Large Plasmonic Resonance Shifts from Metal Loss in Slits

Plasmonics - The impact of loss on the plasmonic resonances in metal–insulator–metal slits is analyzed, particularly the significant effect of loss on the reflection phase. The...     

Super-Resolution Long-Depth Focusing by Radially Polarized Light Irradiation Through Plasmonic Lens in Optical Meso-field

In this paper, we propose a novel plasmonic lens design consisting of an annular slit and concentric grooves. The simulation results show that under radially polarized illumination, a super-resolution long depth of focus (DOF) spot can be achieved in optical meso-field due to the constructive interference of scattered light by the concentric grooves. We also analyze the influence of depth-tuned annular grooves on focusing performance, including focal length, DOF, and full-width half-maximum. Moreover, focusing efficiency can be enhanced (～350 %) by introducing a circular metallic grating which surrounds the annular slit. This plasmonic lens has potential applications in nano-imaging and nano-photolithography.     

Far-Field Focusing of Spiral Plasmonic Lens

In this paper, we study the nanoscale-focusing effect in the far field for a spiral plasmonic lens with a concentric annular groove by using finite-difference time domain simulation. The simulation result demonstrates that a left-hand spiral plasmonic lens can concentrate an incident right-hand circular polarization light into a focal spot at the exit surface. And this spot can be focused into far field due to constructive interference of the scattered light by the annular groove. The focal length and the focal depth can be adjusted by changing the groove radius and number of grooves within a certain range. These properties make it possible to probe the signal of spiral plasmonic lens in far field by using conventional optical devices.     

Effect of the Number of Zones in a One-Dimensional Plasmonic Zone Plate Lens: Simulation and Experiment

A 1D plasmonic zone plate lens (PZPL) consisting of nano-slits within a metal film introduces a phase delay distribution across the planar device surface by a modulation of the slit widths and positions to achieve light focusing. Using the finite-difference time-domain method, the number of zones is found to be a crucial factor for a well-controlled focal length, i.e. at least three zones are necessary for a PZPL exhibiting a focal length in agreement with the design. This conclusion is confirmed by confocal scanning optical microscopy on PZPLs patterned in an aluminium film. In addition, subwavelength light focusing is demonstrated both theoretically and experimentally in a PZPL. A larger PZPL, i.e. more zones, shows a higher resolution. A full full-width half-maximum of 0.37λ in the focal plane is shown theoretically in a PZPL with seven zones. A comparison between the PZPL and the plasmonic Fresnel zone plate shows that PZPLs have a higher contrast at the focus.     

Magnetically Controlled Nanofocusing of a Graphene Plasmonic Lens

In this paper, we propose a method to tailor the nanofocusing of plasmons on graphene plasmonic lens, which is composed of graphene and circular dielectric gratings of magneto-optical material beneath it. With an external magnetic field parallel to graphene surface, the magneto-optical effect of substrate leads to the difference in modal indices of graphene plasmons, which also introduces an additional relative phase difference between these two plasmons during excitation and propagation. Together, these two effects enable us to tailor the position of focal points through external magnetic field, which has been described by an analytical approach based on phase matching and verified by numerical simulations. With an operation wavelength of 8500 nm and an external magnetic field from B = ?1 T to B = 1 T, a shift distance over one and a half times of plasmons wavelength for focal points or donut-shaped field profiles can be obtained under linearly or circularly polarized light. The proposed scheme has potentials in diverse applications, such as the tunable nanofocusing and particle manipulation.     

Complex Polarization Response in Plasmonic Nanospirals

Archimedean nanospirals exhibit many far-field resonances that result from the lack of symmetry and strong intra-spiral plasmonic interactions. Here, we present a computational study, with corroborating experimental results, on the plasmonic response of the 4π Archimedean spiral as a function of incident polarization, for spirals in which the largest linear dimension is less than 550 nm. We discuss the modulation of the near-field structure for linearly and circularly polarized light in typical nanospiral configurations. Computational studies of the near-field distributions excited by circularly polarized light illustrate the effects of chirality on plasmonic mechanisms, while rotation of linearly polarized light provides a detailed view of the effects of broken symmetry on nanospiral fields in any given direction in the plane of the spiral. The rotational geometry exhibits a preference for circular polarization that increases near-field enhancement compared to excitation with linearly polarized light and exchanges near-field configurations and resonant modes. By analyzing the effects of polarization and wavelength on the near-field configurations, we also show how the nanospiral could be deployed in applications such as tunable near-field enhancement of nonlinear optical signals from chiral molecules.     

Analytical Modeling Based on Modified Effective Medium Theories for Optical Properties of Photovoltaic Material-Incorporated Plasmonic Nanoparticles

Theoretical guidance on the optical properties of plasmonic nanoparticles (NPs) is of significant importance in tremendous numbers of fields like photovoltaics. The incorporation of plasmonic NPs into photovoltaic material can promote optical absorption either via the excitation of localized surface plasmon resonance (LSPR) modes or due to multiple light scattering. Since most fabrication techniques for the incorporation of NPs into photovoltaic material result in a random array of NPs with various sizes, numerical simulations based on solving the Maxwell equations are computationally expensive and prohibitively slow for this large number of NPs. Therefore, in this paper, based on modified effective medium theories, taking into account finite size of NPs, size dispersion for NPs, extrinsic dynamic effect, and intrinsic confinement effect, fast and cost-effective analytical modeling, considering both LSPR and scattering effects, is presented to obtain the optical properties of photovoltaic material incorporated by spherical NPs with nonuniform size and random distribution. Then, by means of presented analytical modeling, considering reasonably low and high volume fractions of NPs in addition to small and large size of NPs, the effect of different parameters of embedded NPs into organic and inorganic photovoltaic materials is explored.

     

Optical Properties of Periodic Metallic Slits with Asymmetric Binary Grooves

Plasmonics - The structure of periodic metallic slits with asymmetric binary grooves is proposed to reduce the width of the transmission peak due to the similar Fabry-Perot (F-P) resonances. It is...     

Investigation of Physical Limits of Plasmonic Focusing Lens in Different Regions

We present theoretical studies of three regions for plasmonic focusing, which are surface plasmon-dominating, Fresnel, and Fraunhoffer regions. The boundaries of the three regions are defined and the physical behaviors of plasmonic lenses in terms of focal length and focus size in these regions are investigated. A plasmonic lens that renders a subdiffraction-limit focus in the Fresnel region is presented and the lens performance with respect to the design parameters is studied by using finite-difference time-domain simulations. This work can serve as a basis for understanding plasmonic-focusing phenomenon and designing plasmonic lenses for various applications.     

Plasmonic Optical Trapping in Biologically Relevant Media

We present plasmonic optical trapping of micron-sized particles in biologically relevant buffer media with varying ionic strength. The media consist of 3 cell-growth solutions and 2 buffers and are specifically chosen due to their widespread use and applicability to breast-cancer and angiogenesis studies. High-precision rheological measurements on the buffer media reveal that, in all cases excluding the 8.0 pH Stain medium, the fluids exhibit Newtonian behavior, thereby enabling straightforward measurements of optical trap stiffness from power-spectral particle displacement data. Using stiffness as a trapping performance metric, we find that for all media under consideration the plasmonic nanotweezers generate optical forces 3–4x a conventional optical trap. Further, plasmonic trap stiffness values are comparable to those of an identical water-only system, indicating that the performance of a plasmonic nanotweezer is not degraded by the biological media. These results pave the way for future biological applications utilizing plasmonic optical traps.     

Plasmonic Optical Properties and Applications of Metal Nanostructures

In this review article, we provide an overview of recent research activities in the study of plasmonic optical properties of metal nanostructures with emphasis on understanding the relation between surface plasmon absorption and structure. Both experimental results and theoretical calculations have indicated that the plasmonic absorption strongly depends on the detailed structure of the nanomaterials. Examples discussed include spherical nanoparticles, nanorods, nanowires, hollow nanospheres, aggregates, and nanocages. Plasmon–phonon coupling measured from dynamic studies as a function of particle size, shape, and aggregation state is also reviewed. The fascinating optical properties of metal nanostructures find important applications in a number of technological areas including surface plasmon resonance, surface-enhanced Raman scattering, and photothermal imaging and therapy. Their novel optical properties and emerging applications are illustrated using specific examples from recent literature. The case of hollow nanosphere structures is highlighted to illustrate their unique features and advantages for some of these applications.     

An Annular Plasmonic Lens Under Illumination of Circularly Polarized Light

In this paper, we consider a circular central aperture surrounded with annular depth-tuned grooves and investigate the beaming effect of the structure under illumination of a circularly polarized (CP) plane wave. As a CP plane wave is equivalent to the superposition of two linearly polarized plane waves (TM and TE) with a phase difference of π/2, the superposition of the electric field intensity, ( | E_x |² + | E_y |² ) \left( {{{\left| {E_x} \right|}^2} + {{\left| {E_y} \right|}^2}} \right) , is observed in the transmission field. In addition, two plasmonic modes are found at the resonant wavelengths λ ₁ and λ ₂ with each consisting of multiple wavelengths. At the wavelength λ ₁ = 420 nm, the significant near-field collimation is formed along the direction z, having a long propagation distance up to 1.75 μm (≈4λ) away from the exit plane of the new plasmonic lens.     

Numerical Study of a Nonplanar Two-Stage Surface Plasmonic Lens Illuminated by a Radially Polarized Beam

We design and fabricate a nonplanar two-stage surface plasmonic lens composed of concentric circular slits for exciting propagating surface plasmonic wave and a center-positioned cone-like nanoparticle for generating localized surface plasmonic waves. The numerical investigation based on the finite difference in time domain method is performed. It is found that, when a radially polarized beam illumination is applied, a highly confined electric field with full width half maximum of as small as 6 nm and the transmission enhancement factor of six orders higher than the incident beam is achievable. The optimization design is conducted through comparison of different conic angles and different materials of the cone-like nanoparticles.     

Suppressed Optical Transmission Through an Array of Ultrathin Interlayer Metal Slits

In contrast to the enhanced peak transmission in a subwavelength metal hole array structure (Ebbesen et al., Nature 391:667–669, 1998), here we theoretically investigate the spectral transmission through an array of identical metal slits with ultrathin interlayers and surprisingly find the depressed optical transmission for both infinite and finite array case. Notably, in the latter system, the narrowband dip transmission is evidently produced with the accompaniment of selective field enhancement and phase jumping across the structure. Analyses suggest that this phenomenon is intrinsically related to the penetrant coupling of intracavity surface plasmon polaritons together with the slit termination effect.     

Multiple-Wavelength Focusing and Demultiplexing Plasmonic Lens Based on Asymmetric Nanoslit Arrays

A multiple-wavelength focusing and demultiplexing plasmonic lens based on asymmetric nanoslit arrays is designed. The nanoslit arrays are perforated in a gold film and act as metal–insulator–metal plasmonic waveguides. By manipulating the widths of the slit arrays, the plasmonic lens can concentrate two incident plane wave beams to two separated focal points corresponding to their wavelengths. The full wave simulation is performed to verify the designed lens. This work provides a way to design more compact and integrated wavelength-division multiplexing plasmonic devices for nanophotonic communication and spectral imaging.     

High-Resolution Plasmonic Filter and Refractive Index Sensor Based on Perturbed Square Cavity with Slits and Orthogonal Feeding Scheme

Plasmonics - We present a plasmonic bandpass filter and refractive index sensor based on perturbed square cavity resonator with slits, which is fed by orthogonally oriented feeding waveguides. The...     

Asymmetric Propagation of Optical Signals in Graded Plasmonic Chains

The propagation of optical signals has been studied theoretically and computationally in fully retarded graded plasmonic chains. Asymmetric optical response due to retardation has been observed in various plasmonic chains with gradients in host permittivities, particle sizes, and/or interparticle distances. The range of wavelength-dependent optical response is broadened by the graded effects of host permittivity. Asymmetric propagation ratio is found in the presence of any kind of gradients, and the physical mechanism is analyzed through the gradon modes. These results have potential applications in designing nanostructured plasmonic devices.     

Study of Stress Effect on Optical Performance of Surface-Corrugated Hybrid Plasmonic IBG Filter

Plasmonics - In this paper, design and performance estimation of a hybrid plasmonic-based optical filter operating at 1550 nm in the presence of stress is presented. The proposed integrated Bragg...     

Broadband Optical Response in Ternary Tree Fractal Plasmonic Nanoantenna

The ability to precisely tailor lineshapes, operational bandwidth, and localized electromagnetic field enhancements (“hot spots”) in nanostructures is currently of interest in advancing the performance of plasmonics-based chemical and biological sensing techniques. Fractal geometries are an intriguing alternative in the design of plasmonic nanostructures as they offer tunable multiband response spanning the visible and infrared spectral regions. A numerical study of the optical behavior of ternary tree fractal plasmonic nanoantenna is presented. Self-similar features are seen to emerge in the extinction spectra with the increase in fractal order N of the tree structure. Plasmon oscillations occurring at different length scales are shown to correspond to the multiple peaks and are compared with the spatial maps of electric field enhancement at the surface of the nanoantenna. The multiple peaks are shown to be independently tunable by structural variation. The robustness of the spectral response and polarization dependence arising due to various asymmetries is discussed.     

Optimized Electroless Silver Coating for Optical and Plasmonic Applications

Electroless metal deposition is a simple and convenient technique to fabricate metallic films and to provide isotropic metal functionalization of 3D structures with complex geometries. In this work, we describe the synthesis of silver coatings by means of a modified Tollens reaction and their use as optical coating. The chemical composition of the metallization bath is here addressed to optimize the metal coating deposition. The synthesis parameters have been tailored in order to deposit very smooth films which were characterized by scanning electron microscopy, atomic force microscopy, and optical spectroscopy. 2D diffraction gratings and sinusoidal plasmonic gratings were produced with the proposed method. Optical characterization confirmed the plasmonic activities of the resultant structures, proving the efficiency of the described method for optical applications. Thermal annealing was found to improve the surface roughness of the coating and therefore the optical properties of the plasmonic gratings.