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1.

Purpose

In life cycle assessment (LCA), eutrophication is commonly assessed using site-generic characterisation factors, despite being a site-dependent environmental impact. The purpose of this study was to improve the environmental relevance of marine eutrophication impact assessment in LCA, particularly regarding the impact assessment of waterborne nutrient emissions from Swedish agriculture.

Methods

Characterisation factors were derived using site-dependent data on nutrient transport for all agricultural soils in Sweden, divided into 968 catchment areas, and considering the Baltic Sea, the receiving marine compartment, as both nitrogen- and phosphorus-limited. These new characterisation factors were then applied to waterborne nutrient emissions from typical grass ley and spring barley cultivation in all catchments.

Results and discussion

The site-dependent marine eutrophication characterisation factors obtained for nutrient leaching from soils varied between 0.056 and 0.986 kg Neq/kg N and between 0 and 7.23 kg Neq/kg P among sites in Sweden. On applying the new characterisation factors to spring barley and grass ley cultivation at different sites in Sweden, the total marine eutrophication impact from waterborne nutrient emissions for these crops varied by up to two orders of magnitude between sites. This variation shows that site plays an important role in determining the actual impact of an emission, which means that site-dependent impact assessment could provide valuable information to life cycle assessments and increase the relevance of LCA as a tool for assessment of product-related eutrophication impacts.

Conclusions

Characterisation factors for marine eutrophication impact assessment at high spatial resolution, considering both the site-dependent fate of eutrophying compounds and specific nutrient limitations in the recipient waterbody, were developed for waterborne nutrient emissions from agriculture in Sweden. Application of the characterisation factors revealed variations in calculated impacts between sites in Sweden, highlighting the importance of spatial differentiation of characterisation modelling within the scale of the impact.
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2.
A new method for the spatially differentiated assessment of impacts of airborne pollutants on human health is presented. It is applicable to primary pollutants with linear exposure response functions. This includes the most important primary air pollutants from transportation and energy generation. The article looks at the spatial differentiation of impacts due to emission height and the local population density distribution around the emission site, as has been predicted using a Gaussian plume model. The differentiation due to population density is captured by way of five generic spatial classes: large cities in agglomerations, highly densified districts in agglomerations, cities in urbanized regions, country average districts, and low density rural districts in rural regions. Average impacts are calculated for each class. The method is simple enough to be applied to a large number of emissions within Life Cycle Assessments. It was used to calculate site-dependent exposure efficiencies for a variety of primary pollutants emitted at different heights. For traffic emissions of pollutants with short atmospheric residence times, the exposure efficiencies vary by a factor of 5 across Germany and by a factor of 75 across Europe. This differentiation due to population density decreases significantly with an increasing atmospheric residence time of the pollutants and with an increasing emission height.  相似文献   

3.
Due to a lack of spatial and temporal differentiation in lifecycle assessment (LCA), no environmental concentrations can be predicted. As a consequence, it does not seem possible to evaluate whether a no-effect level is exceeded. Therefore, some LCA studies show a poor relationship between the predicted environmental impact and the expected occurrence of actual environmental impact for impacts of a non-global character. This article discusses possibilities for the inclusion of spatial information in life-cycle impact assessment and provides an outline of a site-dependent approach. The required level of complexity in LCA is analysed. The elements of the cause-effect relationships to be incorporated in characterisation modelling, and the need for spatial and temporal differentiation within each of these elements are discussed. It is argued that the accordance between the impact predicted by LCA and the expected occurrence of actual impact can be improved considerably through the use of a site-dependent approach in impact assessment, and without unacceptable increasing uncertainty. In such an approach, the assessment process is extended with a few general site-parameters.  相似文献   

4.
Background, Aims and Scope Several authors have shown that spatially derived characterisation factors used in life cycle impact assessment (LCIA) can differ widely between different countries in the context of regional impact categories such as acidification or terrestrial eutrophication. Previous methodology studies in Europe have produced country-dependent characterisation factors for acidification and terrestrial eutrophication by using the results of the EMEP and RAINS models and critical loads for Europe. The unprotected ecosystem area (UA) is commonly used as a category indicator in the determination of characterisation factors in those studies. However, the UA indicator is only suitable for large emission changes and it does not result in environmental benefits in terms of characterisation factors if deposition after the emission reduction is still higher than the critical load. For this reason, there is a need to search for a new category indicator type for acidification and terrestrial eutrophying in order to calculate site-dependent characterisation factors. The aim of this study is to explore new site-dependent characterisation factors for European acidifying and eutrophying emissions based on accumulated exceedance (AE) as the category indicator, which integrates both the exceeded area and amount of exceedance. In addition, the results obtained for the AE and UA indicators are compared with each other. Methods The chosen category indicator, accumulated exceedance (AE), was computed according to the calculation methods developed in the work under the United Nations Economic Commission for Europe (UNECE) Convention on Long-range Transboundary Air Pollution (LRTAP). Sulphur and nitrogen depositions to 150x150 km2 grid cells over Europe were calculated by source-receptor matrices derived from the EMEP Lagrangian model of long-range transport of air pollution in Europe. Using the latest critical load data of Europe, the site-dependent characterisation factors for acidification and terrestrial eutrophication were calculated for 35 European countries and 5 sea areas for 2002 emissions and emissions predicted for 2010. In the determination of characterisation factors, the emissions of each country/area were reduced by various amounts in order to find stable characterisation factors. In addition, characterisation errors were calculated for the AE-based characterisation factors. For the comparison, the results based on the use of UA indicator were calculated by 10% and 50% reductions of emissions that corresponded to the common practice used in the previous studies. Results and Discussion The characterisation factors based on the AE indicator were shown to be largely independent of the reduction percentage used to calculate them.. Small changes in emissions (≤100 t) produced the most stable characterisation factors in the case of the AE indicator. The characterisation errors of those characterisation factors were practically zero. This means that the characterisation factors can describe the effects of small changes in national emissions that are mostly looked at in LCAs. The comparison between country-dependent characterisation factors calculated by the AE and UA indicators showed that these two approaches produce differences between characterisation factors for many countries/areas in Europe. The differences were mostly related to the Central and Northern European countries. They were greater for terrestrial eutrophication because the contribution of ammonia emission differ remarkably between the two approaches. The characterisation factors of the AE indicator calculated by the emissions of 2002 were greater than the factors calculated by the predicted emissions for 2010 in almost all countries/sea areas, due to the presumed decrease of acidifying and eutrophying emissions in Europe. Conclusions and Recommendations. In this study, accumulated exceedance was shown to be an appropriate category indicator in LCIA applications for the determination of site-dependent characterisation factors for acidification and terrestrial eutrophication in the context of integrated assessment modelling. In the future, it would be useful to calculate characterisation factors for emissions of separate parts of large countries and sea areas in Europe. In addition, it would also be useful to compare the approach based on the AE indicator with the method of the hazard index, as recommended in the latest CML guidebook.  相似文献   

5.

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DOI: http://dx.doi.org/10.1065/lca2006.04.014

Background, Aims and Scope

In the life cycle of a product, emissions take place at many different locations. The location of the source and its surrounding conditions influence the fate of the emitted pollutant and the subsequent exposure it causes. This source of variation is normally neglected in Life Cycle Impact Assessment (LCIA), although it is well known that the impacts predicted by site-generic LCIA in some cases differ significantly from the actual impacts. Environmental impacts of photochemical ozone (ground-level ozone) depend on parameters with a considerable geographical variability (like emission patterns and population densities). A spatially differentiated characterisation model thus seems relevant.

Methods

and Results. The European RAINS model is applied for calculation of site-dependent characterisation factors for Non-Methane Volatile Organic Compounds (NMVOCs) and nitrogen oxides (NOx) for 41 countries or regions within Europe, and compatible characterisation factors for carbon monoxide (CO) are developed based on expert judgement. These factors are presented for three emission years (1990, 1995 and 2010), and they address human health impacts and vegetation impacts in two separate impacts categories, derived from AOT40 and AOT60 values respectively. Compatible site-generic characterisation factors for NMVOC, NOx, CO and methane (CH4) are calculated as emission-weighted European averages to be applied on emissions for which the location is unknown. The site-generic and site-dependent characterisation factors are part of the EDIP2003 LCIA methodology. The factors are applied in a specific case study, and it is demonstrated how the inclusion of spatial differentiation may alter the results of the photochemical ozone characterisation of life cycle impact assessment.

Discussion

and Conclusions. Compared to traditional midpoint characterisation modelling, this novel approach is spatially resolved and comprises a larger part of the cause-effect chain including exposure assessment and exceeding of threshold values. This positions it closer to endpoint modelling and makes the results easier to interpret. In addition, the developed model allows inclusion of the contributions from NOx, which are ne- glected when applying the traditional approaches based on Photochemical Ozone Creation Potentials (POCPs). The variation in site-dependent characterisation factors is far larger than the variation in POCP factors. It thus seems more important to represent the spatially determined variation in exposure than the difference in POCP among the substances.
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6.
Background, aim, and scope  Traditional life cycle impact assessment methodologies have used aggregated characterization factors, neglecting spatial and temporal variations in regional impacts like photochemical oxidant formation. This increases the uncertainty of the LCA results and diminishes the ease of decision-making. This study compares four common impact assessment methods, CML2001, Eco-indicator 99, TRACI, and EDIP2003, on their underlying models, spatial and temporal resolution, and the level at which photochemical oxidant impacts are calculated. A new characterization model is proposed that incorporates spatial and temporal differentiation. Materials and methods  A photochemical air quality modeling system (CAMx-MM5-SMOKE) is used to simulate the process of formation, transformation, transport, and removal of photochemical pollutants. Monthly characterization factors for individual US states are calculated at three levels along the cause–effect chain, namely, fate level, human and ecosystem exposure level, and human effect level. Results and discussion  The results indicate that a spatial variability of one order of magnitude and a temporal variability of two orders of magnitude exist in both the fate level and human exposure and effect level characterization factors for NOx. The summer time characterization factors for NOx are higher than the winter time factors. However, for anthropogenic VOC, the summer time factors are lower than the winter time in almost half of the states. This is due to the higher emission rates of biogenic VOCs in the summer. The ecosystem exposure factors for NOx and VOC do not follow a regular pattern and show a spatial variation of about three orders of magnitude. They do not show strong correlation with the human exposure factors. Sensitivity analysis has shown that the effect of meteorology and emission inputs is limited to a factor of three, which is several times smaller than the variation seen in the factors. Conclusions  Uncertainties are introduced in the characterization of photochemical precursors due to a failure to consider the spatial and temporal variations. Seasonal variations in photochemical activity influence the characterization factors more than the location of emissions. The human and ecosystem exposures occur through different mechanisms, and impacts calculated at the fate level based only on ozone concentration are not a good indicator for ecosystem impacts. Recommendations and perspectives  Spatial and temporal differentiation account for fate and transport of the pollutant, and the exposure of and effect on the sensitive human population or ecosystem. Adequate resolution for seasonal and regional processes, like photochemical oxidant formation, is important to reduce the uncertainty in impact assessment and improve decision-making power. An emphasis on incorporating some form of spatial and temporal information within standard LCI databases and using adequately resolved characterization factors will greatly increase the fidelity of a standard LCA. Electronic supplementary material  The online version of this article (doi:) contains supplementary material, which is available to authorized users.  相似文献   

7.
Goal, Scope and Background Taking into account the location of emissions and its subsequent, site-dependent impacts improves the accuracy of LCIA. Opponents of site-dependent impact assessment argue that it is too time-consuming to collect the required additional inventory data. In this paper we quantify this time and look into the added value of site-dependent LCIA results. Methods We recalculated the acidifying impact for three existing LCA studies: linoleum, stone wool, and water piping systems. The amount of time needed to collect the required additional data is reported. The EDIP2003 methodology provides site-generic and site-dependent acidification factors. We used these factors to recalculate acidification for the case studies. We analyzed differences between site-generic and site-dependent acidification and reported problems experienced. Results and Discussion Finding the location of processes and emissions was easy. The reports of the three case studies contained most of this information. Far more time was needed to disaggregate processes to the level where emissions can be localized. Although the overall conclusions with regard to acidification did not change in the case studies, the relative importance of processes shifted when considering sub-levels. This is especially important for improvement analysis. Site-dependent acidification assessment was hampered in the linoleum case study where about 40% of the acidification originates from non-European emissions. However, EDIP2003 provides no site-dependent factors for these countries and site-generic factors had to be used instead. Thus, calculating site-dependent acidification is only feasible for LCA studies in which the majority of the emissions originate in Europe. We could not reproduce all parts of the three case studies using the report and additional public resources. This hindered our recalculation. In fact, any additional analysis will be hampered by this lack of reproducibility. ISO recommends such reproducibility for comparative assertion disclosed to the public. Conclusion Spatially differentiated acidification is feasible for each of the three case studies. Finding the location of processes and emissions was easy, but quite some time was needed to disaggregate processes and emissions to the appropriate level. Overall conclusions on acidification remained the same for the case studies, but the relative contribution of basic processes changed when applying site-dependent impact assessment. Though the three case studies were all rather detailed and complete, none of them was fully reproducible. This complicated recalculation of acidification, and will in fact make any additional analysis difficult.  相似文献   

8.
- Part 1: Characterisation factors (DOI: http://dx.doi.org/10.1065/lca2004.12.194.1) Part 2: Damage scores (DOI: http://dx.doi.org/10.1065/lca2004.12.194.2) - Preamble. In this series of two papers, a methodology to calculate damages to human health caused by indoor emissions from building materials is presented and applied. Part 1 presents the theoretical foundation of the indoor emission methodology developed, as well as characterisation factors calculated for 36 organic compounds, radon and gamma radiation. Part 2 calculates damage scores of building materials with the characterisation factors presented in part 1. The relevancy of including indoor air emission in the full damage scores at a material level and a dwelling level is also quantified and discussed. Goal, Scope and Background In industrialized countries such as the Netherlands, the concentration of pollutants originating from building materials in the indoor environment has shown an increasing trend during the last decades due to improved isolation and decreased ventilation of dwellings. These pollutants may give rise to negative impacts on human health, ranging from irritation to tumours. However, such negative impacts on health are not included in current life cycle assessments of dwellings. In this study, damages to the health of occupants caused by a number of organic compounds and by radioactivity emitted by building materials, including those due to indoor exposure, have been calculated for a number of categories of common building materials. The total damage to human health due to emissions occurring in the use phase of the Dutch reference dwelling is compared with the total damage to human health associated with the rest of the life cycle of the same dwelling. Methods Human health damage scores per kilogram of building material for compartments of the Dutch reference dwelling have been calculated using the methodology described in part I of this research. This methodology includes the calculation of the fate, effect and damage factors, based on disability adjusted life years (DALYs), and has been applied assuming average concentrations of pollutants in building materials. Damage scores for health impacts of exposure to pollutants emitted during the production and the disposal phase of the same building materials were calculated using standard LCIA methodology. Results and Discussion Human health damage scores due to emissions of pollutants occurring in the use phase of building materials applied at the first or second floor are up to 20 times lower or higher than the corresponding damage scores associated with the rest of the life cycle of the same building materials. The damage scores due to emissions occurring in the use phase of building materials applied in the crawlspace are up to 105 times lower than those of building materials applied in the other compartments. The total damage to human health due to emissions occurring in the use phase of the Dutch reference dwelling has the same order of magnitude as the total damage to human health associated with the rest of the life cycle of the same dwelling. At a dwelling level, radon and gamma radiation are dominant in the human health damage score among the pollutants studied. Conclusion Health damages due to indoor exposure to contaminants emitted by building materials cannot be neglected for several materials when compared with damage scores associated with the rest of the life cycle of the same building materials. Indoor exposure to pollutants emitted by building materials should be included in the life cycle assessment of dwellings in order to make the assessment better reflect full impact of the life cycle.  相似文献   

9.
- Part 1: Characterisation factors (DOI: http://dx.doi.org/10.1065/lca2004.12.194.1) Part 2: Damage scores (DOI: http://dx.doi.org/10.1065/lca2004.12.194.2) - Preamble. In this series of two papers, a methodology to calculate damages to human health caused by indoor emissions from building materials is presented and applied. Part 1 presents the theoretical foundation of the indoor emission methodology developed, as well as characterisation factors calculated for 36 organic compounds, radon and gamma radiation. Part 2 calculates damage scores of building materials with the characterisation factors presented in part 1. The relevancy of including indoor air emission in the full damage scores at a material level and a dwelling level is also quantified and discussed. Goal, Scope and Background Methodologies based on life cycle assessment have been developed to calculate the environmental impact of dwellings. Human health damage due to exposure to substances emitted to indoor air are not included in these methodologies. In order to compare this damage with human health damages associated with the rest of the life cycle of the dwelling, a methodology has been developed to calculate damages to human health caused by pollutants emitted from building materials. Methods Fate, exposure and health effects are addressed in the calculation procedure. The methodology is suitable for organic substances, radon and elements emitting gamma radiation. The (Dutch reference) dwelling used in the calculation was divided in three compartments: crawl space, first floor and second floor. Fate factors have been calculated based on indoor and outdoor intake fractions, dose conversion factors or extrapolation from measurements. Effect factors have been calculated based on unit risk factors, (extrapolated) effect doses or linear relationship between dose and cancer cases. Damage factors are based on disability adjusted life years (DALYs). Results and Discussion Characterisation factors have been calculated for 36 organic compounds, radon and gamma radiation emitted by building materials applied in a Dutch reference dwelling. For organic compounds and radon, the characterisation factors of emissions to the second floor are 10–20% higher than the characterisation factors of emissions to the first floor. For the first and second floor, the characterisation factors are dominated by damage to human health as a result of indoor exposure. The relative contribution of carcinogenic and non-carcinogenic effects to the characterisation factors is generally within one order of magnitude, and up to three orders of magnitude for formaldehyde. Conclusion Health effects due to indoor exposure to pollutants emitted from building materials appear to be dominant in the characterisation factors over outdoor exposure to such pollutants. The health effects of emissions of organic compounds and gamma radiation in the crawl space are very small compared to the health effects of emissions into the other compartments. Using the characterisation factors calculated in this study, it is possible to calculate the human health damage due to emissions of substances and radiation emitted to indoor air and compare this damage with damages to human health associated with the rest of the life cycle of the material. This is the subject of part II of this research.  相似文献   

10.

Purpose

The inclusion of land-use activities in life cycle assessment (LCA) has been subject to much debate in the LCA community. Despite the recent methodological developments in this area, the impacts of land occupation and transformation on its long-term ability to produce biomass (referred to here as biotic production potential [BPP]) — an important endpoint for the Area of Protection (AoP) Natural Resources — have been largely excluded from LCAs partly due to the lack of life cycle impact assessment methods.

Materials and methods

Several possible methods/indicators for BPP associated with biomass, carbon balance, soil erosion, salinisation, energy, soil biota and soil organic matter (SOM) were evaluated. The latter indicator was considered the most appropriate for LCA, and characterisation factors for eight land use types at the climate region level were developed.

Results and discussion

Most of the indicators assessed address land-use impacts satisfactorily for land uses that include biotic production of some kind (agriculture or silviculture). However, some fail to address potentially important land use impacts from other life cycle stages, such as those arising from transport. It is shown that the change in soil organic carbon (SOC) can be used as an indicator for impacts on BPP, because SOC relates to a range of soil properties responsible for soil resilience and fertility.

Conclusions

The characterisation factors developed suggest that the proposed approach to characterize land use impacts on BBP, despite its limitations, is both possible and robust. The availability of land-use-specific and biogeographically differentiated data on SOC makes BPP impact assessments operational. The characterisation factors provided allow for the assessment of land-use impacts on BPP, regardless of where they occur thus enabling more complete LCAs of products and services. Existing databases on every country’s terrestrial carbon stocks and land use enable the operability of this method. Furthermore, BPP impacts will be better assessed by this approach as increasingly spatially specific data are available for all geographical regions of the world at a large scale. The characterisation factors developed are applied to the case studies (Part D of this special issue), which show the practical issues related to their implementation.  相似文献   

11.

Purpose

A framework for the inclusion of land use impact assessment and a set of land use impact indicators has been recently proposed for life cycle assessment (LCA) and no case studies are available for forest biomass. The proposed methodology is tested for Scandinavian managed forestry; a comparative case study is made for energy from wood, agro-biomass and peat; and sensitivity to forest management options is analysed.

Methods

The functional unit of this comparative case study is 1 GJ of energy in solid fuels. The land use impact assessment framework of the United Nations Environment Programme and the Society of Environmental Toxicology and Chemistry (UNEP-SETAC) is followed and its application for wood biomass is critically analysed. Applied midpoint indicators include ecological footprint and human appropriation of net primary production, global warming potential indicator for biomass (GWPbio-100) and impact indicators proposed by UNEP-SETAC on ecosystem services and biodiversity. Options for forest biomass land inventory modelling are discussed. The system boundary covers only the biomass acquisition phase. Management scenarios are formulated for forest and barley biomass, and a sensitivity analysis focuses on impacts of land transformations for agro-biomass.

Results and discussion

Meaningful differences were found in between solid biofuels from distinct land use classes. The impact indicator results were sensitive to land occupation and transformation and differed significantly from inventory results. Current impact assessment method is not sensitive to land management scenarios because the published characterisation factors are still too coarse and indicate differences only between land use types. All indicators on ecosystem services and biodiversity were sensitive to the assumptions related with land transformation. The land occupation (m2a) approach in inventory was found challenging for Scandinavian wood, due to long rotation periods and variable intensities of harvests. Some suggestions of UNEP-SETAC were challenged for the sake of practicality and relevance for decision support.

Conclusions

Land use impact assessment framework for LCA and life cycle impact assessment (LCIA) indicators could be applied in a comparison of solid bioenergy sources. Although forest bioenergy has higher land occupation than agro-bioenergy, LCIA indicator results are of similar magnitude or even lower for forest bioenergy. Previous literature indicates that environmental impacts of land use are significant, but it remains questionable if these are captured with satisfactory reliability with the applied LCA methodology, especially for forest biomass. Short and long time perspectives of land use impacts should be studied in LCA with characterisation factors for all relevant timeframes, not only 500 years, with a forward-looking perspective. Characterisation factors need to be modelled further for different (forest) land management intensities and for peat excavation.  相似文献   

12.
Throughout their life cycle stages—material production, package manufacture, distribution, end-of-life management—packaging systems consume natural resources and energy, generate waste, and emit pollutants. Each of these stages also carries a financial cost. Motivated by a desire to decrease environmental burdens while reducing financial costs associated with the packaging of accessory and service parts, Toyota Motor Sales (TMS) partnered with the Donald Bren School of Environmental Science & Management to build a life cycle assessment and costing tool to support packaging design decisions. The resulting Environmental Packaging Impact Calculator (EPIC) provides comprehensive life cycle assessment (LCA) and life cycle costing (LCC). It allows packaging designers to identify environmentally and economically preferable packaging systems in daily decision-making. EPIC's parameterized process flow model allows users to assess many different packaging systems using a single model. Its input/output interface is designed for users without preexisting knowledge of LCA theory or practice and calculates results based on relatively few input data. The main motivation behind this environmental design tool is to provide relevant information to those individuals who are in the best position to reduce life cycle impacts and costs from TMS's packaging and distribution systems.  相似文献   

13.

Purpose

Life cycle impact assessment (LCIA) translates emissions and resource extractions into a limited number of environmental impact scores by means of so-called characterisation factors. There are two mainstream ways to derive characterisation factors, i.e. at midpoint level and at endpoint level. To further progress LCIA method development, we updated the ReCiPe2008 method to its version of 2016. This paper provides an overview of the key elements of the ReCiPe2016 method.

Methods

We implemented human health, ecosystem quality and resource scarcity as three areas of protection. Endpoint characterisation factors, directly related to the areas of protection, were derived from midpoint characterisation factors with a constant mid-to-endpoint factor per impact category. We included 17 midpoint impact categories.

Results and discussion

The update of ReCiPe provides characterisation factors that are representative for the global scale instead of the European scale, while maintaining the possibility for a number of impact categories to implement characterisation factors at a country and continental scale. We also expanded the number of environmental interventions and added impacts of water use on human health, impacts of water use and climate change on freshwater ecosystems and impacts of water use and tropospheric ozone formation on terrestrial ecosystems as novel damage pathways. Although significant effort has been put into the update of ReCiPe, there is still major improvement potential in the way impact pathways are modelled. Further improvements relate to a regionalisation of more impact categories, moving from local to global species extinction and adding more impact pathways.

Conclusions

Life cycle impact assessment is a fast evolving field of research. ReCiPe2016 provides a state-of-the-art method to convert life cycle inventories to a limited number of life cycle impact scores on midpoint and endpoint level.
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14.
Background, aim and scope  The methodological choices and framework to assess environmental impacts in life cycle assessment are still under discussion. Despite intensive developments worldwide, few attempts have been made hitherto to systematically present the role of different factors of characterisation models in life cycle impact assessment (LCIA). The aim of this study is to show how European average and country-dependent characterisation factors for acidifying and eutrophying emissions differ when using (a) acidifying and eutrophying potentials alone, (b) depositions from an atmospheric dispersion model or (c) critical loads in conjunction with those depositions. Furthermore, in the latter case, the contributions of emissions, an atmospheric transport model and critical loads to changes in characterisation factors of NO2 are studied. In addition, the new characterisation factors based on the accumulated exceedance (AE) method are presented using updated emissions, a new atmospheric transport model and the latest critical loads. Materials and methods  In this study, characterisation factors for acidifying and eutrophying emissions are calculated by three different methods. In the ‘no fate’ (NF) methods, acidifying and eutrophying potentials alone are considered as characterisation factors. In the ‘only above terrestrial environment’ (OT) approach, characterisation factors are based on the deposition of the acidifying or eutrophying substances to terrestrial land surfaces. The third method is the so-called AE method in which critical loads are used in conjunction with depositions. The results of the methods are compared both at the European and the country level using weighted mean, weighted standard deviation, minimum and maximum values. To illustrate the sensitivity of the AE method, changes in European emissions, employed atmospheric dispersion model and the critical loads database are conducted step-by-step, and the differences between the results are analysed. Results and discussion  For European average characterisation factors, the three characterisation methods of acidification produce results in which the contributions of NH3, NO2 and SO2 to the acidification indicator do not differ much within each method when 1 kg of each acidifying substance is emitted. However, the NF methods cannot describe any spatial aspects of environmental problems. Both OT and AE methods show that the spatial aspects play an important role in the characterisation factors. The AE method results in greater differentiations between country-dependent characterisation factors than does the OT method. In addition, the results of the AE and OT methods differ from each other for individual countries. A major shortcoming of the OT approach is that it does not consider the sensitivity of the ecosystems onto which the pollutants are deposited, whereas the AE approach does. In the case of the AE method, a new atmospheric dispersion model, new information on emissions and critical loads have a different influence on the characterisation factors, depending on the country. The results of statistics show that the change in the atmospheric dispersion model has a greatest influence on the results, since ecosystem-specific depositions are taken into account for the first time. Conclusions and recommendations  The simple NF methods can be used in a first approximation to assess the impacts of acidification and terrestrial eutrophication in cases where we do not know where the emissions occur. The OT approach is a more advanced method compared with the NF method, but its capability to describe spatial aspects is limited. The AE factors are truly impact-oriented characterisation factors and the information used here represents the current best knowledge about the assessment practice of acidification and terrestrial eutrophication in Europe. The key message of this study is that there is no shortcut to achieving advanced characterisation of acidification and terrestrial eutrophication: an advanced methodology cannot develop without atmospheric dispersion models and information on ecosystem sensitivity.  相似文献   

15.

Purpose

As a consequence of the multi-functionality of land, the impact assessment of land use in Life Cycle Impact Assessment requires the modelling of several impact pathways covering biodiversity and ecosystem services. To provide consistency amongst these separate impact pathways, general principles for their modelling are provided in this paper. These are refinements to the principles that have already been proposed in publications by the UNEP-SETAC Life Cycle Initiative. In particular, this paper addresses the calculation of land use interventions and land use impacts, the issue of impact reversibility, the spatial and temporal distribution of such impacts and the assessment of absolute or relative ecosystem quality changes. Based on this, we propose a guideline to build methods for land use impact assessment in Life Cycle Assessment (LCA).

Results

Recommendations are given for the development of new characterization models and for which a series of key elements should explicitly be stated, such as the modelled land use impact pathways, the land use/cover typology covered, the level of biogeographical differentiation used for the characterization factors, the reference land use situation used and if relative or absolute quality changes are used to calculate land use impacts. Moreover, for an application of the characterisation factors (CFs) in an LCA study, data collection should be transparent with respect to the data input required from the land use inventory and the regeneration times. Indications on how generic CFs can be used for the background system as well as how spatial-based CFs can be calculated for the foreground system in a specific LCA study and how land use change is to be allocated should be detailed. Finally, it becomes necessary to justify the modelling period for which land use impacts of land transformation and occupation are calculated and how uncertainty is accounted for.

Discussion

The presented guideline is based on a number of assumptions: Discrete land use types are sufficient for an assessment of land use impacts; ecosystem quality remains constant over time of occupation; time and area of occupation are substitutable; transformation time is negligible; regeneration is linear and independent from land use history and landscape configuration; biodiversity and multiple ecosystem services are independent; the ecological impact is linearly increasing with the intervention; and there is no interaction between land use and other drivers such as climate change. These assumptions might influence the results of land use Life Cycle Impact Assessment and need to be critically reflected.

Conclusions and recommendations

In this and the other papers of the special issue, we presented the principles and recommendations for the calculation of land use impacts on biodiversity and ecosystem services on a global scale. In the framework of LCA, they are mainly used for the assessment of land use impacts in the background system. The main areas for further development are the link to regional ecological models running in the foreground system, relative weighting of the ecosystem services midpoints and indirect land use.  相似文献   

16.
The present work focuses on impact assessment of noise disturbance in the framework of LCA studies. A number of difficulties arose in the course of the study, namely expressing noise measurements in an easy-to-handle unit, imputing disturbance engendered by several simultaneous sources to every single source, handling additive quantities non-linearly, taking into account the space and time dependence of potential impacts associated with noise, It is shown how all these issues were tackled in a I.CA study that assessed different modes of transportation. The methodology developed takes into account the disturbance to noise level exceeding a set threshold and no other kinds of noise effects. It is obvious that disturbance due to noise emissions depends on people density in the neighborhood of the emission source. In this context, a “site-dependent approach” was taken, meaning that we did include local factors into the valuation. The methodology developed in this article may be extended to other types of emissions when it is necessary to integrate local factors in the assessment phase of LCA. This document is the property of Ecobilan and can not be reproduced without its prior authorization  相似文献   

17.
Goal, Scope and Background Canadian LCA practitioners currently use European or American methodologies when conducting comprehensive impact assessments, despite the fact that these methods may not be appropriate for Canadian conditions. Due to the lack of suitable models that are currently available, work has been undertaken to develop an LCIA method by adapting existing LCIA models to the Canadian context. This new method allows the characterization of 10 impact categories. Methods This project is strongly based on preliminary outcomes from SETAC recommendations for the best available practices in LCIA. Models from 3 recent LCIA site-dependent methods, EDIP2003, IMPACT2002+ and TRACI, were used in this midpoint Canadian-specific method. Characterization models were chosen based on their level of comprehensiveness, scientific sophistication and the possibility of integrating site-specific values in the models. Results and Discussion All regional and local impact categories in the method are site-differentiated. For aquatic eutrophication, (eco)toxicity and land-use impact categories, regionally-differentiated models taking into account fate and effect were already available: the parameters of these models were modified for the Canadian context. For acidification, aquatic and terrestrial eutrophication, existing models were spatially differentiated for fate: regionalization of the effect factor was also included, based on the level of sensitivity of each ecozone assessed with vulnerability factors. The default spatial resolution selected for this method was Canadian ecozones, which define spaces in an ecologically meaningful way where organisms and their physical environment evolve as a system. For each ecozone, 2334 site-dependent characterization factors have been calculated. Conclusion This LCIA methodology proposes an attractive and useful set of site-dependent characterization factors for the 15 Canadian terrestrial ecozones. Recommendation and Outlook Efforts are being carried out to extend the specificity of some factors used in eutrophication modelization. Finally, the transparency of the methodology will allow to re-calculate site-dependent characterization factors for different regions and for additional substances.  相似文献   

18.
The status of Life Cycle Assessment (LCA) activities in the Nordic Region (period 1995-97) is presented, based on more than 350 reported studies from industrial companies and research institutes in Sweden, Denmark, Norway, and Finland. A large number of industrial sectors is represented, with car components, building materials, pulp and paper products, electronic components and packaging as the most important ones. All aspects of LCA methodology are used: 90% use impact assessment, 80% impact assessment and valuation step. In most studies, more than one valuation method is used for ranking environmental impacts. LCA studies are well integrated in the business activities in many large Nordic corporations. From the early attempts, more familiar with LCA methodology, LCA has been integrated in strategy development, product development, process development and, to some extent, marketing. LCA has not only been used in the strict sense presented in the ISO 14040-43 standards. The systems approach, which is the basis for LCA, has also been modified and used in Sustainable Product Development, and in Environmental Performance Indicator and Product Declarations development. Future applications should be within Environmental Impact Assessments.  相似文献   

19.
The status of Life Cycle Assessment (LCA) activities in the Nordic Region (period 1995-97) is presented, based on more than 350 reported studies from industrial companies and research institutes in Sweden, Denmark, Norway, and Finland. A large number of industrial sectors is represented, with car components, building materials, pulp and paper products, electronic components and packaging as the most important ones. All aspects of LCA methodology are used: 90% use impact assessment, 80% impact assessment and valuation step. In most studies, more than one valuation method is used for ranking environmental impacts. LCA studies are well integrated in the business activities in many large Nordic corporations. From the early attempts, more familiar with LCA methodology, LCA has been integrated in strategy development, product development, process development and, to some extent, marketing. LCA has not only been used in the strict sense presented in the ISO 14040-43 standards. The systems approach, which is the basis for LCA, has also been modified and used in Sustainable Product Development, and in Environmental Performance Indicator and Product Declarations development. Future applications should be within Environmental Impact Assessments.  相似文献   

20.

Purpose

Rarely considered in environmental assessment methods, potential land use impacts on a series of ecosystem services must be accounted for in widely used decision-making tools such as life cycle assessment (LCA). The main goal of this study is to provide an operational life cycle impact assessment characterization method that addresses land use impacts at a global scale by developing spatially differentiated characterization factors (CFs) and assessing the extent of their spatial variability using different regionalization levels.

Methods

The proposed method follows the recommendations of previous work and falls within the framework and principles for land use impact assessment established by the United Nations Environment Programme/Society of Environmental Toxicology and Chemistry Life Cycle Initiative. Based on the spatial approach suggested by Saad et al. (Int J Life Cycle Assess 16: 198–211, 2011), the intended impact pathways that are modeled pertain to impacts on ecosystem services damage potential and focus on three major ecosystem services: (1) erosion regulation potential, (2) freshwater regulation potential, and (3) water purification potential. Spatially-differentiated CFs were calculated for each biogeographic region of all three regionalization scale (Holdridge life regions, Holdridge life zones, and terrestrial biomes) along with a nonspatial world average level. In addition, seven land use types were assessed considering both land occupation and land transformation interventions.

Results and discussion

A comprehensive analysis of the results indicates that, when compared to all resolution schemes, the world generic averaged CF can deviate for various ecosystem types. In the case of groundwater recharge potential impacts, this range varied up to factors of 7, 4.7, and 3 when using the Holdridge life zones, the Holdridge regions, and the terrestrial biomes regionalization levels, respectively. This validates the importance of introducing a regionalized assessment and highlights how a finer scale increases the level of detail and consequently the discriminating power across several biogeographic regions, which could not have been captured using a coarser scale. In practice, the implementation of such regionalized CFs suggests that an LCA practitioner must identify the ecosystem in which land occupation or transformation activities occur in addition to the traditional inventory data required—namely, the land use activity and the inventory flow.

Conclusions

The variability of CFs across all three regionalization levels provides an indication of the uncertainty linked to nonspatial CFs. Among other assumptions and value choices made throughout the study, the use of ecological borders over political boundaries was deemed more relevant to the interpretation of environmental issues related to specific functional ecosystem behaviors.  相似文献   

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