Purpose
One of the main trends in life cycle assessment (LCA) today is towards increased regionalization in inventories and impact assessment methods. LCA studies require the collection of activity data but also of increasingly region-specific background data to accurately depict supply chain processes and enable the application of an increasing number of geographically explicit impact assessment models. This is particularly important for agri-food products. In this review, we assess progress in Portugal towards this goal and provide recommendations for future developments.Methods
We perform a comprehensive review of available LCA studies conducted for Portuguese agri-food products, in order to evaluate the current state of Portuguese agri-food LCA. Among other issues, we assess availability of data, methods used, level of regionalization, impact assessment model relevance and coherence for inter-product comparability. We also provide conclusions and recommendations based on recent developments in the field.Results and discussion
We found 22 LCA studies, covering 22 different products. The analysis of these studies reveals limitations in inter-study comparability. The main challenges have to do with a lack of country-specific foreground data sources applied consistently in the studies found, with discrepancies in impact assessment categories, and with the use of simple functional units that may misrepresent the product analyzed.Conclusions
We conclude that Portuguese agri-food LCA studies do not have a systematic and country-scale approach in order to guarantee regional accuracy and comparability. We propose a research strategy to engage the Portuguese agri-food LCA community in devising a consistent framework before practical application studies are conducted.Purpose
Applied life cycle assessment (LCA) studies often lead to a comparison of rather few alternatives; we call this the “ad hoc LCA approach.” This can seem surprising since applied LCAs normally cover countless options for variations and derived potentials for improvements in a product life cycle. In this paper, we will suggest an alternative approach to the ad hoc approach, which more systematically addresses the many possible variations to identify the most promising. We call it the “structural LCA approach.” The goals of this paper are (1) to provide basic guidelines for the structural approach, including an easy expansion of the LCA space; (2) to show that the structural LCA approach can be used for different types of optimization in LCA; and (3) to improve the transparency of the LCA work.Methods
The structural approach is based on the methodology “design of experiments” (Montgomery 2005). Through a biodiesel well-to-wheel study, we demonstrate a generic approach of applying explanatory variables and corresponding impact categories within the LCA methodology. Explanatory variables are product system variables that can influence the environmental impacts from the system. Furthermore, using the structural approach enables two different possibilities for optimization: (1) single-objective optimization (SO) based on response surface methodology (Montgomery 2005) and (2) multiobjective optimization (MO) by the hypervolume estimation taboo search (HETS) method. HETS enables MO for more than two or three objectives.Results and discussion
Using SO, the explanatory variable “use of residual straw from fields” is, by far, the explanatory variable that can contribute with the highest decrease of climate change potential. For the respiratory inorganics impact category, the most influencing explanatory variable is found to be the use of different alcohol types (bioethanol or petrochemical methanol) in biodiesel production. Using MO, we found the Pareto front based on 5 different life cycle pathways which are nondominated solutions out of 66 different analyzed solutions. Given that there is a fixed amount of resources available for the LCA practitioner, it becomes a prioritizing problem whether to apply the structural LCA approach or not. If the decision maker only has power to change a single explanatory variable, it might not be beneficial to apply the structural LCA approach. However, if the decision maker (such as decision makers at the societal level) has power to change more explanatory variables, then the structural LCA approach seems beneficial for quantifying and comparing the potentials for environmental improvement between the different explanatory variables in an LCA system and identifying the overall most promising product system configurations among the chosen PWs.Conclusions
The implementation of the structural LCA approach and the derived use of SO and MO have been successfully achieved and demonstrated in the present paper. In addition, it is demonstrated that the structural LCA approach can lead to more transparent LCAs since the potentially most important explanatory variables which are used to model the LCAs are explicitly presented through the structural LCA approach. The suggested structural approach is a new approach to LCA and it seems to be a promising approach for searching or screening product systems for environmental optimization potentials. In the presented case, the design has been a rather simple full factorial design. More complicated problems or designs, such as fractional designs, nested designs, split plot designs, and/or unbalanced data, in the context of LCA could be investigated further using the structural approach. 相似文献Purpose
Multifunctionality in life-cycle assessment (LCA) is solved with allocation, for which many different procedures are available. Lack of sufficient guidance and difficulties to identify the correct allocation approach cause a large number of combinations of methods to exist in scientific literature. This paper reviews allocation procedures for recycling situations, with the aim to identify a systematic approach to apply allocation.Methods
Assumptions and definitions for the most important terms related to multifunctionality and recycling in LCA are given. The most relevant allocation procedures are identified from literature. These procedures are expressed in mathematical formulas and schemes and arranged in a systematic framework based on the underlying objectives and assumptions of the procedures.Results and discussion
If the LCA goal asks for an attributional approach, multifunctionality can be solved by applying system expansion—i.e. including the co-functions in the functional unit—or partitioning. The cut-off approach is a form of partitioning, attributing all the impacts to the functional unit. If the LCA goal asks for a consequential approach, substitution is applied, for which three methods are identified: the end-of-life recycling method and the waste mining method, which are combined in the 50/50 method. We propose to merge these methods in a new formula: the market price-based substitution method. The inclusion of economic values and maintaining a strict separation between attributional and consequential LCA are considered to increase realism and consistency of the LCA method.Conclusions and perspectives
We identified the most pertinent allocation procedures—for recycling as well as co-production and energy recovery—and expressed them in mathematical formulas and schemes. Based on the underlying objectives of the allocation procedures, we positioned them in a systematic and consistent framework, relating the procedures to the LCA goal definition and an attributional or consequential approach. We identified a new substitution method that replaces the three existing methods in consequential LCA. Further research should test the validity of the systematic framework and the market price-based substitution method by means of case studies.Background
The editor of this journal has been waiting for such a contribution of the life cycle assessment (LCA) practitioners and users for years, since the last debate of this kind dates back to beginning of the new century. It is remembered as the “Two planets debate” and coincided with the emergence of life cycle management, i.e. the use of life-cycle based methods in industry.The “Two planets”
This is a metaphor coined at the Society of Environmental Toxicology and Chemistry (SETAC) Europe case studies symposium 2000 and designates the fact that many academic LCA developers and the LCA practitioners seem to live in different spheres. The editorial note by Baitz et al. shows that this seems to be true still today. It is argued that the practitioners do not frequently enough participate in the working groups organized by SETAC, the UNEP/SETAC life cycle initiative and other international organizations and therefore cannot bring in the practical experience they have acquired in performing “real-life” LCA studies. The new LCIA methods, for instance, are often not accepted by the LCA practitioners and commissioners, since essential aspects were not recognised during method development.Tentative proposal for a solution
The solution of the problems pointed out in Baitz et al. cannot be to hinder the inhabitants of the academic planet in inventing ingenious new methods for reasons of academic freedom. It is proposed that new methods developed should be tested by practitioners in real-life LCA studies. Data asymmetries in comparative (i.e. most) LCA studies using more demanding methods may shift problems from LCIA to the LCI databases. With regard to the financing of such studies, it should be remembered that practitioners do their living by performing LCAs and other studies and have to calculate a full overhead in addition to the pure working costs. 相似文献Purpose
In LCA, a multi-functionality problem exists whenever the environmental impacts of a multi-functional process have to be allocated between its multiple functions. Methods for fixing this multi-functionality problem are controversially discussed because the methods include ambiguous choices. To study the influence of these choices, the ISO standard requires a sensitivity analysis. This work presents an analytical method for analyzing sensitivities and uncertainties of LCA results with respect to the choices made when a multi-functionality problem is fixed.Methods
The existing matrix algebra for LCA is expanded by explicit equations for methods that fix multi-functionality problems: allocation and avoided burden. For allocation, choices exist between alternative allocation factors. The expanded equations allow calculating LCA results as a function of allocation factors. For avoided burden, choices exist in selecting an avoided burden process from multiple candidates. This choice is represented by so-called aggregation factors. For avoided burden, the expanded equations calculate LCA results as a function of aggregation factors. The expanded equations are used to derive sensitivity coefficients for LCA results with respect to allocation factors and aggregation factors. Based on the sensitivity coefficients, uncertainties due to fixing a multi-functionality problem by allocation or avoided burden are analytically propagated. The method is illustrated using a virtual numerical example.Results and discussion
The presented approach rigorously quantifies sensitivities of LCA results with respect to the choices made when multi-functionality problems are fixed with allocation and avoided burden. The uncertainties due to fixing multi-functionality problems are analytically propagated to uncertainties in LCA results using a first-order approximation. For uncertainties in allocation factors, the first-order approximation is exact if no loops of the allocated functional flows exist. The contribution of uncertainties due to fixing multi-functionality problems can be directly compared to the uncertainty contributions induced by uncertain process data or characterization factors. The presented method allows the computationally efficient study of uncertainties due to fixing multi-functionality problems and could be automated in software tools.Conclusions
This work provides a systematic method for the sensitivity analysis required by the ISO standard in case choices between alternative allocation procedures exist. The resulting analytical approach includes contributions of uncertainties in process data, characterization factors, and—in extension to existing methods—uncertainties due to fixing multi-functionality problems in a unifying rigorous framework. Based on the uncertainty contributions, LCA practitioners can select fields for data refinement to decrease the overall uncertainty in LCA results. 相似文献Purpose
The analysis of uncertainty in life cycle assessment (LCA) studies has been a topic for more than 10 years, and many commercial LCA programs now feature a sampling approach called Monte Carlo analysis. Yet, a full Monte Carlo analysis of a large LCA system, for instance containing the 4,000 unit processes of ecoinvent v2.2, is rarely carried out by LCA practitioners. One reason for this is computation time. An alternative faster than Monte Carlo method is analytical error propagation by means of a Taylor series expansion; however, this approach suffers from being explained in the literature in conflicting ways, hampering implementation in most software packages for LCA. The purpose of this paper is to compare the two different approaches from a theoretical and practical perspective.Methods
In this paper, we compare the analytical and sampling approaches in terms of their theoretical background and their mathematical formulation. Using three case studies—one stylized, one real-sized, and one input–output (IO)-based—we approach these techniques from a practical perspective and compare them in terms of speed and results.Results
Depending on the precise question, a sampling or an analytical approach provides more useful information. Whenever they provide the same indicators, an analytical approach is much faster but less reliable when the uncertainties are large.Conclusions
For a good analysis, analytical and sampling approaches are equally important, and we recommend practitioners to use both whenever available, and we recommend software suppliers to implement both. 相似文献Life cycle assessment (LCA) is a data-intensive methodology; therefore, experts usually focus collection efforts on a few activities, while generic data on remaining activities are taken from databases. Even though increased availability of databases has facilitated LCA takeoff, assuring data quality is fundamental to ensure meaningful results and reliable interpretation.
MethodsEcoinvent has become a global reference for inventory data. Its current version released three impact partition modeling options—the recycled content, “allocation at the point of substitution” (APOS), and consequential models—whose adequate choice is crucial for yielding meaningful assessments. Tutorials and manuals describe the distribution algorithm that backs each system model, to ground decision-making regarding the best fit to a study’s goals. We performed a systematic literature review to investigate—within the papers published on the International Journal of LCA (IJLCA)—how transparently authors addressed the system model choices.
Results and discussionAbout 70% of LCA practitioners continued to use earlier versions of ecoinvent after version 3 was launched in 2013. The number of papers using versions 3.x only showed an increased growth trend 2 years later. Eighty-three papers actually adopted the newest version of the database. From those, only 29 papers clearly mentioned the adopted system model. Our SLR also suggests a trend regarding authorship profile of LCA-related studies: the number of studies conducted by practitioners aware of the intricacies of sound modeling of background and foreground data might have been surpassed by those conducted by non-LCA specialists who use LCA as a supporting tool for investigations in applied fields, and merely scratch the surface.
ConclusionsOur results point to a need for a caveat: ecoinvent users must take time to understand the general concept behind each system model and practice one of the most important actions when performing an LCA—state methodological choices clearly.
相似文献Purpose
The objective of the paper is to discuss the role of a new guidance document for life cycle assessment (LCA) in the construction sector available as an online InfoHub.Methods
This InfoHub derives from the EeBGuide European project that aimed at developing a guidance document for energy-efficient building LCA studies. The InfoHub is built on reference documents such as the ISO 14040-44 standards, the EN 15804 and EN 15978 standards as well as the ILCD Handbook. The guidance document was filled with expertise and knowledge of several experts. The focus was put on providing scientifically sound, yet practical guidance.Results
The EeBGuide InfoHub is an online guidance document, setting rules for conducting LCA studies and giving instructions on how to do this. The document has a section on buildings—new and existing—and a section on construction products. It is structured according to the life cycle stages of the European standards EN 15804 and EN 15978, covering all aspects of LCA studies by applying provisions from these standards and the ILCD handbook, wherever applicable. The guidance is presented for different scopes of studies by means of three study types. For the same system boundaries, default values are proposed in early or quick assessment (screening and simplified LCA) while detailed calculation rules correspond to a complete LCA. Such approach is intended to better match the user needs in the building sector.Conclusions and recommendations
This paper can be viewed as a contribution to the ongoing efforts to improve the consistency and harmonisation in LCA studies for building products and buildings. Further contributions are now needed to improve building LCA guidance and to strengthen links between research, standardisation and implementation of LCA in the construction practice. 相似文献Purpose
Numerous publications in the last years stressed the growing importance of nanotechnology in our society, highlighting both positive as well as in the negative topics. Life cycle assessment (LCA) is amongst the most established and best-developed tool in the area of product-related assessment. In order to use this tool in the area of nanotechnology, clear rules of how emissions of nanomaterials should be taken into account on the level of life cycle inventory (LCI) modelling are required—i.e. what elements and properties need to be reported for an emission of a nanomaterial. The objective of this paper is to describe such a framework for an adequate and comprehensive integration of releases of nanomaterials.Methods
With a three-step method, additional properties are identified that are necessary for an adequate integration of releases of nanomaterials into LCA studies.Result and discussion
In the first step, a comprehensive characterisation of the release of a nanomaterial is compiled—based on reviewing scientific publications, results from expert workshops and publications from public authorities and international organisations. In the second step, this comprehensive overview is refined to a list containing only those properties that are effectively relevant for LCA studies—i.e. properties that influence the impacts in the areas of human toxicity and ecotoxicity, respectively. For this, an academic approach is combined with a second, more practical, view point, resulting together in a prioritisation of this list of properties. Finally, in a third step, these findings are translated into the LCA language—by showing how such additional properties could be integrated into the current LCA data formats for a broader use by the LCA community.Conclusions
As a compromise between scholarly knowledge and the (toxicological) reality, this paper presents a clear proposal of an LCI modelling framework for the integration of releases of nanomaterials in LCA studies. However, only the broad testing of this framework in various situations will show if the suggested simplifications and reductions keep the characterisation of releases of nanomaterials specific enough and/or if assessment is accurate enough. Therefore, a next step has to come from the impact assessment, by the development of characterisation factors as a function of size and shape of such releases. 相似文献Despite the wide use of LCA for environmental profiling, the approach for determining the system boundary within LCA models continues to be subjective and lacking in mathematical rigor. As a result, life cycle models are often developed in an ad hoc manner, and are difficult to compare. Significant environmental impacts may be inadvertently left out. Overcoming this shortcoming can help elicit greater confidence in life cycle models and their use for decision making.
MethodsThis paper describes a framework for hybrid life cycle model generation by selecting activities based on their importance, parametric uncertainty, and contribution to network complexity. The importance of activities is determined by structural path analysis—which then guides the construction of life cycle models based on uncertainty and complexity indicators. Information about uncertainty is from the available life cycle inventory; complexity is quantified by cost or granularity. The life cycle model is developed in a hierarchical manner by adding the most important activities until error requirements are satisfied or network complexity exceeds user-specified constraints.
Results and DiscussionThe framework is applied to an illustrative example for building a hybrid LCA model. Since this is a constructed example, the results can be compared with the actual impact, to validate the approach. This application demonstrates how the algorithm sequentially develops a life cycle model of acceptable uncertainty and network complexity. Challenges in applying this framework to practical problems are discussed.
ConclusionThe presented algorithm designs system boundaries between scales of hybrid LCA models, includes or omits activities from the system based on path analysis of environmental impact contribution at upstream network nodes, and provides model quality indicators that permit comparison between different LCA models.
相似文献