of the film edge. It is shown that the maximum value of the tangential component of the electric field is reached at the film edge and amounts to E _max ≈ |φ₀|/2d (where φ₀ < 0 is the electric potential applied to the metal and d is the film thickness), which for typical conditions of experiments on the excitation of MPDs on metal surfaces (φ₀ ≈–400 V, d ≈ 1 μm) yields E _max ≈ 2 MV/cm. The results of kinetic simulations confirm the qualitative idea about the mechanism of the formation of a strong electric field resulting in the excitation of MPDs at the edge of a dielectric film on a metal surface in a plasma flow and agree with experimental data.     

Effect of microplasma discharges on aluminum surfaces

Excitation of microplasma discharges on the surfaces of V95 aluminum alloy samples placed in a uniform pulsed plasma flow was studied experimentally. Strong localized interaction of microplasma discharges with aluminum leads to the melting and subsequent fast cooling of micrometer-size regions on the sample surface. Due to the multiple action of microplasma discharges, a continuous remelted layer with a thickness of up to 20 μm forms on the aluminum surface. The physical, structural, and tribotechnical properties of this layer differ substantially from those before microplasma processing.     

Strong localized interaction of microplasma discharges with titanium

Excitation of microplasma discharges on the surfaces of titanium samples placed in a uniform pulsed plasma flow was studied experimentally. Strong localized interaction of microplasma discharges with titanium leads to the rapid melting and subsequent fast cooling of micrometer-size regions on the sample surface. Due to the multiple action of microplasma discharges, a continuous remelted layer with a thickness of up to 20 μm forms on the titanium surface. The physical, structural, and tribotechnical properties of this layer differ substantially from those before microplasma processing.     

Propagation of Microplasma Discharge over Titanium Surface Covered with Thin Dielectric Film

Plasma Physics Reports - Propagation and structure of the pulsed microplasma discharge initiated on the titanium sample surface covered with a thin dielectric film with a thickness of approximately...     

Determination of the electron temperature in microplasma discharges excited on a titanium surface

Results are presented from experimental studies of the emission spectra of microplasma discharges excited on a titanium surface by a pulsed plasma flow. The excited discharges are maintained by current pulses with an amplitude of 200 A and a duration of 20 ms. Analysis of more than 100 spectral lines of titanium atoms and ions in the wavelength range of 350–800 nm shows that the electron temperature of a microplasma discharge is in the range of 0.2–1.3 eV.     

Creation of a hard microrelief on a titanium surface processed by microplasma discharges with a current amplitude of 200 A and pulse duration of 20 ms

The interaction of microplasma discharges with samples made of VT1 commercial titanium was studied experimentally. The amplitude of the current pulses of microplasma discharges was 200 A, the pulse duration was 20 ms, and the number of current pulses was from 1 to 10. After microplasma processing, a 10-μm-thick solid remelted surface layer with an increased hardness formed on the titanium samples. As compared to the initial state of titanium samples, the surface layer hardened by microplasma discharges possesses improved parameters: the microhardness increases fivefold, the maximum admissible pressure applied to the samples during friction increases more than 20-fold, the friction wear rate is reduced by three orders of magnitude, and the friction coefficient decreases sixfold.     

Theory of propagation of ordinary surface cyclotron waves

The dispersion properties of ordinary surface cyclotron waves in a semiinfinite nonuniform plasma are investigated. The waves propagate across the external magnetic field directed along the plasma surface in a metal waveguide the internal surface of which is covered with a dielectric. The problem is solved analytically in the framework of a kinetic model for plasma particles under the assumption of weak spatial dispersion. The influence of the parameters of the dielectric layer separating the plasma from the metal wall, the shape of the plasma density profile, and the value of the external magnetic field on the dispersion properties of surface cyclotron waves is studied both numerically and analytically.     

Azimuthally asymmetric eigenmodes of a magnetized plasma cylinder around a dielectric rod in a circular waveguide

The electrodynamics of a circular waveguide with a dielectric rod surrounded by a magnetized plasma layer is considered. A general dispersion relation for azimuthally asymmetric perturbations is derived, and its solutions describing slow waves—specifically, electromagnetic and plasma modes, as well as (and primarily) hybrid waves that combine the properties of both mode types—are investigated numerically. For the fundamental waveguide mode of the system—the HE₁₁ mode—the parameters of the plasma layer are determined at which the mode cannot be subject to Cherenkov interaction with a relativistic electron beam at a given frequency. For both waveguide and plasma modes, the radial profiles of the longitudinal components of the electric field and Poynting vector, the fractions of RF power carried within the dielectric and plasma regions and vacuum gap, and the coupling impedance are calculated as functions of the parameters of the plasma layer. The evolution of the field structure during the formation of asymmetric hybrid waves is traced. The results of calculating the dispersion and coupling impedance are analyzed as applied to an antenna-amplifier—a relativistic traveling-wave tube operating on the HE₁₁ mode of the dielectric rod: specifically, the implementability of the concept in the presence of a plasma at the rod surface is estimated, and the possible role of azimuthally asymmetric and symmetric plasma modes is examined.     

Wall plasma in a wideband dielectric cherenkov maser

Results are reported of experimental investigations that have revealed the presence of a plasma in the interaction region of a model wideband relativistic microwave amplifier—a dielectric Cherenkov maser. The electrodynamic properties of a hybrid system—a waveguide with an annular dielectric liner and a plasma layer adjacent to its inner wall—are analyzed. Experiments with a high-current accelerator have revealed that the power of the emitted microwaves at the output of the system increases strongly when an external microwave source at different frequencies in the X-band is switched on. However, this effect was found to be hard to reproduce. Indirect evidence is obtained of the fact that, during the transport of an electron beam and under the action of the signal from a high-power pulsed magnetron, the plasma in the system is created at the surface of the dielectric. In the model of a cold magnetized plasma, a dispersion relation is derived for axisymmetric waves in a system with a wall plasma layer. The spectra of the waveguide and plasma modes in the system and the transverse structure of their electromagnetic fields are investigated thoroughly as functions of the plasma density and layer thickness. It is shown that even a very thin layer of a high-density plasma results in a large frequency shift of the dispersion curve of the waveguide mode, in which case the coupling impedance at a fixed frequency decreases sharply. On the other hand, a layer of a moderately dense plasma increases the coupling impedance for the waveguide mode. It is established that, in a configuration with a wall plasma layer, the longitudinal component of the electric field of a plasma mode whose power flux in the dielectric is of a volumetric nature reverses direction across the layer.     

Plasmon Polariton Imaging Characteristics of Near-Field Optical Fiber Probes

The influence of different near-field optical (near-field scanning optical microscopy) probes on the imaging of surface plasmon polaritons propagating on thin metal films is investigated. Metal-coated fiber probes exhibit a suppression of the measured plasmon signal close to the metal film surface and increased local scattering of the plasmon field. Purely dielectric fiber probes are shown to be largely free of these effects.     

Coupled plasmon-waveguide resonators: a new spectroscopic tool for probing proteolipid film structure and properties.

A variant of surface plasmon resonance (SPR) spectroscopy has been developed that involves a coupling of plasmon resonances in a thin metal film and waveguide modes in a dielectric overcoating. This new technique is referred to as coupled plasmon-waveguide resonance (CPWR) spectroscopy. It combines a greatly enhanced sensitivity (due to increased electromagnetic field intensities at the dielectric surface) and spectral resolution (due to decreased resonance linewidths), with the ability to directly measure anisotropies in refractive index and optical absorption coefficient in a dielectric film adsorbed onto the surface of the overcoating. Experimental data obtained with an egg phosphatidylcholine bilayer are presented to document these properties.     

Asymmetric long-wavelength surface modes of isotropic plasma waveguides

A theoretical study is made of the dispersion properties of electromagnetic surface waves with arbitrary azimuthal mode numbers and a small axial wavenumber in cylindrical isotropic waveguides partially filled with plasma. The plasma is assumed to be cold and radially inhomogeneous, and the problem is solved in the hydrodynamic approximation. The eigenfrequency of the waves is investigated as a function of the plasma parameters, the width and the permittivity of the dielectric gap between the metal waveguide wall and the plasma column, the axial wavenumber, and the azimuthal mode number. It is shown that the axial phase velocities of asymmetric surface modes are higher than the speed of light in a dielectric and that the surface modes do not propagate in a waveguide with a vanishingly small width of the dielectric gap. The theory developed is employed in practice in the calculation of the electrodynamic model of a gas discharges maintained by asymmetric long-wavelength surface modes. The power absorbed by the gas-discharge plasma in the regimes of Ohmic damping and resonant damping is calculated, and the plasma produced during the discharge is shown to be azimuthally homogeneous.     

Study of the surface barrier discharge generated by electrodes in the form of a series of parallel metal strips

A surface discharge in a system where metal electrodes in the form of a series of parallel strips are positioned on the dielectric surface is studied. Analytical formulas for calculating the spatial distribution of the potential and the electric field in a discharge cell are derived. It is shown that the geometry of the metal electrodes should be taken into account (along with physical and chemical characteristics of the dielectric, the voltage applied to the electrodes, and other parameters of the system) for generation of the electric field with optimal configuration in the discharge cell. The obtained results are also applicable for analysis of discharge cells with a coplanar barrier discharge where metal electrodes are positioned in the dielectric at small depths. The results are of interest since a barrier discharge is one of the efficient methods for generating non-equilibrium plasma at high pressures for a variety of technological applications.     

Some features of imaging of the processes occurring in an extended arc discharge in atmospheric-pressure air

Processes occurring in the low-temperature plasma of extended quasi-stationary arc discharges in air between graphite electrodes are investigated. Along with the conventional (constricted) discharge geometry, other discharge modes—diffuse (distributed) and diffuse-constricted—are studied. Contraction, stratification, and shunting processes are considered. Current oscillation modes are revealed that are caused by the interaction between the cathode and anode jets and the origination of plasma jets and solid particles from the locally overheated anode surface. 1 The use of graphite electrodes with standard atmospheric pressure excludes the presence of the liquid phase in the electrode spots     

Interaction of a high-current electron beam with hybrid waveguide and plasma modes in a dielectric Cherenkov maser with a plasma layer

The characteristics of a high-current electron beam-driven microwave amplifier—a dielectric Cherenkov maser—are investigated in the framework of linear theory for the case of a plasma layer present at the surface of the maser slow-wave structure. The dispersion relation for axisymmetric perturbations is obtained for the conventional configuration (a circular dielectric-lined waveguide and a thin annular beam propagating within the vacuum region inside the annular plasma) in the model of a fully magnetized plasma and beam. The results of numerically solving the dispersion relation for different beam and plasma parameters are presented, and an analysis based on these results is given with regard to the features of the beam interaction with the hybrid waves of the system (both hybrid waveguide and hybrid plasma modes). For the hybrid waveguide mode, the dependences of the spatial growth rate on the frequency demonstrate an improvement in the gain at moderate plasma densities, along with narrowing the amplification band and shifting it toward higher frequencies. For the hybrid plasma mode, the interaction with a mildly relativistic (200–250 keV) beam, when the wave phase velocity is close to the speed of light in the dielectric medium, is most interesting and, therefore, has been studied in detail. It is shown that, depending on the beam and plasma parameters, different regimes of the hybrid plasma mode coupling to the hybrid waveguide mode or a usual, higher order plasma mode take place; in particular, a flat gain vs. frequency dependence is possible over a very broad band. The parameters at which the ?3-dB bandwidth calculated for the 30-dB peak gain exceeds an octave are found.     

Influence of the shape of the cross section of a plasma-dielectric interface on the dispersion properties of high-frequency azimuthal surface modes

Theoretical study of the propagation of a packet of surface electromagnetic surface waves with a zero axial wavenumber in a circular-cross-section cylindrical metal waveguide within the frequency range that is higher than upper hybrid resonance is carried out. The waveguide is partially filled by plasma and immersed into axial magnetic field. The cross section of the plasma column is assumed to differ from circular shape. The effect of this shape on the dispersion properties of azimuthal surface modes is investigated by the method of successive approximations. The fields of the waves and their eigenfrequencies are determined up to terms of the second order in the deviation of the plasma cross section shape from the ring one. The correction to the eigenfrequency of azimuthal surface modes caused by this feature of the plasma column section is proved to increase with decreasing the external magnetic field and increasing the value of the dielectric constant of the dielectric, that separates the plasma from the metal wall of the waveguide. The spectral composition of the wave packet, in the form of which these modes propagate, is studied. The amplitudes of the satellite harmonics of these modes are found to increase with increasing the plasma density and decreasing the external magnetic field.     

Selective enhancement of Raman or fluorescence spectra of biomolecules using specifically annealed thick gold films

Annealing of "thick" metal films deposited onto a smooth dielectric substrate leads to high-order self-organization of metal clusters on the film surface. This work presents the first experimental evidence that the "thick" gold film (TGF) may be specifically annealed to serve as a substrate for surface-enhanced fluorescence or surface-enhanced Raman scattering (SERS) spectroscopy of the same molecule. High-resolved SERS spectra of mitoxantrone (mitox) were recorded on the TGF annealed at 340 degrees C whereas no Raman enhancement but an increase of mitox fluorescence signal were detected on the TGF annealed at 240 degrees C. The mitox fluorescence was further enhanced by deposition of monolayers of pentanethiol or poly-L-lysine on the surface of annealed TGF. The maximal fluorescence enhancement factor per mitox molecule of approximately 50 that was obtained on the annealed TGF covered with poly-L-lysine makes the system promising for applications in immunofluorescence assays and in microspectrofluorescence analysis.     

Surface Plasmon Polariton Propagation at the Interface of a Metal and an Ambichiral Nanostructured Medium

The propagation of a surface plasmon polariton wave at the interface of a metal and an ambichiral nanostructured medium was theoretically investigated in the Kretschmann configuration using transfer matrix method. The dependence of optical absorption linear polarization on structural parameters was reported. The results were compared with those obtained from the interface of a metal and a chiral dielectric medium as a reference structure. We found that multiple plasmon modes are excited at the interface of metal and ambichiral dielectric medium. Our calculations revealed that there exist five plasmon modes for chiral, trigonal, and tetragonal structures; three plasmon modes for pentagonal structure; two plasmon modes for hexagonal structure; and one plasmon mode for dodecagonal structure that propagate with different phase speeds. The obtained results showed that only one plasmon mode occurs at all pitches, while other modes exist at some of the pitches of anisotropic chiral and ambichiral dielectric mediums. The time-averaged Poynting vector versus the thickness of metal film confirmed that the energy of photons of incident light is transferred to surface plasmon polariton quasiparticles and the surface plasmon polariton wave is localized at the interface of metal and ambichiral dielectric medium.     

Structure of the surface streamers of an AC barrier corona in argon

Results are presented from experimental studies of the structure of an ac surface discharge excited by a metal needle over a plane dielectric surface. A barrier corona discharge was ignited in atmospheric-pressure argon at frequencies of the applied sinusoidal voltage from 50 Hz to 30 kHz. In experiments, the area of a dielectric covered with the discharge plasma increased with applied voltage. The discharge structure in diffuse and streamer modes was recorded using a digital camera and a high-speed image tube operating in a frame mode. It is found that, in the positive and negative half-periods of the applied voltage, the structure of the surface discharge is substantially different. The statistical characteristics of the branching surface streamers in the positive and negative half-periods are determined as functions of the voltage frequency. The most intense lines in the emission spectrum of the barrier corona are determined for both half-periods. The correlation between the dynamics of the emission intensity and the dynamics of the discharge current and voltage is investigated.     

A powerful electrohydrodynamic flow generated by a high-frequency dielectric barrier discharge in a gas

Theoretical and experimental studies of an electrohydrodynamic flow induced by a high-frequency dielectric barrier discharge distributed over a dielectric surface in a gas have been conducted. Dependences of the ion current, the gas flow velocity, and the spatial distributions thereof on the parameters of the power supply of the plasma ion emitter and an external electric field determined by the collector grid voltage have been described.