Formation of nanostructures in a plasma focus discharge

A new method for creating nanostructures in a plasma focus discharge is proposed. It is shown that the material of a micron-size dust target produced at the discharge axis efficiently evaporates and is then involved in the pinching process. After the pinch decays, the plasma expands with the thermal velocity and the evaporated dust material is deposited on the collectors in the form of fractal particles or nanoclusters organized into various structures. Such structures have a well-developed surface, which is important for various technological applications.     

Current halo structures in high-current plasma experiments: θ-pinch

Experimental data elucidating mechanisms for halo formation in θ-pinch discharges are presented and discussed. The experiments were performed with different gases (H₂, D₂, He, and Ar) in a theta-pinch device with a porcelain vacuum chamber and an excitation coil 15 cm in diameter and 30 cm in length. The stored energy, the current in the excitation coil, and the current half-period were W = 10 kJ, I = 400 kA, and T/2 = 14 μs, respectively. It is found that the plasma rings (halos) surrounding the pinch core arise as a result of coaxial pinch stratification due to both the excitation of closed currents (inductons) inside the pinch and the radial convergence of the plasma current sheaths produced after the explosion of T-layers formed near the wall in the initial stage of the discharge. It is concluded that halo structures observed in pinches, tokamaks, and other high-current devices used in controlled fusion research have the same nature.     

Study of the azimuthal magnetic fields and scaling laws at the KPF-4-Phoenix facility

Results are presented from magnetic probe measurements in the pinching region formed during the compression of the plasma current sheath (PCS) in a discharge in deuterium at the KPF-4-Phoenix plasma focus facility. The fine structure (shock front-magnetic piston) of the PCS and its time evolution in the course of plasma compression toward the facility axis was studied by means of magnetic probes. It is shown that the fraction of the current transported into the axial region by the PCS does not exceed 65% of the total discharge current. The integral neutron yield Y _n is well described by the formula Y _n ≈ (1.5–3) × 10¹⁰ I _p ⁴ , where I _p (in MA) is the pinch current flowing in the region r ≤ 22 mm.     

Hydrodynamic model of a dielectric-barrier discharge in pure chlorine

A one-dimensional hydrodynamic model of a dielectric-barrier discharge (DBD) in pure chlorine is developed, and the properties of the discharge are modeled. The discharge is excited in an 8-mm-long discharge gap between 2-mm-thick dielectric quartz layers covering metal electrodes. The DBD spatiotemporal characteristics at gas pressures of 15–100 Torr are modeled for the case in which a 100-kHz harmonic voltage with an amplitude of 8 kV is applied to the electrodes. The average power density deposited in the discharge over one voltage period is 2.5–5.8 W/cm³. It is shown that ions and electrons absorb about 95 and 5% of the discharge power, respectively. In this case, from 67 to 97% of the power absorbed by electrons is spent on the dissociation and ionization of Cl₂ molecules. Two phases can be distinguished in the discharge dynamics: the active (multispike) phase, which follows the breakdown of the discharge gap, and the passive phase. The active phase is characterized by the presence of multiple current spikes, a relatively high current, small surface charge density on the dielectrics, and large voltage drop across the discharge gap. The passive phase (with no current spikes) is characterized by a low current, large surface charge density on the dielectrics, and small voltage drop across the discharge gap. The peak current density in the spikes at all pressures is about 4 mA/cm². In the multispike phase, there are distinct space charge sheaths with thicknesses of 1.5–1.8 mm and a mean electron energy of 4.3–7 eV and the central region of quasineutral plasma with a weak electric field and a mean electron energy of 0.8–3 eV. The degree of ionization of chlorine molecules in the discharge is ~0.02% at a pressure of 15 Torr and ~0.01% at 100 Torr. The DBD plasma is electronegative due to the fast attachment of electrons to chlorine atoms: e + Cl₂ → Cl + Cl^–. The most abundant charged particles are Cl ₂ ⁺ and Cl^? ions, and the degree of ionization during current spikes in the active phase is (4.1–5.5) × 10^–7. The mechanism of discharge sustainment is analyzed. The appearance of a series of current spikes in the active phase of the discharge is explained.     

Nonlinear dust-acoustic structures in space plasmas with superthermal electrons,positrons, and ions

Some features of nonlinear dust-acoustic (DA) structures are investigated in a space plasma consisting of superthermal electrons, positrons, and positive ions in the presence of negatively charged dust grains with finite-temperature by employing a pseudo-potential technique in a hydrodynamic model. For this purpose, it is assumed that the electrons, positrons, and ions obey a kappa-like (κ) distribution in the background of adiabatic dust population. In the linear analysis, it is found that the dispersion relation yield two positive DA branches, i.e., the slow and fast DA waves. The upper branch (fast DA waves) corresponds to the case in which both (negatively charged) dust particles and (positively charged) ion species oscillate in phase with electrons and positrons. On the other hand, the lower branch (slow DA waves) corresponds to the case in which only dust particles oscillate in phase with electrons and positrons, while ion species are in antiphase with them. On the other hand, the fully nonlinear analysis shows that the existence domain of solitons and their characteristics depend strongly on the dust charge, ion charge, dust temperature, and the spectral index κ. It is found that the minimum/maximum Mach number increases as the spectral index κ increases. Also, it is found that only solitons with negative polarity can propagate and that their amplitudes increase as the parameter κ increases. Furthermore, the domain of Mach number shifts to the lower values, when the value of the dust charge Z _d increases. Moreover, it is found that the Mach number increases with an increase in the dust temperature. Our analysis confirms that, in space plasmas with highly charged dusts, the presence of superthermal particles (electrons, positrons, and ions) may facilitate the formation of DA solitary waves. Particularly, in two cases of hydrogen ions H⁺ (Z _i = 1) and doubly ionized Helium atoms He²⁺ (Z _i = 2), the mentioned results are the same. Additionally, the mentioned dusty plasma does not support DA solitons with positive polarity (compressive solitons). Furthermore, our analysis confirms that DA double layers cannot exist in such a system. Moreover, the positron density has not a considerable effect on the behavior of DA solitons in our model.     

Controlling plasma composition during carbon film deposition in microwave discharges by means of optical-emission spectroscopy

Optical emission spectra from the microwave discharge plasma that is used to activate gas-phase deposition of carbon films are systematically investigated under various deposition conditions. The line emission intensities from CH and C₂ radicals, which are responsible for the growth of the diamond and graphite phases, respectively, are studied as functions of the main macroparameters of the process. To find the relation between the features of the emission spectra and the composition of the films obtained, the films were examined using Raman spectroscopy and electron microscopy. It is shown that monitoring the relative intensities of the spectral lines can be used to obtain the desired type of film, in which case the state of the substrate surface and the presence of a catalyst on it also play an important role. Experiments on the deposition of carbon films in the pulsed regime of plasma excitation show the possibility of changing the phase composition of the film by varying both the pulse repetition rate and the off-duty factor. At the same average microwave power, the rate of film deposition in the pulsed regime of plasma excitation is lower than that in a continuous discharge; however, the growth rate of the graphite phase decreases insignificantly.     

Determination of the electron density and electric field in the plasma of a low-pressure microwave electrode discharge in hydrogen from the measured spectral line intensities

The parameters of the plasma of a microwave electrode discharge in hydrogen at pressures of 1–8 torr and incident powers of 20–80 W are measured by the so-called “relative intensity” method. The method allows one to determine the electron density and electric field in plasma by measuring the relative intensities of the H_α, H_β, and 763.5-nm Ar line emission and calculating the electron-impact rate constants from the homogeneous Boltzmann equation. The measurements show that there are regions in the discharge where the electron density is higher (a bright electrode sheath) and lower (a spherical region) than the critical density for the frequency 2.45 GHz (n_cr～7×10¹⁰ cm^?3). Inside the spherical region, the electric field varies slightly over the radius and the electron density increases as the discharge boundary is approached. The observed discharge structure can be attributed to the presence of a self-sustained discharge zone (electrode sheath); a non-self-sustained discharge zone (spherical region); and a decaying plasma region, which is separated from the active discharge zone by an electric double layer.     

Sterilization of medical productsin low-pressure glow discharges

Results are presented from experimental and theoretical studies of the sterilization of medical products by the plasmas of dc glow discharges in different gas media. The sterilization efficiency is obtained as a function of discharge parameters. The plasma composition in discharges in N₂ and O₂ is investigated under the operating conditions of a plasma sterilizer. It is shown that free surfaces of medical products are sterilized primarily by UV radiation from the discharge plasma, while an important role in sterilization of products with complicated shapes is played by such chemically active particles as oxygen atoms and electronically excited O₂ molecules.     

Experimental studies of the dynamics of dust grains in gas-discharge plasmas

Results of the experimental studies of the dynamics of dust grains in the plasmas of an rf capacitive discharge and a dc glow discharge are presented. The dusty plasma of a dc glow discharge was investigated in both ground-based experiments and experiments carried out under microgravity conditions (on board the Mir space station). The pair correlation function, temperature, and diffusion coefficient of dust grains are measured in a wide range of the dusty-plasma parameters. Dimensionless parameters responsible for the microscopic transport of dust-grains in a gas-discharge plasma are determined. A nonintrusive diagnostic technique for determining the dust-grain charges and screening lengths under the assumption of screened interaction between the grains is proposed. This technique is used to estimate the surface potential of dust grains of different size in a gas-discharge plasma.     

Scaling of a fast spherical discharge

The influence of the discharge cavity dimensions on the properties of the spherical plasma formed in a fast discharge was studied experimentally. The passage of a current pulse with an amplitude of 30–40 kA and a rise rate of ~10¹² A/s (a fast discharge) through a spherical ceramic (Al₂O₃) cavity with an inner diameter of 11 mm filled with argon at a pressure of 80 Pa results in the formation of a 1- to 2-mm-diameter spherical plasma with an electron temperature of several tens of electronvolts and a density of 10¹⁸–10¹⁹ cm^–3. It is shown that an increase in the inner diameter of the discharge cavity from 11 to 21 mm leads to the fourfold increase in the formation time of the spherical plasma and a decrease in the average ion charge. A decrease in the cavity diameter to 7 mm makes the spherical plasma unstable.     

Study of the current-sheath formation during the implosion of multishell gas puffs

Results are presented from experimental studies of the dynamics of large-diameter multishell gas puffs imploded by microsecond megampere current pulses. The experiments were conducted on the GIT-12 generator in the regime of microsecond implosion (t _imp = 1.1–1.2 μs, I ₀ = 3.4–3.7 MA). The influence of the load configuration on the dynamics of current losses and gas-puff radiative characteristics was studied. The correlation between the radial compression ratio (the ratio between the initial and final Z-pinch radii) and the magnitude of the current flowing at the plasma periphery was investigated. The experiments show that, in a multishell gas puff, large-scale instabilities insignificantly affect the gas-puff implosion even over microsecond time intervals and that a compact dense pinch with a relatively high average electron temperature (400–600 eV) forms at the Z-pinch axis. The diameter of the plasma column radiating in the K-shell lines of neon is about 3–4 mm, the K-shell radiation yield being 5–11 kJ/cm. In the final stage of implosion, only a small portion of the current flows through the high-temperature central region of the pinch plasma, whereas the major part of the generator current flows through the residual peripheral plasma.     

Potential of a dust grain in a nitrogen plasma with a condensed disperse phase at room and cryogenic temperatures

The first numerical study is presented of the self-consistent potential of a dust grain in a nitrogen plasma with a condensed disperse phase at room and cryogenic temperatures and at high gas pressures for which the electron and ion transport in the plasma can be described in the hydrodynamic approximation. It is shown that the potential of the dust grain is described with good accuracy by the Debye potential, in which case, however, the screening radius turns out to be larger than the electron Debye radius. The difference between the radii is especially large in a plasma with high ionization rates (about 10¹⁶–10¹⁸ cm^?3 s^?1) at room temperature. It is found that, in a certain range of the parameters of a nitrogen dusty plasma, the parameter describing the interaction between the grains exceeds the critical value above which one would expect the formation of plasma-dust structures such as Coulomb crystals. For a plasma at cryogenic temperature (T=77 K), this range is significantly wider.     

Study of the fine structure of the plasma current sheath and magnetic fields in the axial region of the PF-1000 facility

Results of measurements of magnetic fields in the plasma pinching region during the compression of the deuterium plasma current sheath (PCS) at the PF-1000 plasma focus facility are presented. The fine structure of the PCS (shock wave-magnetic piston) and its variations in the course of plasma compression toward the facility axis are studied using magnetic probes and laser interferometry. The radial distributions of the plasma density and current in the PCS are compared. It is shown that, in the shock wave region, the electron density of the compressed plasma is on the order of ～10¹⁸ cm^?3, whereas the PCS current is almost entirely concentrated in the magnetic piston region—a plasma layer with an electron density of less than 10¹⁵ cm^?3. Efficient transportation of the current by the PCS into the axial region of the facility in discharges with a high neutron yield (Y _n > 10¹¹ neutrons/shot) is detected. It is shown that the total neutron yield is well described by the dependence Y _n ≈ (1.5–3) × 10¹⁰ I _p ⁴ , where I _p is the pinch current (in MA) flowing within the region r ≤ 13 mm.     

Controlling the characteristics of a repetitive volume discharge in CFC-12 and its mixtures with argon

The parameters of a repetitive volume discharge in CF₂Cl₂ (CFC-12) and its mixtures with argon at pressures of P(CF₂Cl₂)≤0.4 kPa and P(Ar)≤1.2 kPa are studied. The discharge was ignited in an electrode system consisting of a spherical anode and a plane cathode by applying a dc voltage U_ch≤1 kV to the anode. The electrical and optical characteristics of a volume discharge (such as the current-voltage characteristics; the plasma emission spectra; and the waveforms of the discharge voltage, the discharge current, and the total intensity of plasma emission) are investigated. It is found that, by shunting the discharge gap with a pulsed capacitor with a capacitance of C₀≤3.5 nF, it is possible to control the amplitude and duration of the discharge current pulses, as well as the characteristics of the pulsed plasma emission. The increase in the capacitance C₀ from 20 to 3500 pF leads to a significant increase in the amplitude and duration of the discharge current pulses, whereas the pulse repetition rate decreases from 70 to 3 kHz. The glow discharge exists in the form of a domain with a height of up to 3 cm and diameter of 0.5–3.0 cm. The results obtained can be used to design an untriggered repetitive germicidal lamp emitting in the Cl₂(257/200 nm) and ArCl (175 nm) molecular bands and to develop plasmachemical methods for depositing amorphous fluorocarbon and chlorocarbon films.     

Generation of hard X-ray emission by the electron beam in plasma focus facilities

The results of measurements of the temporal characteristics of hard X-ray emission generated at plasma focus (PF) facilities are presented. Mechanisms of electron beam generation in the PF pinch are analyzed. On the basis of the known mechanisms and experimental data on the measured temporal characteristics of hard X-ray pulses, a mechanism of fast electron generation that takes into account both the effect of the anomalous pinch resistance and the current redistribution in the near-pinch region is proposed. The processes occurring in the pinch plasma are simulated on the basis of the proposed mechanism by using the MicroCap code. It is shown that only a small fraction of the discharge current (1–10%) can be transformed into the electron beam current.     

Charging of dust grains in a nonequilibrium plasma of a stratified glow discharge

A theoretical model is presented that describes the charging of dust grains in the positive plasma column of a stratified glow dc discharge in argon. A one-dimensional self-consistent model is used to obtain axial profiles of the electric field, as well as the electron energy distribution function along the axis of the discharge tube. Radial profiles of the electric field are determined in the ambipolar diffusion approximation. It is assumed that, in the radial direction, the electron distribution function depends only on the total electron energy. Two-dimensional distributions of the discharge plasma parameters are calculated and used to determine the potential and charge of a test dust grain at a certain point within the discharge and the electrostatic forces acting on it. It is shown that the grain charge distribution depends strongly on the nonequilibrium electron distribution function and on the nonuniform distribution of the electric field in a stratified glow discharge. A discussion is presented on the suspension of dust grains, the separation of grains by size in the discharge striations, and a possible mechanism for the onset of vortex dust motion at the edge of a dust cloud.     

Effect of the anode material on the X-ray spectrum of micropinch discharge plasma

The effect of the elemental composition of the anode material on the parameters and X-ray spectrum of micropinch discharge plasma have been studied using a low-inductance vacuum spark device. It is shown that the plasma electron temperature T _e and intensity of hard X-ray emission increase with increasing nuclear charge number Z of the anode material of the discharge system.     

Study of the implosion of foam-wire loads at the Angara-5-1 facility

Results are presented from experiments on studying the compactness of compression of imploding nested foam-wire loads at currents of up to 4 MA at the Angara-5-1 facility. The degree of pinch compression was estimated from the dynamics of the spatial distribution of the current (magnetic field) and the shape of the soft X-ray pulse. The load consisted of nested cascades, one of which being a wire array and the other being a hollow or solid low-density cylinder made of agar-agar foam with a wall thickness of 100?C200 ??m. In some experiments, one of the cascades was made of C₂₀H₁₇O₆ solid-state organic acid foam. The radial distribution of the magnetic field inside the nested cascades of the imploding foam-wire load (both between the cascades and inside the inner cascade) was measured using tiny magnetic probes. The measured radial distributions of the magnetic field are compared with the magnetic field configuration calculated using a one-dimensional MHD code simulating the implosion of a nested foam-wire load. It is shown that the spatial structure of the current and magnetic field during the implosion of such a load is determined by the development of supersonic and subsonic magnetized plasma flows in its cascades. The specific features of pinch formation and methods for the compensation of the nonsimultaneous pinch compression between the anode and the cathode (the zipper effect) during the implosion of a nested foam-wire load are analyzed.     

Production of XeI(<Emphasis Type="Italic">B</Emphasis>) and I<Subscript>2</Subscript>(<Emphasis Type="Italic">B</Emphasis>) molecules in the plasma of a steady electric discharge in Xe/I<Subscript>2</Subscript> mixtures

The production of excited xenon iodides and iodine dimers in the plasma of a longitudinal dc glow discharge is investigated. The discharge was ignited in iodine vapor and Xe/I₂ mixtures at xenon pressures of P(Xe)=0.1–1.5 kPa and deposited powers of 10–100 W. The current-voltage characteristics of a glow discharge, the plasma emission spectra in the spectral range of 200–650 nm, and the intensities of spectral lines and molecular bands are studied as functions of the deposited power and the xenon partial pressure in a Xe/I₂ mixture. It is found that the discharge plasma emits within the spectral range of 206–343 nm, which includes the 206-nm resonant line of atomic iodine and the XeI(B-X) 253-nm and I₂(B-X) 343-nm molecular bands. The power deposited in the plasma and the xenon pressure P(Xe) are optimized to achieve the maximum UV emission intensity. The 7-W total UV power emitted from the entire surface of the cylindrical discharge tube is achieved with an efficiency of ≤5%.     

Glow discharge in singlet oxygen

Currently, there is no experimental data on the plasma balance in gas mixtures with a high content of singlet delta oxygen O₂(¹Δ_g). These data can be obtained by studying the parameters of an electric discharge in singlet oxygen produced by a chemical generator. The O₂(¹Δ_g) molecules significantly change the kinetics of electrons and negative ions in plasma. Hence, the discharge conditions at low and high. O₂(¹Δ_g) concentrations are very different. Here, the parameters of the positive column of a glow discharge in a gas flow from a chemical singlet-oxygen generator are studied. It is experimentally shown that, at an O₂(¹Δ_g) concentration of 50% and at pressures of 1.5 and 2 torr, the electric field required to sustain the discharge is considerably lower than in the case when all of the oxygen molecules are in the ground state. A theoretical model of the glow discharge is proposed whose predictions are in good agreement with the experimental data.