An annular high-current electron beam with an energy spread in a coaxial magnetically insulated diode

An elementary theory of an annular high-current electron beam in a uniform transport channel and a coaxial magnetically insulated diode is generalized to the case of counterpropagating electron beams with a spread over kinetic energies. Expressions for the sum of the absolute values of the forward and backward currents in a uniform transport channel and for the flux of the longitudinal component of the generalized momentum in a coaxial magnetically insulated diode as functions of the maximum electron kinetic energy are derived for different values of the relative width of the energy distribution function. It is shown that, in a diode with an expanding transport channel and a virtual cathode limiting the extracted current, counterpropagating particle flows are established between the cathode and the virtual cathode within a certain time interval after the beginning of electron emission. The accumulation of electrons in these flows is accompanied by an increase in their spread over kinetic energies and the simultaneous decrease in the maximum kinetic energy. The developed model agrees with the results of particle-in-cell simulations performed using the KARAT and OOPIC-Pro codes.     

Energy distribution of runaway electrons generated by a nanosecond discharge in atmospheric-pressure air

The spectra of an ultrashort avalanche electron beam generated by a nanosecond discharge in atmospheric-pressure air were investigated. The temporal characteristics of the beam current pulses, gap voltage, and discharge current in a gas diode were measured with a time resolution of ～0.1 ns. A simple technique was developed for recovering electron spectra from the curves of beam attenuation by aluminum foils. The effect of the cathode design, electrode gap length, and generator parameters on the electron spectra were studied using seven setups. It is shown that generation of electrons with anomalously high energies requires the use of cathodes with increased curvature radius.     

Study of the formation of a fast electron beam in a coaxial gas diode in the unlimited emission model

The formation of a fast electron beam in a coaxial gas diode is simulated using the OOPIC Pro particle-in-cell code under the assumption of unlimited cathode emissivity. It is shown that fast electrons are generated near the cathode. The so-called “contracting-capacitor” mechanism of electron acceleration does not operate in the parameter range under study, because the boundary of the dense plasma is spread out due to preionization of the electrode gap by fast electrons.     

Nonlinear Right-Hand Polarized Wave in Plasma in the Electron Cyclotron Resonance Region

The propagation of a nonlinear right-hand polarized wave along an external magnetic field in subcritical plasma in the electron cyclotron resonance region is studied using numerical simulations. It is shown that a small-amplitude plasma wave excited in low-density plasma is unstable against modulation instability with a modulation period equal to the wavelength of the excited wave. The modulation amplitude in this case increases with decreasing detuning from the resonance frequency. The simulations have shown that, for large-amplitude waves of the laser frequency range propagating in plasma in a superstrong magnetic field, the maximum amplitude of the excited longitudinal electric field increases with the increasing external magnetic field and can reach 30% of the initial amplitude of the electric field in the laser wave. In this case, the energy of plasma electrons begins to substantially increase already at magnetic fields significantly lower than the resonance value. The laser energy transferred to plasma electrons in a strong external magnetic field is found to increase severalfold compared to that in isotropic plasma. It is shown that this mechanism of laser radiation absorption depends only slightly on the electron temperature.     

Energy of electrons emitted as a result of separation of surfaces

Experiments indicating acceleration of charged particles as a result of separation of solid surfaces are analyzed. As a possible mechanism of such acceleration, generation of surface charge on the separated surfaces of a cleaved ionic crystal is considered. The maximum electric field generated due to the charging of the separated surfaces and the energy of electrons accelerated in such a field are estimated. It is shown that, for the maximum attainable electric field, conditions are created for the generation of runaway electrons that, even at atmospheric pressure, electrons are accelerated to high energies, not experiencing collisions with gas particles.     

Role of secondary electrons and metastable atoms in the electron-beam activation of argon-silane mixtures

The energy and spatial degradation of the primary beam electrons and the production of high-energy secondary electrons in ionizing collisions are analyzed by solving the Boltzmann integral equation for the electron distribution function. The effect of the primary and secondary electrons on the direct ionization of an Ar-SiH₄ mixture, the production of metastable argon atoms, and the dissociation of monosilane molecules is investigated over a wide range of the beam electron energies, argon pressures, and monosilane concentrations. The influence of metastable Ar* atoms on the dissociation of SiH₄ is studied by using the balance equation for metastable argon atoms and the equation for the ambipolar diffusion of ions and low-energy secondary (plasma) electrons in the beam plasma. It is shown that the main contribution to the activation of an Ar-SiH₄ mixture in an electron-beam plasma is provided by secondary electrons with energies higher than the excitation threshold for argon and the dissociation threshold for monosilane, whereas the contribution from metastable argon atoms, though potentially being comparable with that from secondary electrons, is less than in gas-discharge plasmas.     

Spatiotemporal behavior of X-ray emission above 20 keV from a Z-pinch produced by wire-array implosion

Results are presented from experimental studies of hard X-ray (HXR) emission in the photon energy range above 20 keV from dense radiating Z-pinch plasmas. The work is aimed at revealing the nature of fast-electron (electron beam) generation during the implosion of cylindrical and conical wire arrays in the Angara-5-1 facility at currents of up to 3 MA. It is found that the plasma implosion zippering caused by the inclination of wires affects the parameters of the HXR pulse emitted during the implosion of a conical array. It is shown that HXR emission correlates well with the decay of the plasma column near the cathode in the stagnation phase. HXR images of the pinch are produced by the bremsstrahlung of fast electrons generated during plasma column decay and interacting with plasma ions and the anode target. It is found that the use of conical arrays makes it possible to control the direction of plasma implosion zippering and the spatiotemporal and energy parameters of the pinch X-ray emission, in particular the X-ray yield. For wire array with diameters of 12 mm and linear masses of 200–400 μg/cm, the current of the fast electron beam is 20 kA and its energy is 60 J, which is about 1/500 of the energy of the main soft X-ray pulse.     

Probe measurements of the electron distribution function in an electron-beam-produced ytterbium plasma

A nonequilibrium anisotropic plasma produced by an electron beam in the residual air with a low content of ytterbium vapor was investigated by the probe method. It is found that a minor (at a level of a few ppm) admixture of ytterbium to low-pressure air substantially modifies the electron energy distribution function (EEDF): the main peak corresponding to thermal electrons broadens, and new peaks appear. It is shown that the observed change in the EEDF is caused by the low ionization energy of ytterbium, due to which one beam electron can ionize several ytterbium atoms. The new peaks in the EEDF correspond to the final energies of a beam electron after each subsequent ionizing collision with ytterbium atoms.     

Acceleration of electron bunches injected into a wake wave

The process of trapping and acceleration of nonmonoenergetic electron bunches by a wake wave excited by a laser pulse in a plasma channel is investigated. The electrons are injected into the vicinity of the maximum of the wakefield potential with a velocity lower than the wave phase velocity. The study is aimed at utilizing specific features of a wakefield with substantially overlapped focusing and accelerating phases for achieving monoenergetic electron acceleration. Conditions are found under which electrons in a finite-length nonmonoenergetic bunch are accelerated to high energies, while the energy spread between them is minimal. The effect of energy grouping of electrons makes it possible to obtain compact high-energy electron bunches with a small energy spread during laser plasma acceleration.     

Picosecond runaway electron beams in air

Experimental data on the generation of picosecond runaway electron beams in an air gap with an inhomogeneous electric field at a cathode voltage of up to 500 kV are presented. The methods and equipment developed for these experiments made it possible to measure the beam characteristics with a time resolution of better than 10⁻¹¹ s, determine the voltage range and the beam formation time in the breakdown delay stage, and demonstrate the influence of the state of the cathode surface on the stability of runaway electron generation. It is demonstrated that the critical electron runaway field in air agrees with the classical concepts and that the accelerated beam can be compressed to ∼20 ps. It is unlikely that, under these conditions, the beam duration is limited due to the transition of field emission from the cathode to a microexplosion of inhomogeneities. The maximum energy acquired by runaway electrons in the course of acceleration does not exceed the value corresponding to the electrode voltage.     

Investigation of the electron energy distribution function in hollow-cathode glow discharges in nitrogen and oxygen

The mechanism for the formation of the inverse electron distribution function is proposed and realized experimentally in a nitrogen plasma of a hollow-cathode glow discharge. It is shown theoretically and experimentally that, for a broad range of the parameters of an N₂ discharge, it is possible to form a significant dip in the profile of the electron distribution function in the energy range ε=2–4 eV and, accordingly, to produce the inverse distribution with df(ε)/d?>0. The formation of a dip is associated with both the vibrational excitation of N₂ molecules and the characteristic features of a hollow-cathode glow discharge. In such a discharge, the applied voltage drops preferentially across a narrow cathode sheath. In the main discharge region, the electric field E is weak (E<0.1 V/cm at a pressure of about p～0.1 torr) and does not heat the discharge plasma. The gas is ionized and the ionization-produced electrons are heated by a beam of fast electrons (with an energy of about 400 eV) emitted from the cathode. A high-energy electron beam plays an important role in the formation of a dip in the profile of the electron distribution function in the energy range in which the cross section for the vibrational excitation of nitrogen molecules is maximum. A plasma with an inverted electron distribution function can be used to create a population inversion in which more impurity molecules and atoms will exist in electronically excited states.     

Monte Carlo simulation of strand-break induction on plasmid DNA in aqueous solution by monoenergetic electrons

The radiation-induced process of strand breaks on pBR322 plasmid DNA in aqueous solution for different energy electrons was studied by Monte Carlo simulation. Assumptions of induction mechanisms of single- and double-strand breaks (SSBs and DSBs) used in the simulation are that SSB is induced by OH or H reaction with DNA and that DSB is induced by two SSBs on the opposite strands within 10 bp. Dose-response relationships of SSBs and DSBs were demonstrated for monoenergetic electrons of 100 eV, 10 keV, 1 keV and 1 MeV, and the yields of SSB and DSB were calculated. The dose-response relationships of SSBs and DSBs can be fitted by linear and linear-quadratic functions, respectively. The ratio of quadratic to linear components of DSB induction changes due to the electron energy. A high contribution of the linear component is observed for 1 keV electrons in the dose range below 160 Gy. The yields of SSBs and DSBs for all examined electron energies lie well within the experimental data when the probability of strand-break induction by OH and H is assumed to be around 0.1-0.2. The yield of SSBs has a minimum at 1 keV, while the yield of DSBs has a maximum at 1 keV in the examined energies. The strand breaks are formed most densely for 1 keV electrons.     

Dynamics of the ion energy spectrum in EUV-induced hydrogen plasma

The dynamics of the ion energy spectrum in low-pressure (10–100 Pa) hydrogen plasma induced by extreme ultraviolet (EUV) pulses in the wavelength range of 10–20 nm was studied experimentally. The plasma was generated under cathode irradiation due to both direct gas ionization by EUV photons and impact ionization by high-energy secondary electrons. The dynamics of the spectra of ions incident on the cathode was measured using a time-resolved retarding field energy analyzer. It is shown that the ion spectrum dynamics is completely determined by the time evolution of the cathode sheath. At low gas pressures (<20 Pa), the ion spectrum at early moments after the EUV pulse has a peaked shape, typical of a collisionless plasma sheath, and is mainly determined by the cathode voltage. As the pressure increases, the peak broadens and low energy ions appear in the spectrum due to ion collisions in the cathode sheath. An increase in the role of collisions with decreasing plasma density is also observed in the time evolution of ion spectra.     

Beam-plasma interaction in a hybrid plasma waveguide in the pulsed mode of microwave generation

Results are presented from experimental studies of the energy spectra of an electron beam in a model beam-plasma oscillator based on a hybrid plasma waveguide in the pulsed mode of microwave generation with a pulse duration of 1 µs or shorter. The beam energy spent on sustaining the beam-plasma discharge in a slow-wave structure is measured. A correlation between the type of excited waves and the generation of a group of accelerated beam electrons with energies exceeding the injection energy is revealed. It is shown that the pulsed mode of microwave generation is related to the time variations in the plasma density profile in the waveguide and the trapping of beam electrons by the excited microwave field.     

Radio-frequency discharge in a molecular gas flow at a frequency of 1.76 MHz

Results are presented from experiments on the initiation of a homogeneous stable capacitive RF discharge at a frequency of 1.76 MHz in a high-speed molecular gas flow between metal electrodes at a pressure of 5 Torr or dielectric-coated electrodes at a pressure of up to 50 Torr. A mechanism of the current closure in the electrode sheaths related to the primary photoelectric current generated alternately from different electrodes is proposed. The average electron energy increases via second-kind (superelastic) collisions, and fast electrons with energies corresponding to the amplitude value of the RF voltage appear in the electron energy spectrum. As a result, primary emission arises due to the excitation of emitting states from metastable molecular levels. The primary photoelectric current initiates electron avalanches in the electrode sheaths due to secondary photoelectron emission. According to calculations, the current?voltage characteristic of the sheath in this type of discharge is ascending and the field strengths in the electrode sheath and positive column are lower than those in a self-sustained dc discharge. The calculated results are compared with the experimental data.     

Nonequilibrium electron distribution functions in a semiconductor plasma irradiated with fast ions

A kinetic equation for the electrons scattered by acoustic phonons in a solid is derived, and relationships between power-law asymptotic solutions and the particle and energy fluxes in phase space are established. The dependence of the nonextensivity parameter on the intensity of the particle flow in phase space is determined for a nonequilibrium solid-state plasma with sources and sinks. The formation of a steady-state nonequilibrium electron distribution function in a semiconductor with a source and a sink in phase space is numerically simulated using the Landau and Fokker-Planck collision integrals. The nonequilibrium electron distributions formed in the solid-state plasmas of semiconductors and of a Sb/Cs cathode are studied experimentally. It is shown that, within the electron energy range of 5–100 eV, the electron distribution functions decrease with energy according to a power law.     

产电微生物及微生物燃料电池最新研究进展

新型产电微生物(Electricigens)的发现,使得微生物燃料电池概念的内涵发生了根本性的变化,展现了广阔的应用前景。这种微生物能够以电极作为唯一电子受体,把氧化有机物获得的电子通过电子传递链传递到电极产生电流,同时微生物从中获得能量而生长。这种代谢被认为是一种新型微生物呼吸方式。以这种新型微生物呼吸方式为基础的微生物燃料电池可以同时进行废水处理和生物发电,有望可以把废水处理发展成一个有利可图的产业,是MFC最有发展前景的方向。     

利用电化学活跃微生物协助电解发酵产氢

摘要：电解协助发酵产氢是在外源电解协助下,利用电化学活跃微生物在石墨阳极上生长达到彻底氧化因发酵产氢残存的有机酸,产生CO2、电子与质子,电子进入石墨阳极经导线传到铂阴极,而质子则穿过阳离子膜进入阴极池,在无氧环境下,通过外加电压和铂的催化下,电子与质子结合为氢。此过程电子回收率可达90%以上,产氢效率可达8-9mol H2/mol Glucose。这一战略从根本上克服发酵产氢的发酵障碍和代谢产物的反馈抑制,极大地提高了氢转化率,极有可能率先应用于能源作物原料的氢能转化、以及有机污水和有机废弃物处理。     

Effective cross sections for production of single-strand breaks in plasmid DNA by 0.1 to 4.7 eV electrons

We determined effective cross sections for production of single-strand breaks (SSBs) in plasmid DNA [pGEM 3Zf(-)] by electrons of 10 eV and energies between 0.1 and 4.7 eV. After purification and lyophilization on a chemically clean tantalum foil, dry plasmid DNA samples were transferred into a high-vacuum chamber and bombarded by a monoenergetic electron beam. The amount of the circular relaxed DNA in the samples was separated from undamaged molecules and quantified using agarose gel electrophoresis. The effective cross sections were derived from the slope of the yield as a function of exposure and had values in the range of 10(-15)- 10(-14) cm2, giving an effective cross section of the order of 10(-18) cm2 per nucleotide. Their strong variation with incident electron energy and the resonant enhancement at 1 eV suggest that considerable damage is inflicted by very low-energy electrons to DNA, and it indicates the important role of pi* shape resonances in the bond-breaking process. Furthermore, the fact that the energy threshold for SSB production is practically zero implies that the sensitivity of DNA to electron impact is universal and is not limited to any particular energy range.     

Electron and nuclear dynamics in many-electron atoms, molecules and chlorophyll-protein complexes: a review

It has been shown [V.A. Shuvalov, Quantum dynamics of electrons in many-electron atoms of biologically important compounds, Biochemistry (Mosc.) 68 (2003) 1333-1354; V.A. Shuvalov, Quantum dynamics of electrons in atoms of biologically important molecules, Uspekhi biologicheskoi khimii, (Pushchino) 44 (2004) 79-108] that the orbit angular momentum L of each electron in many-electron atoms is L=mVr=nPlanck's and similar to L for one-electron atom suggested by N. Bohr. It has been found that for an atom with N electrons the total electron energy equation E=-(Z(eff))(2)e(4)m/(2n(2)Planck's(2)N) is more appropriate for energy calculation than standard quantum mechanical expressions. It means that the value of L of each electron is independent of the presence of other electrons in an atom and correlates well to the properties of virtual photons emitted by the nucleus and creating a trap for electrons. The energies for elements of the 1st up to the 5th rows and their ions (total amount 240) of Mendeleev' Periodical table were calculated consistent with the experimental data (deviations in average were 5 x 10(-3)). The obtained equations can be used for electron dynamics calculations in molecules. For H(2) and H(2)(+) the interference of electron-photon orbits between the atoms determines the distances between the nuclei which are in agreement with the experimental values. The formation of resonance electron-photon orbit in molecules with the conjugated bonds, including chlorophyll-like molecules, appears to form a resonance trap for an electron with E values close to experimental data. Two mechanisms were suggested for non-barrier primary charge separation in reaction centers (RCs) of photosynthetic bacteria and green plants by using the idea of electron-photon orbit interference between the two molecules. Both mechanisms are connected to formation of the exciplexes of chlorophyll-like molecules. The first one includes some nuclear motion before exciplex formation, the second one is related to the optical transition to a charge transfer state.